Charge‐Rearrangement Averaged Dye Design for Precise, Real‐Time, and Portable Monitoring of Complex Solvent Environments
Although solvatochromic materials provide visual function to differentiate solvents, they fail to precisely monitor complex solvent environments where solvent composition varies dynamically, because of an insensitive absorptional shift in these environments. Relatively, their fluorescence signal cha...
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| Published in | Angewandte Chemie International Edition |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
22.08.2025
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| Abstract | Although solvatochromic materials provide visual function to differentiate solvents, they fail to precisely monitor complex solvent environments where solvent composition varies dynamically, because of an insensitive absorptional shift in these environments. Relatively, their fluorescence signal change, which should be more sensitive, has always been inefficient, resulting from inherent challenges in excited‐state dynamics. Here, we present a charge‐rearrangement averaged dye design, instead of traditional donor‐acceptor structures, to enable a high locally excited or twisted intramolecular charge transfer emission efficiency. A ratiometric dual‐fluorescence behavior can be observed along with a solvent‐dependent emission trade‐off rather than complete quenching. In this case, the dyes can not only precisely visualize various mixed solvents but also enable heterogeneous detection with over hundreds of reuse cycles after being integrated into a crosslinked polymer. The leading portable material achieves a self‐calibrated visual tracking of ethanol content (error<0.2%) with a robust working curve ( R 2 = 0.9992) while applied to E10 ethanol gasoline, operable via user‐friendly software analysis through mobile phone photography. |
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| AbstractList | Although solvatochromic materials provide visual function to differentiate solvents, they fail to precisely monitor complex solvent environments where solvent composition varies dynamically, because of an insensitive absorptional shift in these environments. Relatively, their fluorescence signal change, which should be more sensitive, has always been inefficient, resulting from inherent challenges in excited‐state dynamics. Here, we present a charge‐rearrangement averaged dye design, instead of traditional donor‐acceptor structures, to enable a high locally excited or twisted intramolecular charge transfer emission efficiency. A ratiometric dual‐fluorescence behavior can be observed along with a solvent‐dependent emission trade‐off rather than complete quenching. In this case, the dyes can not only precisely visualize various mixed solvents but also enable heterogeneous detection with over hundreds of reuse cycles after being integrated into a crosslinked polymer. The leading portable material achieves a self‐calibrated visual tracking of ethanol content (error<0.2%) with a robust working curve ( R 2 = 0.9992) while applied to E10 ethanol gasoline, operable via user‐friendly software analysis through mobile phone photography. |
| Author | Li, Zhongyu Shen, Shen Sahoo, Smruti R. Zhang, Man Ågren, Hans Baryshnikov, Gleb Zhu, Liangliang Sun, Hao |
| Author_xml | – sequence: 1 givenname: Zhongyu surname: Li fullname: Li, Zhongyu organization: State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular Science Fudan University Shanghai 200438 China – sequence: 2 givenname: Smruti R. surname: Sahoo fullname: Sahoo, Smruti R. organization: Laboratory of Organic Electronics Department of Science and Technology Linköping University Norrköping 60174 Sweden, Department of Physics and Astronomy Uppsala University Box 516 Uppsala SE‐751 20 Sweden – sequence: 3 givenname: Shen surname: Shen fullname: Shen, Shen organization: State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular Science Fudan University Shanghai 200438 China – sequence: 4 givenname: Hao surname: Sun fullname: Sun, Hao organization: State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular Science Fudan University Shanghai 200438 China – sequence: 5 givenname: Hans surname: Ågren fullname: Ågren, Hans organization: Department of Physics and Astronomy Uppsala University Box 516 Uppsala SE‐751 20 Sweden – sequence: 6 givenname: Man surname: Zhang fullname: Zhang, Man organization: State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular Science Fudan University Shanghai 200438 China – sequence: 7 givenname: Gleb surname: Baryshnikov fullname: Baryshnikov, Gleb organization: Laboratory of Organic Electronics Department of Science and Technology Linköping University Norrköping 60174 Sweden – sequence: 8 givenname: Liangliang orcidid: 0000-0001-6268-3351 surname: Zhu fullname: Zhu, Liangliang organization: State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular Science Fudan University Shanghai 200438 China |
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