Behavior of dissolved silica in parent solution at the formation of calcium carbonate

The authors have studied experimentally on the coprecipitation of dissolved silica with calcium carbonate (calcite or aragonite) and on the influence of silica dissolved in a parent calcium bicarbonate solution on the crystal form of calcium carbonate precipitated from the parent solution. The copre...

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Published inGEOCHEMICAL JOURNAL Vol. 13; no. 6; pp. 253 - 260
Main Authors Kitano, Yasushi, Okumura, Minoru, Idogaki, Masatoshi
Format Journal Article
LanguageEnglish
Published GEOCHEMICAL SOCIETY OF JAPAN 01.01.1979
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Abstract The authors have studied experimentally on the coprecipitation of dissolved silica with calcium carbonate (calcite or aragonite) and on the influence of silica dissolved in a parent calcium bicarbonate solution on the crystal form of calcium carbonate precipitated from the parent solution. The coprecipitation of dissolved silica with calcium carbonate is affected significantly by the crystal form of precipitated calcium carbonate and by the presence of sodium chloride in a parent solution. That is, dissolved silica is more easily coprecipitated with aragonite than with calcite. The presence of dissolved silica in a parent solution favors the formation of calcite and inhibits that of aragonite. The amounts of silica coprecipitated with calcite and also with aragonite increase with increasing concentration of sodium chloride, that is, with increasing value of ionic strength in the parent solution. This trend is observed at the coprecipitation of undissociated chemical species with calcium carbonate.
AbstractList The authors have studied experimentally on the coprecipitation of dissolved silica with calcium carbonate (calcite or aragonite) and on the influence of silica dissolved in a parent calcium bicarbonate solution on the crystal form of calcium carbonate precipitated from the parent solution. The coprecipitation of dissolved silica with calcium carbonate is affected significantly by the crystal form of precipitated calcium carbonate and by the presence of sodium chloride in a parent solution. That is, dissolved silica is more easily coprecipitated with aragonite than with calcite. The presence of dissolved silica in a parent solution favors the formation of calcite and inhibits that of aragonite. The amounts of silica coprecipitated with calcite and also with aragonite increase with increasing concentration of sodium chloride, that is, with increasing value of ionic strength in the parent solution. This trend is observed at the coprecipitation of undissociated chemical species with calcium carbonate.
Author Idogaki, Masatoshi
Okumura, Minoru
Kitano, Yasushi
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  fullname: Okumura, Minoru
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  fullname: Idogaki, Masatoshi
  organization: Faculty of Science, Shimane Univ
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References KITANO, Y., OKUMURA, M. and IDOGAKI, M. (1978d) Coprecipitation of borate-boron with calcium carbonate. Geochem. J. 12, 183-189.
HARNED, H. S. and OWEN, B. B. (1958) The physical chemistry of electrolytic solutions, 3rd ed. Reinhold, New York.
MIYAKE, Y. and KITANO, Y. (1976) Chemical analysis of water quality. Chizinshoin, Tokyo, 265 (in Japanese).
KITANO, Y., TOKUYAMA, A. and KANAMORI, N. (1968) Measurement of the distribution coefficient of zinc and copper between carbonate precipitate and solution. J. Earth Sci. Nagoya Univ. 16, 1-102.
KITANO, Y., YOSHIOKA, S. and KANAMORI, N. (1972) The mineral composition of calcium carbonate formed in the processes of separation from bicarbonate solution. Kaseki 23/24, 3-14 (in Japanese).
KITANO, Y., KANAMORI, N. and TOKUYAMA, A. (1969) Effect of organic matter on solubilities and crystal form of carbonates. Am. Zoologist 9, 681-688.
KITANO, Y. (1962) The behavior of various inorganic ions in the separation of calcium carbonate from a bicarbonate solution. Bull. Chem. Soc. Japan 35, 1973-1980.
LIVINGSTONE, H. D. and THOMPSON, G. (1971) Trace element concentrations in some modern corals. Limnol. Oceanogr. 16, 786-796.
KITANO, Y., OKUMURA, M. and IDOGAKI, M. (1978c) Uptake of phosphate ions by calcium carbonate. Geochem. J. 12, 29-37.
KITANO, Y. and TERAO, H. (1972) Measurement of the distribution coefficient of minor elements between carbonate precipitate and solution - Strontium-barium coexisting system. Kaseki 23/24, 26-32 (in Japanese).
KITANO, Y. and OKUMURA, M. (1973) Coprecipitation of fluoride with calcium carbonate. Geochem. J. 7, 37-49.
GARRELS, R. M. and CHRIST, C. L. (1965) Solutions, minerals, and equilibria. Harper and Row, New York.
KITANO, Y., KANAMORI, N. and FUJIYOSHI, R. (1978a) Distribution of cadmium between calcium carbonate and solution (part 1) “Ca(HCO3)2 + Cd2+ + bipyridine → carbonate” system. Geochem. J. 12, 137-145.
MILLIMAN, J. D. (1974) Marine carbonates. Springer-Verlag.
KATO, K. and KITANO, Y. (1966) Salt error in colorimetric determination of the molybdate-reactive silica in sea water. J. Earth Sci. Nagoya Univ. 14, 151-158.
KITANO, Y., OKUMURA, M. and IDOGAKI, M. (1975) Incorporation of sodium, chloride and sulfate with calcium carbonate. Geochem. J. 9, 75-84.
KITANO, Y. and OOMORI, T. (1971) The coprecipitation of uranium with calcium carbonate. J. Oceanogr. Soc. Japan 27, 34-42.
KITANO, Y., PARK, K. and HOOD, D. W. (1962) Pure aragonite synthesis. J. Geophys. Res. 67, 4873-4874.
KITANO, Y. and HOOD, D. W. (1962) Calcium carbonate crystal formed from sea water by inorganic processes. J. Oceanogr. Soc. Japan 18, 208-219.
KITANO, Y., KANAMORI, N. and OOMORI, T. (1971) Measurements of distribution coefficients of strontium and barium between carbonate and solution - Abnormally high values of distribution coefficients measured at early stages of carbonate formation. Geochem. J. 4, 183-206.
KITANO, Y., KANAMORI, N. and FUJIYOSHI, R. (1978b) Distribution of cadmium between calcium carbonate and solution (part 2) “Ca(HCO3)2 + Cd2+ + NaCl → carbonate” system. Geochem. J. 12, 147-151.
KITANO, Y., OKUMURA, M. and IDOGAKI, M. (1979) Influence of borate-boron on crystal form of calcium carbonate. Geochem. J. 13, 223-224.
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