Orbital-selective time-domain signature of nematicity dynamics in the charge-density-wave phase of La$_{1.65}$Eu$_{0.2}$Sr$_{0.15}$CuO$_4
Understanding the interplay between charge, nematic, and structural ordering tendencies in cuprate superconductors is critical to unraveling their complex phase diagram. Using pump-probe time-resolved resonant x-ray scattering on the (0 0 1) Bragg peak at the Cu $L_3$ and O $K$ resonances, we invest...
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Format | Journal Article |
Language | English |
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23.09.2022
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Abstract | Understanding the interplay between charge, nematic, and structural ordering
tendencies in cuprate superconductors is critical to unraveling their complex
phase diagram. Using pump-probe time-resolved resonant x-ray scattering on the
(0 0 1) Bragg peak at the Cu $L_3$ and O $K$ resonances, we investigate
non-equilibrium dynamics of $Q_a = Q_b = 0$ nematic order and its association
with both charge density wave (CDW) order and lattice dynamics in
La$_{1.65}$Eu$_{0.2}$Sr$_{0.15}$CuO$_4$. The orbital selectivity of the
resonant x-ray scattering cross-section allows nematicity dynamics associated
with the planar O 2$p$ and Cu 3$d$ states to be distinguished from the response
of anisotropic lattice distortions. A direct time-domain comparison of CDW
translational-symmetry breaking and nematic rotational-symmetry breaking
reveals that these broken symmetries remain closely linked in the photoexcited
state, consistent with the stability of CDW topological defects in the
investigated pump fluence regime. |
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AbstractList | Understanding the interplay between charge, nematic, and structural ordering
tendencies in cuprate superconductors is critical to unraveling their complex
phase diagram. Using pump-probe time-resolved resonant x-ray scattering on the
(0 0 1) Bragg peak at the Cu $L_3$ and O $K$ resonances, we investigate
non-equilibrium dynamics of $Q_a = Q_b = 0$ nematic order and its association
with both charge density wave (CDW) order and lattice dynamics in
La$_{1.65}$Eu$_{0.2}$Sr$_{0.15}$CuO$_4$. The orbital selectivity of the
resonant x-ray scattering cross-section allows nematicity dynamics associated
with the planar O 2$p$ and Cu 3$d$ states to be distinguished from the response
of anisotropic lattice distortions. A direct time-domain comparison of CDW
translational-symmetry breaking and nematic rotational-symmetry breaking
reveals that these broken symmetries remain closely linked in the photoexcited
state, consistent with the stability of CDW topological defects in the
investigated pump fluence regime. |
Author | Geck, Jochen Reid, Alexander H Lee, Byungjune Sutarto, Ronny Turner, Joshua J Choi, Hyeongi Bluschke, Martin Moen, Peter Jang, Dogeun Dakovski, Georgi L Na, MengXing Revcolevschi, Alexandre Burdet, Nicolas G Smit, Steef Hawthorn, David G Park, Jae-Hoon Coslovich, Giacomo Remedios, Brandon Dos Lin, Ming-Fu Husain, Ali A Kim, Minseok Park, Sang-Youn Gupta, Naman K Damascelli, Andrea Jang, Hoyoung Nguyen, Quynh L |
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BackLink | https://doi.org/10.48550/arXiv.2209.11528$$DView paper in arXiv https://doi.org/10.1073/pnas.2400727121$$DView published paper (Access to full text may be restricted) |
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Title | Orbital-selective time-domain signature of nematicity dynamics in the charge-density-wave phase of La$_{1.65}$Eu$_{0.2}$Sr$_{0.15}$CuO$_4 |
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