Cu 3 (hexaiminotriphenylene) 2 : An Electrically Conductive 2D Metal–Organic Framework for Chemiresistive Sensing
The utility of metal–organic frameworks (MOFs) as functional materials in electronic devices has been limited to date by a lack of MOFs that display high electrical conductivity. Here, we report the synthesis of a new electrically conductive 2D MOF, Cu 3 (HITP) 2 (HITP=2,3,6,7,10,11‐hexaiminotriphen...
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| Published in | Angewandte Chemie (International ed.) Vol. 54; no. 14; pp. 4349 - 4352 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
Wiley
27.03.2015
|
| Subjects | |
| Online Access | Get full text |
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| Abstract | The utility of metal–organic frameworks (MOFs) as functional materials in electronic devices has been limited to date by a lack of MOFs that display high electrical conductivity. Here, we report the synthesis of a new electrically conductive 2D MOF, Cu
3
(HITP)
2
(HITP=2,3,6,7,10,11‐hexaiminotriphenylene), which displays a bulk conductivity of 0.2 S cm
−1
(pellet, two‐point‐probe). Devices synthesized by simple drop casting of Cu
3
(HITP)
2
dispersions function as reversible chemiresistive sensors, capable of detecting sub‐ppm levels of ammonia vapor. Comparison with the isostructural 2D MOF Ni
3
(HITP)
2
shows that the copper sites are critical for ammonia sensing, indicating that rational design/synthesis can be used to tune the functional properties of conductive MOFs. |
|---|---|
| AbstractList | The utility of metal–organic frameworks (MOFs) as functional materials in electronic devices has been limited to date by a lack of MOFs that display high electrical conductivity. Here, we report the synthesis of a new electrically conductive 2D MOF, Cu
3
(HITP)
2
(HITP=2,3,6,7,10,11‐hexaiminotriphenylene), which displays a bulk conductivity of 0.2 S cm
−1
(pellet, two‐point‐probe). Devices synthesized by simple drop casting of Cu
3
(HITP)
2
dispersions function as reversible chemiresistive sensors, capable of detecting sub‐ppm levels of ammonia vapor. Comparison with the isostructural 2D MOF Ni
3
(HITP)
2
shows that the copper sites are critical for ammonia sensing, indicating that rational design/synthesis can be used to tune the functional properties of conductive MOFs. |
| Author | Liu, Sophie F. Dincă, Mircea Campbell, Michael G. Sheberla, Dennis Swager, Timothy M. |
| Author_xml | – sequence: 1 givenname: Michael G. surname: Campbell fullname: Campbell, Michael G. – sequence: 2 givenname: Dennis surname: Sheberla fullname: Sheberla, Dennis – sequence: 3 givenname: Sophie F. surname: Liu fullname: Liu, Sophie F. – sequence: 4 givenname: Timothy M. surname: Swager fullname: Swager, Timothy M. – sequence: 5 givenname: Mircea surname: Dincă fullname: Dincă, Mircea |
| BackLink | https://www.osti.gov/biblio/1385576$$D View this record in Osti.gov |
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| Title | Cu 3 (hexaiminotriphenylene) 2 : An Electrically Conductive 2D Metal–Organic Framework for Chemiresistive Sensing |
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