Biogeochemistry and isotope geochemistry of a landfill leachate plume
The biogeochemical processes were identified which improved the leachate composition in the flow direction of a landfill leachate plume (Banisveld, The Netherlands). Groundwater observation wells were placed at specific locations after delineating the leachate plume using geophysical tests to map su...
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| Published in | Journal of contaminant hydrology Vol. 65; no. 3; pp. 245 - 268 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier B.V
01.09.2003
Elsevier Science |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The biogeochemical processes were identified which improved the leachate composition in the flow direction of a landfill leachate plume (Banisveld, The Netherlands). Groundwater observation wells were placed at specific locations after delineating the leachate plume using geophysical tests to map subsurface conductivity. Redox processes were determined using the distribution of solid and soluble redox species, hydrogen concentrations, concentration of dissolved gases (N
2, Ar, and CH
4), and stable isotopes (
δ
15N–NO
3,
δ
34S–SO
4,
δ
13C–CH
4,
δ
2H–CH
4, and
δ
13C of dissolved organic and inorganic carbon (DOC and DIC, respectively)). The combined application of these techniques improved the redox interpretation considerably. Dissolved organic carbon (DOC) decreased downstream in association with increasing
δ
13C-DOC values confirming the occurrence of degradation. Degradation of DOC was coupled to iron reduction inside the plume, while denitrification could be an important redox process at the top fringe of the plume. Stable carbon and hydrogen isotope signatures of methane indicated that methane was formed inside the landfill and not in the plume. Total gas pressure exceeded hydrostatic pressure in the plume, and methane seems subject to degassing. Quantitative proof for DOC degradation under iron-reducing conditions could only be obtained if the geochemical processes cation exchange and precipitation of carbonate minerals (siderite and calcite) were considered and incorporated in an inverse geochemical model of the plume. Simulation of
δ
13C-DIC confirmed that precipitation of carbonate minerals happened. |
|---|---|
| AbstractList | The biogeochemical processes were identified which improved the leachate composition in the flow direction of a landfill leachate plume (Banisveld, The Netherlands). Groundwater observation wells were placed at specific locations after delineating the leachate plume using geophysical tests to map subsurface conductivity. Redox processes were determined using the distribution of solid and soluble redox species, hydrogen concentrations, concentration of dissolved gases (N sub(2), Ar, and CH sub(4)), and stable isotopes ( delta super(15)N-NO sub(3), delta super(34)S-SO sub(4), delta super(13)C-CH sub(4), delta super(2)H-CH sub(4), and delta super(13)C of dissolved organic and inorganic carbon (DOC and DIC, respectively)). The combined application of these techniques improved the redox interpretation considerably. Dissolved organic carbon (DOC) decreased downstream in association with increasing delta super(13)C-DOC values confirming the occurrence of degradation. Degradation of DOC was coupled to iron reduction inside the plume, while denitrification could be an important redox process at the top fringe of the plume. Stable carbon and hydrogen isotope signatures of methane indicated that methane was formed inside the landfill and not in the plume. Total gas pressure exceeded hydrostatic pressure in the plume, and methane seems subject to degassing. Quantitative proof for DOC degradation under iron-reducing conditions could only be obtained if the geochemical processes cation exchange and precipitation of carbonate minerals (siderite and calcite) were considered and incorporated in an inverse geochemical model of the plume. Simulation of delta super(13)C-DIC confirmed that precipitation of carbonate minerals happened. The biogeochemical processes were identified which improved the leachate composition in the flow direction of a landfill leachate plume (Banisveld, The Netherlands). Groundwater observation wells were placed at specific locations after delineating the leachate plume using geophysical tests to map subsurface conductivity. Redox processes were determined using the distribution of solid and soluble redox species, hydrogen concentrations, concentration of dissolved gases (N 2, Ar, and CH 4), and stable isotopes ( δ 15N–NO 3, δ 34S–SO 4, δ 13C–CH 4, δ 2H–CH 4, and δ 13C of dissolved organic and inorganic carbon (DOC and DIC, respectively)). The combined application of these techniques improved the redox interpretation considerably. Dissolved organic carbon (DOC) decreased downstream in association with increasing δ 13C-DOC values confirming the occurrence