A pyrene-based hydrogen-bonded framework with excimer induced ratiometric emission for discriminative luminescence detection of metal ions

Discriminatory fluorescence detection of various metal ions is of significant importance in environmental and health-related applications. A luminescent hydrogen-bonded organic framework (HOF) material, PFC-1 was synthesized using 1,3,6,8-tetra(4-carboxylbenzene) pyrene (H4TBAPy) as the organic buil...

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Published inMicroporous and mesoporous materials Vol. 381; p. 113348
Main Authors Shen, Penglei, Xu, Hui, Zhao, Tao, Zhang, Wei, Bai, Gongxun, Alshahrani, Thamraa, Chen, Banglin, Gao, Junkuo, Xu, Shiqing
Format Journal Article
LanguageEnglish
Published Elsevier Inc 01.01.2025
Subjects
Discriminative sensing
Excimer
Fluorescence sensor
Hydrogen-bonded organic frameworks (HOFs)
Metal ions
Fluorescence sensor
Discriminative sensing
Hydrogen-bonded organic frameworks (HOFs)
Excimer
Metal ions
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Abstract Discriminatory fluorescence detection of various metal ions is of significant importance in environmental and health-related applications. A luminescent hydrogen-bonded organic framework (HOF) material, PFC-1 was synthesized using 1,3,6,8-tetra(4-carboxylbenzene) pyrene (H4TBAPy) as the organic building block. The fluorescence behavior of PFC-1 is influenced by the concentration of the suspension, demonstrating different emissions characteristic of monomer and excimer fluorescence, which are highly sensitive to the surrounding environment. This allows for the potential differentiation and sensing of different target analytes. PFC-1 showed discriminatory fluorescence sensing performance towards metal ions such as Al3+, Sc3+, Cr3+, and Cu2+, with changes in fluorescence intensity, emission peak shifts, and intensity ratio changes between monomer and excimer emissions. Furthermore, a smartphone-based detection strategy was proposed, leveraging color recognition capabilities of smartphones for onsite and real-time sensing. The work demonstrate that PFC-1 is a promising material for the development of portable, cost-effective fluorescent sensors for onsite and real-time detection of metal ions. The integration of PFC-1 with smartphone technology paves the way for practical applications in environmental monitoring, industrial processes, and healthcare diagnostics. Discriminatory fluorescence detection of different metal ions is realized by a luminescent HOF PFC-1 with different emissions characteristic of monomer and excimer fluorescence, which are highly sensitive to the metal ions Fe3+, Al3+, Sc3+, Cr3+, and Cu2+. [Display omitted] •A luminescent HOF material PFC-1 was constructed and showed monomer and excimer fluorescence behavior.•PFC-1 showed discriminatory fluorescence sensing performance towards different metal ions.•A smartphone-based detection strategy was realized for onsite and real-time sensing.
AbstractList Discriminatory fluorescence detection of various metal ions is of significant importance in environmental and health-related applications. A luminescent hydrogen-bonded organic framework (HOF) material, PFC-1 was synthesized using 1,3,6,8-tetra(4-carboxylbenzene) pyrene (H4TBAPy) as the organic building block. The fluorescence behavior of PFC-1 is influenced by the concentration of the suspension, demonstrating different emissions characteristic of monomer and excimer fluorescence, which are highly sensitive to the surrounding environment. This allows for the potential differentiation and sensing of different target analytes. PFC-1 showed discriminatory fluorescence sensing performance towards metal ions such as Al3+, Sc3+, Cr3+, and Cu2+, with changes in fluorescence intensity, emission peak shifts, and intensity ratio changes between monomer and excimer emissions. Furthermore, a smartphone-based detection strategy was proposed, leveraging color recognition capabilities of smartphones for onsite and real-time sensing. The work demonstrate that PFC-1 is a promising material for the development of portable, cost-effective fluorescent sensors for onsite and real-time detection of metal ions. The integration of PFC-1 with smartphone technology paves the way for practical applications in environmental monitoring, industrial processes, and healthcare diagnostics. Discriminatory fluorescence detection of different metal ions is realized by a luminescent HOF PFC-1 with different emissions characteristic of monomer and excimer fluorescence, which are highly sensitive to the metal ions Fe3+, Al3+, Sc3+, Cr3+, and Cu2+. [Display omitted] •A luminescent HOF material PFC-1 was constructed and showed monomer and excimer fluorescence behavior.•PFC-1 showed discriminatory fluorescence sensing performance towards different metal ions.•A smartphone-based detection strategy was realized for onsite and real-time sensing.
ArticleNumber 113348
Author Chen, Banglin
Shen, Penglei
Alshahrani, Thamraa
Xu, Shiqing
Zhang, Wei
Gao, Junkuo
Zhao, Tao
Xu, Hui
Bai, Gongxun
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Hydrogen-bonded organic frameworks (HOFs)
Excimer
Metal ions
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SSID ssj0017121
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Snippet Discriminatory fluorescence detection of various metal ions is of significant importance in environmental and health-related applications. A luminescent...
SourceID crossref
elsevier
SourceType Aggregation Database
Publisher
StartPage 113348
SubjectTerms Discriminative sensing
Excimer
Fluorescence sensor
Hydrogen-bonded organic frameworks (HOFs)
Metal ions
Title A pyrene-based hydrogen-bonded framework with excimer induced ratiometric emission for discriminative luminescence detection of metal ions
URI https://dx.doi.org/10.1016/j.micromeso.2024.113348
Volume 381
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