Using PHREEQC to Simulate Solute Transport in Fractured Bedrock
The geochemical computer model PHREEQC can simulate solute transport in fractured bedrock aquifers that can be conceptualized as dual-porosity flow systems subject to one-dimensional advective-dispersive transport in the bedrock fractures and diffusive transport in the bedrock matrix. This article d...
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| Published in | Ground water Vol. 45; no. 4; pp. 468 - 472 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Malden, USA
Malden, USA : Blackwell Publishing Inc
01.07.2007
Blackwell Publishing Inc Ground Water Publishing Company |
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| Online Access | Get full text |
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| Abstract | The geochemical computer model PHREEQC can simulate solute transport in fractured bedrock aquifers that can be conceptualized as dual-porosity flow systems subject to one-dimensional advective-dispersive transport in the bedrock fractures and diffusive transport in the bedrock matrix. This article demonstrates how the physical characteristics of such flow systems can be parameterized for use in PHREEQC, it provides a method for minimizing numerical dispersion in PHREEQC simulations, and it compares PHREEQC simulations with results of an analytical solution. The simulations assumed a dual-porosity conceptual model involving advective-reactive-dispersive transport in the mobile zone (bedrock fracture) and diffusive-reactive transport in the immobile zone (bedrock matrix). The results from the PHREEQC dual-porosity transport model that uses a finite-difference approach showed excellent agreement compared with an analytical solution. |
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| AbstractList | The geochemical computer model PHREEQC can simulate solute transport in fractured bedrock aquifers that can be conceptualized as dual‐porosity flow systems subject to one‐dimensional advective‐dispersive transport in the bedrock fractures and diffusive transport in the bedrock matrix. This article demonstrates how the physical characteristics of such flow systems can be parameterized for use in PHREEQC, it provides a method for minimizing numerical dispersion in PHREEQC simulations, and it compares PHREEQC simulations with results of an analytical solution. The simulations assumed a dual‐porosity conceptual model involving advective‐reactive‐dispersive transport in the mobile zone (bedrock fracture) and diffusive‐reactive transport in the immobile zone (bedrock matrix). The results from the PHREEQC dual‐porosity transport model that uses a finite‐difference approach showed excellent agreement compared with an analytical solution. The geochemical computer model PHREEQC can simulate solute transport in fractured bedrock aquifers that can be conceptualized as dual-porosity flow systems subject to one-dimensional advective-dispersive transport in the bedrock fractures and diffusive transport in the bedrock matrix. This article demonstrates how the physical characteristics of such flow systems can be parameterized for use in PHREEQC, it provides a method for minimizing numerical dispersion in PHREEQC simulations, and it compares PHREEQC simulations with results of an analytical solution. The simulations assumed a dual-porosity conceptual model involving advective-reactive-dispersive transport in the mobile zone (bedrock fracture) and diffusive-reactive transport in the immobile zone (bedrock matrix). The results from the PHREEQC dual-porosity transport model that uses a finite-difference approach showed excellent agreement compared with an analytical solution. [PUBLICATION ABSTRACT] The geochemical computer model PHREEQC can simulate solute transport in fractured bedrock aquifers that can be conceptualized as dual-porosity flow systems subject to one-dimensional advective-dispersive transport in the bedrock fractures and diffusive transport in the bedrock matrix. This article demonstrates how the physical characteristics of such flow systems can be parameterized for use in PHREEQC, it provides a method for minimizing numerical dispersion in PHREEQC simulations, and it compares PHREEQC simulations with results of an analytical solution. The simulations assumed a dual-porosity conceptual model involving advective-reactive-dispersive transport in the mobile zone (bedrock fracture) and diffusive-reactive transport in the immobile zone (bedrock matrix). The results from the PHREEQC dual-porosity transport model that uses a finite-difference approach showed excellent agreement compared with an analytical solution.The geochemical computer model PHREEQC can simulate solute transport in fractured bedrock aquifers that can be conceptualized as dual-porosity flow systems subject to one-dimensional advective-dispersive transport in the bedrock fractures and diffusive transport in the bedrock matrix. This article demonstrates how the physical characteristics of such flow systems can be parameterized for use in PHREEQC, it provides a method for minimizing numerical dispersion in PHREEQC simulations, and it compares PHREEQC simulations with results of an analytical solution. The simulations assumed a dual-porosity conceptual model involving advective-reactive-dispersive transport in the mobile zone (bedrock fracture) and diffusive-reactive transport in the immobile zone (bedrock matrix). The results from the PHREEQC dual-porosity transport model that uses a finite-difference approach showed excellent agreement compared with an analytical solution. |
| Author | McCray, John E. Lipson, David S. Thyne, Geoffrey D. |
