Vegetation-Atmosphere Partitioning of Polycyclic Aromatic Hydrocarbons
A study examined the partitioning of polycyclic aromatic hydrocarbons between vegetation and the atmosphere throughout the growing season and under natural conditions. Evidence indicates that atmospheric semivolatile organic compounds undergo an annual partitioning cycle with the surface of the eart...
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| Published in | Environmental science & technology Vol. 28; no. 5; pp. 939 - 943 |
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| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
Washington, DC
American Chemical Society
01.05.1994
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| Subjects | |
| Online Access | Get full text |
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| Abstract | A study examined the partitioning of polycyclic aromatic hydrocarbons between vegetation and the atmosphere throughout the growing season and under natural conditions. Evidence indicates that atmospheric semivolatile organic compounds undergo an annual partitioning cycle with the surface of the earth. |
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| AbstractList | The partitioning of polycyclic aromatic hydrocarbons (PAH) between vegetation and the atmosphere was studied throughout the growing season and under natural conditions. A vegetation-atmosphere partition coefficient (K sub(v)) was derived by analogy to partition coefficients for gas-particle partitioning and fish-water partitioning. K sub(v) is temperature dependent, and from this functional relationship we calculated PAH-vegetation binding energies. These energies were highly correlated with heats of vaporization. The PAH-vegetation partitioning process is primarily dependent upon the atmospheric gas-phase PAH concentration and ambient temperature. At low ambient temperatures (spring and fall) gas-phase PAH partition into vegetation, and at high ambient temperatures (summer), some PAH volatilize and return to the atmosphere. This study provides further evidence that atmospheric semivolatile organic compounds undergo an annual partitioning cycle with the surface of the earth. A study examined the partitioning of polycyclic aromatic hydrocarbons between vegetation and the atmosphere throughout the growing season and under natural conditions. Evidence indicates that atmospheric semivolatile organic compounds undergo an annual partitioning cycle with the surface of the earth. The partitioning of polycyclic aromatic hydrocarbons (PAH) between vegetation and the atmosphere was studied throughout the growing season and under natural conditions. A vegetation-atmosphere partition coefficient (K[sub v]) was derived by analogy to partition coefficients for gas-particle partitioning and fish-water partitioning. K[sub v] is temperature dependent, and from this functional relationship we calculated PAH-vegetation binding energies. These energies were highly correlated with heats of vaporization. The PAH-vegetation partitioning process is primarily dependent upon the atmospheric gas-phase PAH concentration and ambient temperature. At low ambient temperatures (spring and fall) gas-phase PAH partition into vegetation, and at high ambient temperatures (summer), some PAH volatilize and return to the atmosphere. This study provides further evidence that atmospheric semivolatile organic compounds undergo an annual partitioning cycle with the surface of the earth. 39 refs., 3 figs., 1 tab. PAH partitioning between the atmosphere and vegetation was examined during the growing season by analysis of plant and air samples collected in Bloomington, IN. The derived vegetation-atmosphere partition coefficient, shown to be temperature dependent, was used to determine PAH-vegetation binding energies. The latter were strongly correlated with heats of vaporization, and the partitioning process was governed by the ambient temperature and the atmospheric gas-phase PAH concentration. Gas-phase PAH partition into vegetation at low ambient temperature and volatile and return to the atmosphere at higher temperatures. |
| Author | Hites, Ronald A Simonich, Staci L |
| Author_xml | – sequence: 1 givenname: Staci L surname: Simonich fullname: Simonich, Staci L – sequence: 2 givenname: Ronald A surname: Hites fullname: Hites, Ronald A |
| BackLink | http://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=4150966$$DView record in Pascal Francis https://www.ncbi.nlm.nih.gov/pubmed/22191838$$D View this record in MEDLINE/PubMed https://www.osti.gov/biblio/6977491$$D View this record in Osti.gov |
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| Snippet | A study examined the partitioning of polycyclic aromatic hydrocarbons between vegetation and the atmosphere throughout the growing season and under natural... PAH partitioning between the atmosphere and vegetation was examined during the growing season by analysis of plant and air samples collected in Bloomington,... The partitioning of polycyclic aromatic hydrocarbons (PAH) between vegetation and the atmosphere was studied throughout the growing season and under natural... |
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| SubjectTerms | 400201 - Chemical & Physicochemical Properties 540120 - Environment, Atmospheric- Chemicals Monitoring & Transport- (1990-) 540220 - Environment, Terrestrial- Chemicals Monitoring & Transport- (1990-) AIR POLLUTION MONITORING AROMATICS Atmosphere Convection, turbulence, diffusion. Boundary layer structure and dynamics Earth, ocean, space ENTHALPY Environmental monitoring ENVIRONMENTAL SCIENCES ENVIRONMENTAL TRANSPORT EVAPORATION Exact sciences and technology External geophysics HYDROCARBONS INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY LAND POLLUTION MASS TRANSFER MATHEMATICAL MODELS Meteorology MONITORING ORGANIC COMPOUNDS PARTITION PHASE TRANSFORMATIONS PHYSICAL PROPERTIES PLANTS POLLUTION POLYCYCLIC AROMATIC HYDROCARBONS SEASONAL VARIATIONS TEMPERATURE DEPENDENCE THERMODYNAMIC PROPERTIES TRANSITION HEAT VAPORIZATION HEAT VARIATIONS |
| Title | Vegetation-Atmosphere Partitioning of Polycyclic Aromatic Hydrocarbons |
| URI | http://dx.doi.org/10.1021/es00054a028 https://api.istex.fr/ark:/67375/TPS-PKHG40VF-R/fulltext.pdf https://www.ncbi.nlm.nih.gov/pubmed/22191838 https://www.proquest.com/docview/230129357 https://search.proquest.com/docview/14336063 https://search.proquest.com/docview/16880211 https://search.proquest.com/docview/912640525 https://www.osti.gov/biblio/6977491 |
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