Ion Sieve: Tailoring Zn 2+ Desolvation Kinetics and Flux toward Dendrite-Free Metallic Zinc Anodes
Tip-induced dendrites on metallic zinc anodes (MZAs) fundamentally deteriorate the rechargeability of aqueous Zn metal batteries (ZMBs). Herein, an intriguing ion sieve (IS) consisting of 3D intertwined bacterial cellulose, deposited on the surface of MZAs (Zn@IS) through an in situ self-assembly ro...
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| Published in | ACS nano Vol. 16; no. 1; pp. 1013 - 1024 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
25.01.2022
|
| Subjects | |
| Online Access | Get full text |
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| Abstract | Tip-induced dendrites on metallic zinc anodes (MZAs) fundamentally deteriorate the rechargeability of aqueous Zn metal batteries (ZMBs). Herein, an intriguing ion sieve (IS) consisting of 3D intertwined bacterial cellulose, deposited on the surface of MZAs (Zn@IS) through an in situ self-assembly route, is first presented to be effective in inhibiting dendrite-growth on MZAs. Experimental analyses together with theoretical calculations suggested that the IS coating can facilitate the desolvation of [Zn(H
O)
]
clusters via a strong interplay with Zn ions, weaken hydrogen evolution reaction of MZAs, and homogenize the ion flux with the abundant nanopores serving as ion tunnels, synergistically enabling dendrite-free Zn deposition on the Zn@IS anodes. Consequently, a lifespan up to 3000 h at a cutoff capacity of 0.25 mA h cm
was observed in a Zn@IS
Zn@IS symmetric cell. In terms of application, pairing with a carbon-nanotube@MnO
cathode as an example, the full ZMBs acquired enhanced rechargeability with much higher capacity retention over 73.3% after 3000 cycles compared to the counterpart with pristine MZA (21%). |
|---|---|
| AbstractList | Tip-induced dendrites on metallic zinc anodes (MZAs) fundamentally deteriorate the rechargeability of aqueous Zn metal batteries (ZMBs). Herein, an intriguing ion sieve (IS) consisting of 3D intertwined bacterial cellulose, deposited on the surface of MZAs (Zn@IS) through an in situ self-assembly route, is first presented to be effective in inhibiting dendrite-growth on MZAs. Experimental analyses together with theoretical calculations suggested that the IS coating can facilitate the desolvation of [Zn(H
O)
]
clusters via a strong interplay with Zn ions, weaken hydrogen evolution reaction of MZAs, and homogenize the ion flux with the abundant nanopores serving as ion tunnels, synergistically enabling dendrite-free Zn deposition on the Zn@IS anodes. Consequently, a lifespan up to 3000 h at a cutoff capacity of 0.25 mA h cm
was observed in a Zn@IS
Zn@IS symmetric cell. In terms of application, pairing with a carbon-nanotube@MnO
cathode as an example, the full ZMBs acquired enhanced rechargeability with much higher capacity retention over 73.3% after 3000 cycles compared to the counterpart with pristine MZA (21%). |
| Author | Fu, Jimin Jiao, Shangqing Hua, Tao Wu, Mingzai Hu, Haibo |
| Author_xml | – sequence: 1 givenname: Shangqing surname: Jiao fullname: Jiao, Shangqing organization: School of Materials Science and Engineering, Key Laboratory of Structure and Functional Regulation of Hybrid Materials, Ministry of Education, Anhui University, Hefei 230601, China – sequence: 2 givenname: Jimin surname: Fu fullname: Fu, Jimin organization: Nanotechnology Center, Institute of Textiles & Clothing, The Hong Kong Polytechnic University, Hung Hom, Kowloon, Hong Kong 999077, China – sequence: 3 givenname: Mingzai orcidid: 0000-0002-1938-7730 surname: Wu fullname: Wu, Mingzai organization: School of Materials Science and Engineering, Key Laboratory of Structure and Functional Regulation of Hybrid Materials, Ministry of Education, Anhui University, Hefei 230601, China – sequence: 4 givenname: Tao orcidid: 0000-0001-9596-5830 surname: Hua fullname: Hua, Tao organization: Nanotechnology Center, Institute of Textiles & Clothing, The Hong Kong Polytechnic University, Hung Hom, Kowloon, Hong Kong 999077, China – sequence: 5 givenname: Haibo orcidid: 0000-0001-7494-1469 surname: Hu fullname: Hu, Haibo organization: School of Materials Science and Engineering, Key Laboratory of Structure and Functional Regulation of Hybrid Materials, Ministry of Education, Anhui University, Hefei 230601, China |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/34918920$$D View this record in MEDLINE/PubMed |
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| Keywords | desolvation kinetics Zn dendrites Zn metal battery ion sieve bacterial cellulose |
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| Snippet | Tip-induced dendrites on metallic zinc anodes (MZAs) fundamentally deteriorate the rechargeability of aqueous Zn metal batteries (ZMBs). Herein, an intriguing... |
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| Title | Ion Sieve: Tailoring Zn 2+ Desolvation Kinetics and Flux toward Dendrite-Free Metallic Zinc Anodes |
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