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| Cites_doi | 10.1016/0169-7722(95)00088-7 10.1144/1470-9236/2001-52 10.2475/ajs.301.1.16 10.1029/WR018i006p01634 10.1111/j.1745-6584.2005.tb02283.x 10.1016/B978-0-12-083980-3.50005-X |
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| References | Gaus, I., P. Shand, I.N. Gale, and A.T. Williams. 2002. Geochemical modeling of fluoride concentration changes during aquifer storage and recovery (ASR) in the chalk aquifer in Wessex, England. Quarterly Journal of Engineering Geology & Hydrogeology 35, no. 2: 203-208. Xu, T., and K. Pruess. 2001. Modeling multiphase non-isothermal fluid flow and reactive geochemical transport in variably saturated fractured rocks: 1. methodology. American Journal of Science 301, no. 1: 16-33. Bear, J., C.F. Tsang, and G. De Marsily, ed. 1993. Flow and Contaminant Transport in Fractured Rock. San Diego, California: Academic Press. Appelo, C.A.J., and D. Postma. 1993. Geochemistry, Groundwater, and Pollution. Rotterdam, Netherlands: A.A. Balekema. Sudicky, E.A., and E.O. Frind. 1982. Contaminant transport in fractured porous media: Analytical solutions for a system of parallel fractures. Water Resources Research 18, no. 6: 1634-1642. Lipson, D.S., B.H. Kueper, and M.J. Gefell. 2005. Matrix diffusion-derived plume attenuation in fractured bedrock. Ground Water 43, no. 1: 30-39. Therrien, R., and E.A. Sudicky. 1996. Three-dimensional analysis of variably-saturated flow and solute transport in discretely-fractured porous media. Journal of Contaminant Hydrology 23, no. 1-2: 1-44. 2005; 43 1993 1982; 18 2002; 35 2001; 301 1996; 23 1999 e_1_2_5_9_1 e_1_2_5_8_1 e_1_2_5_7_1 e_1_2_5_6_1 Appelo C.A.J. (e_1_2_5_2_1) 1993 e_1_2_5_5_1 e_1_2_5_4_1 e_1_2_5_3_1 |
| References_xml | – reference: Bear, J., C.F. Tsang, and G. De Marsily, ed. 1993. Flow and Contaminant Transport in Fractured Rock. San Diego, California: Academic Press. – reference: Therrien, R., and E.A. Sudicky. 1996. Three-dimensional analysis of variably-saturated flow and solute transport in discretely-fractured porous media. Journal of Contaminant Hydrology 23, no. 1-2: 1-44. – reference: Gaus, I., P. Shand, I.N. Gale, and A.T. Williams. 2002. Geochemical modeling of fluoride concentration changes during aquifer storage and recovery (ASR) in the chalk aquifer in Wessex, England. Quarterly Journal of Engineering Geology & Hydrogeology 35, no. 2: 203-208. – reference: Appelo, C.A.J., and D. Postma. 1993. Geochemistry, Groundwater, and Pollution. Rotterdam, Netherlands: A.A. Balekema. – reference: Xu, T., and K. Pruess. 2001. Modeling multiphase non-isothermal fluid flow and reactive geochemical transport in variably saturated fractured rocks: 1. methodology. American Journal of Science 301, no. 1: 16-33. – reference: Lipson, D.S., B.H. Kueper, and M.J. Gefell. 2005. Matrix diffusion-derived plume attenuation in fractured bedrock. Ground Water 43, no. 1: 30-39. – reference: Sudicky, E.A., and E.O. Frind. 1982. Contaminant transport in fractured porous media: Analytical solutions for a system of parallel fractures. Water Resources Research 18, no. 6: 1634-1642. – volume: 301 start-page: 16 issue: no. 1 year: 2001 end-page: 33 article-title: Modeling multiphase non‐isothermal fluid flow and reactive geochemical transport in variably saturated fractured rocks: 1. methodology publication-title: American Journal of Science – volume: 23 start-page: 1 issue: no. 1–2 year: 1996 end-page: 44 article-title: Three‐dimensional analysis of variably‐saturated flow and solute transport in discretely‐fractured porous media publication-title: Journal of Contaminant Hydrology – volume: 43 start-page: 30 issue: no. 1 year: 2005 end-page: 39 article-title: Matrix diffusion‐derived plume attenuation in fractured bedrock publication-title: Ground Water – year: 1993 – volume: 18 start-page: 1634 issue: no. 6 year: 1982 end-page: 1642 article-title: Contaminant transport in fractured porous media: Analytical solutions for a system of parallel fractures publication-title: Water Resources Research – volume: 35 start-page: 203 issue: no. 2 year: 2002 end-page: 208 article-title: Geochemical modeling of fluoride concentration changes during aquifer storage and recovery (ASR) in the chalk aquifer in Wessex, England publication-title: Quarterly Journal of Engineering Geology & Hydrogeology – year: 1999 – ident: e_1_2_5_6_1 – ident: e_1_2_5_8_1 doi: 10.1016/0169-7722(95)00088-7 – volume-title: Geochemistry, Groundwater, and Pollution year: 1993 ident: e_1_2_5_2_1 – ident: e_1_2_5_4_1 doi: 10.1144/1470-9236/2001-52 – ident: e_1_2_5_9_1 doi: 10.2475/ajs.301.1.16 – ident: e_1_2_5_7_1 doi: 10.1029/WR018i006p01634 – ident: e_1_2_5_5_1 doi: 10.1111/j.1745-6584.2005.tb02283.x – ident: e_1_2_5_3_1 doi: 10.1016/B978-0-12-083980-3.50005-X |
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| Snippet | The geochemical computer model PHREEQC can simulate solute transport in fractured bedrock aquifers that can be conceptualized as dual-porosity flow systems... The geochemical computer model PHREEQC can simulate solute transport in fractured bedrock aquifers that can be conceptualized as dual‐porosity flow systems... |
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| SubjectTerms | analysis Aquifers bedrock Computer based modeling computers Flow system Fresh Water Fresh Water - analysis Geochemistry Groundwater Models, Theoretical Porosity Solute movement Solute transport solutes Water Movements |
| Title | Using PHREEQC to Simulate Solute Transport in Fractured Bedrock |
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