of degradation. Degradation of DOC was coupled to iron reduction inside the plume, while denitrification could be an important redox process at the top fringe of the plume. Stable carbon and hydrogen isotope signatures of methane indicated that methane was formed inside the landfill and not in the plume. Total gas pressure exceeded hydrostatic pressure in the plume, and methane seems subject to degassing. Quantitative proof for DOC degradation under iron-reducing conditions could only be obtained if the geochemical processes cation exchange and precipitation of carbonate minerals (siderite and calcite) were considered and incorporated in an inverse geochemical model of the plume. Simulation of δ 13C-DIC confirmed that precipitation of carbonate minerals happened. At the Bansiveld landfill site near Boxtel, Netherlands, which is not sealed by an artificial or natural liner, the redox processes coupled to the oxidation of dissolved organic carbon in the leachate plume were determined. Stable isotopes were measured to quality the redox processes, and inverse geochemical modeling was performed to quantify the processes causing the observed improvement in leachate composition downstream of the landfill. Reductive dissolution of iron oxides was indicated as the main natural attenuation process, as suggested by the hydrogen concentrations, supersaturation for siderite, and inverse geochemical modeling. A lack of methane production and sulfate reduction inside the plume was found, as indicated by slightly decreasing CH sub(4) concentrations, nondecreasing SO sub(4) concentrations, and an absence of SO sub(4) minerals in the aquifer. The biogeochemical processes were identified which improved the leachate composition in the flow direction of a landfill leachate plume (Banisveld, The Netherlands). Groundwater observation wells were placed at specific locations after delineating the leachate plume using geophysical tests to map subsurface conductivity. Redox processes were determined using the distribution of solid and soluble redox species, hydrogen concentrations, concentration of dissolved gases (N(2), Ar, and CH(4)), and stable isotopes (delta15N-NO(3), delta34S-SO(4), delta13C-CH(4), delta2H-CH(4), and delta13C of dissolved organic and inorganic carbon (DOC and DIC, respectively)). The combined application of these techniques improved the redox interpretation considerably. Dissolved organic carbon (DOC) decreased downstream in association with increasing delta13C-DOC values confirming the occurrence of degradation. Degradation of DOC was coupled to iron reduction inside the plume, while denitrification could be an important redox process at the top fringe of the plume. Stable carbon and hydrogen isotope signatures of methane indicated that methane was formed inside the landfill and not in the plume. Total gas pressure exceeded hydrostatic pressure in the plume, and methane seems subject to degassing. Quantitative proof for DOC degradation under iron-reducing conditions could only be obtained if the geochemical processes cation exchange and precipitation of carbonate minerals (siderite and calcite) were considered and incorporated in an inverse geochemical model of the plume. Simulation of delta13C-DIC confirmed that precipitation of carbonate minerals happened. The biogeochemical processes were identified which improved the leachate composition in the flow direction of a landfill leachate plume (Banisveld, The Netherlands). Groundwater observation wells were placed at specific locations after delineating the leachate plume using geophysical tests to map subsurface conductivity. Redox processes were determined using the distribution of solid and soluble redox species, hydrogen concentrations, concentration of dissolved gases (N(2), Ar, and CH(4)), and stable isotopes (delta15N-NO(3), delta34S-SO(4), delta13C-CH(4), delta2H-CH(4), and delta13C of dissolved organic and inorganic carbon (DOC and DIC, respectively)). The combined application of these techniques improved the redox interpretation considerably. Dissolved organic carbon (DOC) decreased downstream in association with increasing delta13C-DOC values confirming the occurrence of degradation. Degradation of DOC was coupled to iron reduction inside the plume, while denitrification could be an important redox process at the top fringe of the plume. Stable carbon and hydrogen isotope signatures of methane indicated that methane was formed inside the landfill and not in the plume. Total gas pressure exceeded hydrostatic pressure in the plume, and methane seems subject to degassing. Quantitative proof for DOC degradation under iron-reducing conditions could only be obtained if the geochemical processes cation exchange and precipitation of carbonate minerals (siderite and calcite) were considered and incorporated in an inverse geochemical model of the plume. Simulation of delta13C-DIC confirmed