Multistep optimization for the electrodeposited mixed perovskite FA 1−y Cs y PbBr x I 3−x solar cells
The electrodeposition method has recently been developed for the fabrication of perovskite solar cells due to its potential advantages in commercial preparation. However, there is few studies on the preparation of perovskite solar cells by the electrodeposition method, especially on the perovskite F...
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| Published in | Nanotechnology Vol. 35; no. 1; p. 15706 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
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01.01.2024
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| Abstract | The electrodeposition method has recently been developed for the fabrication of perovskite solar cells due to its potential advantages in commercial preparation. However, there is few studies on the preparation of perovskite solar cells by the electrodeposition method, especially on the perovskite FAPbI 3 -based solar cells. Herein, we fabricated the mixed perovskite FA 1− y Cs y PbBr x I 3− x solar cells by an optimized electrodeposition method, in which the electrodeposited PbO 2 reacts directly with FAI and an appropriate amount of CsBr dopants. The corresponding solar cells display the best PCE of 4.97%. By regulating the growth temperature in the reaction between PbO 2 and FAI/CsBr, the efficiency of the mixed perovskite solar cells can be promoted to 10.18%. These results illustrate that the element doping and growth environment regulation can optimize the quality of the perovskite films, thus promoting the efficiency of the perovskite solar cells. With further optimizing the growth process in the electrodeposition method, it is expected to open up a new commercial preparation route for the perovskite solar cells in the near future. |
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| AbstractList | The electrodeposition method has recently been developed for the fabrication of perovskite solar cells due to its potential advantages in commercial preparation. However, there is few studies on the preparation of perovskite solar cells by the electrodeposition method, especially on the perovskite FAPbI
-based solar cells. Herein, we fabricated the mixed perovskite FA
Cs
PbBr
I
solar cells by an optimized electrodeposition method, in which the electrodeposited PbO
reacts directly with FAI and an appropriate amount of CsBr dopants. The corresponding solar cells display the best PCE of 4.97%. By regulating the growth temperature in the reaction between PbO
and FAI/CsBr, the efficiency of the mixed perovskite solar cells can be promoted to 10.18%. These results illustrate that the element doping and growth environment regulation can optimize the quality of the perovskite films, thus promoting the efficiency of the perovskite solar cells. With further optimizing the growth process in the electrodeposition method, it is expected to open up a new commercial preparation route for the perovskite solar cells in the near future. The electrodeposition method has recently been developed for the fabrication of perovskite solar cells due to its potential advantages in commercial preparation. However, there is few studies on the preparation of perovskite solar cells by the electrodeposition method, especially on the perovskite FAPbI 3 -based solar cells. Herein, we fabricated the mixed perovskite FA 1− y Cs y PbBr x I 3− x solar cells by an optimized electrodeposition method, in which the electrodeposited PbO 2 reacts directly with FAI and an appropriate amount of CsBr dopants. The corresponding solar cells display the best PCE of 4.97%. By regulating the growth temperature in the reaction between PbO 2 and FAI/CsBr, the efficiency of the mixed perovskite solar cells can be promoted to 10.18%. These results illustrate that the element doping and growth environment regulation can optimize the quality of the perovskite films, thus promoting the efficiency of the perovskite solar cells. With further optimizing the growth process in the electrodeposition method, it is expected to open up a new commercial preparation route for the perovskite solar cells in the near future. |
| Author | Li, Chunhe Zheng, Ren Ren, Kuankuan Fang, Zebo Shi, Biyun Xiang, Yanhong Liu, Shiyan Ye, Qiufeng |
| Author_xml | – sequence: 1 givenname: Yanhong surname: Xiang fullname: Xiang, Yanhong – sequence: 2 givenname: Ren surname: Zheng fullname: Zheng, Ren – sequence: 3 givenname: Chunhe surname: Li fullname: Li, Chunhe – sequence: 4 givenname: Kuankuan orcidid: 0000-0003-4180-7348 surname: Ren fullname: Ren, Kuankuan – sequence: 5 givenname: Qiufeng surname: Ye fullname: Ye, Qiufeng – sequence: 6 givenname: Biyun surname: Shi fullname: Shi, Biyun – sequence: 7 givenname: Shiyan surname: Liu fullname: Liu, Shiyan – sequence: 8 givenname: Zebo surname: Fang fullname: Fang, Zebo |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/37788663$$D View this record in MEDLINE/PubMed |
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| CitedBy_id | crossref_primary_10_1088_1361_6528_ad3251 crossref_primary_10_1016_j_jallcom_2024_177648 |
| Cites_doi | 10.1002/adfm.201606156 10.1016/j.solener.2020.07.020 10.1021/acs.jpcc.0c11259 10.1016/j.jallcom.2023.169104 10.1016/j.solener.2022.01.064 10.1021/acs.chemmater.1c04021 10.1039/D0EE00385A 10.1002/solr.202100993 10.1016/j.mtadv.2022.100232 10.1016/j.jpowsour.2017.12.075 10.1021/acs.energyfuels.2c04035 10.1021/acs.chemmater.5b03169 10.1038/s41586-022-05346-0 10.1002/solr.202000455 10.1021/acsami.0c09485 10.1038/s41578-023-00582-w 10.1039/d0cs01272f 10.1038/srep15889 10.1002/solr.202200345 10.1039/C9CS00711C 10.1002/solr.202101035 10.1002/solr.202200777 10.1002/smll.202300374 10.1016/j.cej.2021.128460 10.1016/j.ccr.2020.213633 10.1021/acsami.5b07222 10.1021/acs.chemrev.8b00318 10.1038/nmat4014 10.1038/s41598-018-20296-2 10.1039/C9TA12032G 10.1021/acsaem.1c04063 10.1016/j.electacta.2017.06.104 10.1021/acs.chemrev.8b00539 10.1021/acs.chemmater.5b04524 10.1016/j.nanoen.2015.04.025 10.1021/acsomega.6b00351 10.1016/j.mtener.2020.100449 10.1007/s10854-019-02438-y 10.1002/gch2.201900050 10.1021/acs.jpcc.8b05008 |
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| Keywords | mixed perovskite solar cells FA1−y Cs y PbBr x I3−x electrodeposition |
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