Olivine‐Type MgMn 0.5 Zn 0.5 SiO 4 Cathode for Mg‐Batteries: Experimental Studies and First Principles Calculations
Magnesium driven reaction in olivine‐type MgMn 0.5 Zn 0.5 SiO 4 structure is subject of study by experimental tests and density functional theory (DFT) calculations. The partial replacement of Mn in Oh sites by other divalent metal such as Zn to get MgMn 0.5 Zn 0.5 SiO 4 cathode is successfully deve...
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| Published in | Small (Weinheim an der Bergstrasse, Germany) Vol. 19; no. 12; p. e2206010 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
01.03.2023
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1613-6810 1613-6829 |
| DOI | 10.1002/smll.202206010 |
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| Abstract | Magnesium driven reaction in olivine‐type MgMn
0.5
Zn
0.5
SiO
4
structure is subject of study by experimental tests and density functional theory (DFT) calculations. The partial replacement of Mn in Oh sites by other divalent metal such as Zn to get MgMn
0.5
Zn
0.5
SiO
4
cathode is successfully developed by a simple sol–gel method. Its comparison with the well‐known MgMnSiO
4
olivine‐type structure with (Mg)
M1
(Mn)
M2
SiO
4
cations distribution serves as the basis of this study to understand the structure, and the magnesium extraction/insertion properties of novel olivine‐type (Mg)
M1
(Mn
0.5
Zn
0.5
)
M2
SiO
4
composition. This work foresees to extend the study to others divalent elements in olivine‐type (Mg)
M1
(Mn
0.5
M
0.5
)
M2
SiO
4
structure with M = Fe, Ca, Mg, and Ni by DFT calculations. The obtained results indicate that the energy density can be attuned between 520 and 440 W h kg
−1
based on two properties of atomic weight and redox chemistry. The presented results commit to open new paths toward development of cathodes materials for Mg batteries. |
|---|---|
| AbstractList | Magnesium driven reaction in olivine-type MgMn
Zn
SiO
structure is subject of study by experimental tests and density functional theory (DFT) calculations. The partial replacement of Mn in Oh sites by other divalent metal such as Zn to get MgMn
Zn
SiO
cathode is successfully developed by a simple sol-gel method. Its comparison with the well-known MgMnSiO
olivine-type structure with (Mg)
(Mn)
SiO
cations distribution serves as the basis of this study to understand the structure, and the magnesium extraction/insertion properties of novel olivine-type (Mg)
(Mn
Zn
)
SiO
composition. This work foresees to extend the study to others divalent elements in olivine-type (Mg)
(Mn
M
)
SiO
structure with M = Fe, Ca, Mg, and Ni by DFT calculations. The obtained results indicate that the energy density can be attuned between 520 and 440 W h kg
based on two properties of atomic weight and redox chemistry. The presented results commit to open new paths toward development of cathodes materials for Mg batteries. Magnesium driven reaction in olivine‐type MgMn 0.5 Zn 0.5 SiO 4 structure is subject of study by experimental tests and density functional theory (DFT) calculations. The partial replacement of Mn in Oh sites by other divalent metal such as Zn to get MgMn 0.5 Zn 0.5 SiO 4 cathode is successfully developed by a simple sol–gel method. Its comparison with the well‐known MgMnSiO 4 olivine‐type structure with (Mg) M1 (Mn) M2 SiO 4 cations distribution serves as the basis of this study to understand the structure, and the magnesium extraction/insertion properties of novel olivine‐type (Mg) M1 (Mn 0.5 Zn 0.5 ) M2 SiO 4 composition. This work foresees to extend the study to others divalent elements in olivine‐type (Mg) M1 (Mn 0.5 M 0.5 ) M2 SiO 4 structure with M = Fe, Ca, Mg, and Ni by DFT calculations. The obtained results indicate that the energy density can be attuned between 520 and 440 W h kg −1 based on two properties of atomic weight and redox chemistry. The presented results commit to open new paths toward development of cathodes materials for Mg batteries. |
| Author | Ortiz, Gregorio F. Pérez‐Vicente, Carlos Liang, Ziteng Ruiz, Rafaela Rubio, Saúl Zuo, Wenhua Yang, Yong |
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| Keywords | MgMn 0.5Zn 0.5SiO 4 density functional theory (DFT) magnesium olivine silicate batteries |
| Language | English |
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| Snippet | Magnesium driven reaction in olivine‐type MgMn
0.5
Zn
0.5
SiO
4
structure is subject of study by experimental tests and density functional theory (DFT)... Magnesium driven reaction in olivine-type MgMn Zn SiO structure is subject of study by experimental tests and density functional theory (DFT) calculations. The... |
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| Title | Olivine‐Type MgMn 0.5 Zn 0.5 SiO 4 Cathode for Mg‐Batteries: Experimental Studies and First Principles Calculations |
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