that precipitation of carbonate minerals happened.The biogeochemical processes were identified which improved the leachate composition in the flow direction of a landfill leachate plume (Banisveld, The Netherlands). Groundwater observation wells were placed at specific locations after delineating the leachate plume using geophysical tests to map subsurface conductivity. Redox processes were determined using the distribution of solid and soluble redox species, hydrogen concentrations, concentration of dissolved gases (N(2), Ar, and CH(4)), and stable isotopes (delta15N-NO(3), delta34S-SO(4), delta13C-CH(4), delta2H-CH(4), and delta13C of dissolved organic and inorganic carbon (DOC and DIC, respectively)). The combined application of these techniques improved the redox interpretation considerably. Dissolved organic carbon (DOC) decreased downstream in association with increasing delta13C-DOC values confirming the occurrence of degradation. Degradation of DOC was coupled to iron reduction inside the plume, while denitrification could be an important redox process at the top fringe of the plume. Stable carbon and hydrogen isotope signatures of methane indicated that methane was formed inside the landfill and not in the plume. Total gas pressure exceeded hydrostatic pressure in the plume, and methane seems subject to degassing. Quantitative proof for DOC degradation under iron-reducing conditions could only be obtained if the geochemical processes cation exchange and precipitation of carbonate minerals (siderite and calcite) were considered and incorporated in an inverse geochemical model of the plume. Simulation of delta13C-DIC confirmed that precipitation of carbonate minerals happened. |
| Author | Groen, Jacobus Griffioen, Jasper van Breukelen, Boris M. Röling, Wilfred F.M. van Verseveld, Henk W. |
| Author_xml | – sequence: 1 givenname: Boris M. surname: van Breukelen fullname: van Breukelen, Boris M. email: boris.van.breukelen@falw.vu.nl organization: Department of Hydrogeology, Faculty of Earth and Life Sciences, Research School NSG, Vrije Universiteit, De Boelelaan 1085, NL-1081 HV Amsterdam, The Netherlands – sequence: 2 givenname: Wilfred F.M. surname: Röling fullname: Röling, Wilfred F.M. organization: Section Molecular Microbial Ecology, Department of Molecular Cell Physiology, Faculty of Earth and Life Sciences, Research School SENSE, Vrije Universiteit, De Boelelaan 1085, NL-1081 HV Amsterdam, The Netherlands – sequence: 3 givenname: Jacobus surname: Groen fullname: Groen, Jacobus organization: Department of Hydrogeology, Faculty of Earth and Life Sciences, Research School NSG, Vrije Universiteit, De Boelelaan 1085, NL-1081 HV Amsterdam, The Netherlands – sequence: 4 givenname: Jasper surname: Griffioen fullname: Griffioen, Jasper organization: Netherlands Institute of Applied Geosciences TNO, Princetonlaan 6, NL-3508 TA Utrecht, The Netherlands – sequence: 5 givenname: Henk W. surname: van Verseveld fullname: van Verseveld, Henk W. organization: Section Molecular Microbial Ecology, Department of Molecular Cell Physiology, Faculty of Earth and Life Sciences, Research School SENSE, Vrije Universiteit, De Boelelaan 1085, NL-1081 HV Amsterdam, The Netherlands |
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| Keywords | Redox Modelling Natural attenuation Hydrogen Landfills Stable isotopes electromagnetic surveys attenuation degassing plumes ground water degradation hydrostatic pressure sulfates nitrates pollution denitrification landfills S-34/S-32 organic carbon gases stable isotopes C-13/C-12 N-15/N-14 Europe nitrogen concentration interpretation methane argon leachate electrical conductivity |
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| Snippet | The biogeochemical processes were identified which improved the leachate composition in the flow direction of a landfill leachate plume (Banisveld, The... At the Bansiveld landfill site near Boxtel, Netherlands, which is not sealed by an artificial or natural liner, the redox processes coupled to the oxidation of... |
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| SubjectTerms | Calcite Carbonates Cation exchanging Concentration (composition) Degassing Degradation Earth sciences Earth, ocean, space Engineering and environment geology. Geothermics Environmental Monitoring - methods Exact sciences and technology Geochemistry Geological Phenomena Geology Geophysics Groundwater Hydrogen Hydrogeology Hydrology Hydrology. Hydrogeology Isotope geochemistry Isotope geochemistry. Geochronology Isotopes Isotopes - analysis Landfills Modelling Natural attenuation Oxidation-Reduction Pollution, environment geology Precipitation Redox Refuse Disposal Siderite Soil Pollutants - analysis Stable isotopes Water Pollutants - analysis |
| Title | Biogeochemistry and isotope geochemistry of a landfill leachate plume |
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