Sunlight-Induced Formation of Dissolved Gaseous Mercury in Lake Waters
A study shows that sunlight induces the formation of mercury from Hg2positive in natural water samples incubated in situ and may alter the evasion of gaseous mercury in lakes.
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| Published in | Environmental science & technology Vol. 28; no. 13; pp. 2366 - 2371 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Washington, DC
American Chemical Society
01.12.1994
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| Subjects | |
| Online Access | Get full text |
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| Abstract | A study shows that sunlight induces the formation of mercury from Hg2positive in natural water samples incubated in situ and may alter the evasion of gaseous mercury in lakes. |
|---|---|
| AbstractList | Formation of dissolved gaseous mercury (DGM) was measured in lake water incubated at midday in Teflon bottles. DGM production was photoinduced as transparent bottles yield DGM concentrations that were 2.4-9 times higher than dark controls. These results provide the first experimental evidence obtained in the field of a direct link between solar radiation and DGM production. A positive relationship was found between photoinduced DGM production at different times of the year and incident radiation. Removal of UV sub(B) light or addition of hydrogen peroxide during incubation did not result in significant changes in DGM levels. A diel pattern in DGM production was observed, and a depth profile of DGM revealed that most of the production was occurring in the epilimnion. It is concluded that sunlight plays a key role in DGM production in the epilimnion and may alter the fluxes of Hg in aquatic ecosystems. A study shows that sunlight induces the formation of mercury from Hg2positive in natural water samples incubated in situ and may alter the evasion of gaseous mercury in lakes. Dissolved gaseous mercury (DGM) formation was quantified in lake water incubated at midday in Teflon containers. DGM concentrations in transparent bottles were 2.4-9 times higher than in dark controls, demonstrating a photoinduction mechanism. A positive link was confirmed between photoinduced DGM formation at different times of the year and incident solar radiation. A diel pattern in DGM evolution was documented, and depth profiles showed that most of the production occurred in the epilimnion. The effects of sunlight and hydrogen peroxide on dissolved gaseous mercury (DGM) production in lake water were studied. The effect of UV-B light (280-320 nm) was assessed. Samples incubated in transparent bottles yielded DGM levels that were 2.4-8.9 times higher than those kept in black bottles. DGM production rates varied seasonally, ranging from 182 fM per h in August to 17 fM per h in November. UV-B light was responsible for less than 25 per cent of the DGM production. Hydrogen peroxide did not have a significant role. The presence of a diel pattern of DGM production in surface water was investigated. The highest DGM levels were observed at noon and the lowest ones at 6.00 AM, just before sunrise. Depth profiles of DGM concentrations were obtained to identify the site of maximal DGM production in the water column. DGM levels of up to 256 fM were found in the epilimnion, decreasing to 59 fM at 6 m and increasing in the hypolimnion to 100 fM. It is hypothesized that the primary process for DGM production in lakes was the biological or photochemical reduction of mercury in the epilimnion by visible light or UV-A light. |
| Author | Amyot, Marc McQueen, Donald J Mierle, Greg Lean, David R. S |
| Author_xml | – sequence: 1 givenname: Marc surname: Amyot fullname: Amyot, Marc – sequence: 2 givenname: Donald J surname: McQueen fullname: McQueen, Donald J – sequence: 3 givenname: Greg surname: Mierle fullname: Mierle, Greg – sequence: 4 givenname: David R. S surname: Lean fullname: Lean, David R. S |
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| Snippet | A study shows that sunlight induces the formation of mercury from Hg2positive in natural water samples incubated in situ and may alter the evasion of gaseous... The effects of sunlight and hydrogen peroxide on dissolved gaseous mercury (DGM) production in lake water were studied. The effect of UV-B light (280-320 nm)... Dissolved gaseous mercury (DGM) formation was quantified in lake water incubated at midday in Teflon containers. DGM concentrations in transparent bottles were... Formation of dissolved gaseous mercury (DGM) was measured in lake water incubated at midday in Teflon bottles. DGM production was photoinduced as transparent... |
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| Title | Sunlight-Induced Formation of Dissolved Gaseous Mercury in Lake Waters |
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