Comprehensive Review of P2-Type Na 2/3 Ni 1/3 Mn 2/3 O 2 , a Potential Cathode for Practical Application of Na-Ion Batteries

P2-type Na Ni Mn O is a promising cathode material for practical applications in Na-ion batteries, due to its high energy density, high volumetric capacity, excellent Na ion conductivity, ease of synthesis, and good stability in air. Yet, it is subject to structural rearrangements on charging to hig...

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Published inACS applied materials & interfaces Vol. 11; no. 25; pp. 22051 - 22066
Main Authors Zhang, Jiaolong, Wang, Wenhui, Wang, Wei, Wang, Shuwei, Li, Baohua
Format Journal Article
LanguageEnglish
Published United States 26.06.2019
Subjects
Na/vacancy ordering
surface modification
structural transformation
P2-NaNiMnO
cathode
cation substitution
Na-ion batteries
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Abstract P2-type Na Ni Mn O is a promising cathode material for practical applications in Na-ion batteries, due to its high energy density, high volumetric capacity, excellent Na ion conductivity, ease of synthesis, and good stability in air. Yet, it is subject to structural rearrangements on charging to high voltage/low Na content and Na /vacancy ordering transitions, which lead to poor reversibility and dramatic capacity decay upon cycling. In this Review, we present the latest advances related to Na Ni Mn O , with a main focus on strategies to stabilize the structural framework and improve the electrochemical properties. Practical issues and challenges are also proposed on the basis of current research status and progress.
AbstractList P2-type Na Ni Mn O is a promising cathode material for practical applications in Na-ion batteries, due to its high energy density, high volumetric capacity, excellent Na ion conductivity, ease of synthesis, and good stability in air. Yet, it is subject to structural rearrangements on charging to high voltage/low Na content and Na /vacancy ordering transitions, which lead to poor reversibility and dramatic capacity decay upon cycling. In this Review, we present the latest advances related to Na Ni Mn O , with a main focus on strategies to stabilize the structural framework and improve the electrochemical properties. Practical issues and challenges are also proposed on the basis of current research status and progress.
Author Li, Baohua
Wang, Wenhui
Zhang, Jiaolong
Wang, Wei
Wang, Shuwei
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  givenname: Wei
  surname: Wang
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  organization: Engineering Laboratory for the Next Generation Power and Energy Storage Batteries, Graduate School at Shenzhen, Tsinghua University, Shenzhen 518055, China
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  givenname: Shuwei
  surname: Wang
  fullname: Wang, Shuwei
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  surname: Li
  fullname: Li, Baohua
  organization: Engineering Laboratory for the Next Generation Power and Energy Storage Batteries, Graduate School at Shenzhen, Tsinghua University, Shenzhen 518055, China
BackLink https://www.ncbi.nlm.nih.gov/pubmed/31136141$$D View this record in MEDLINE/PubMed
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Keywords Na/vacancy ordering
surface modification
structural transformation
P2-NaNiMnO
cathode
cation substitution
Na-ion batteries
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Snippet P2-type Na Ni Mn O is a promising cathode material for practical applications in Na-ion batteries, due to its high energy density, high volumetric capacity,...
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Title Comprehensive Review of P2-Type Na 2/3 Ni 1/3 Mn 2/3 O 2 , a Potential Cathode for Practical Application of Na-Ion Batteries
URI https://www.ncbi.nlm.nih.gov/pubmed/31136141
Volume 11
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