Measurement of uranium isotope ratios in Fukushima-accident contaminated soil samples using multi collector inductively coupled plasma mass spectrometry
In the present study, 137Cs and 238U activity concentrations, 234U/238U activity ratio, and 235U/238U isotope ratio were measured in fifteen soil samples collected from the exclusion zone around the Fukushima Daiichi Nuclear Power Station (FDNPS). The 137Cs activity concentrations of Fukushima-accid...
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| Published in | Journal of environmental radioactivity Vol. 232; p. 106568 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Elsevier Ltd
01.06.2021
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0265-931X 1879-1700 1879-1700 |
| DOI | 10.1016/j.jenvrad.2021.106568 |
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| Abstract | In the present study, 137Cs and 238U activity concentrations, 234U/238U activity ratio, and 235U/238U isotope ratio were measured in fifteen soil samples collected from the exclusion zone around the Fukushima Daiichi Nuclear Power Station (FDNPS). The 137Cs activity concentrations of Fukushima-accident contaminated soil samples ranged from 29.9 to 4780 kBq kg−1 with a mean of 2007 kBq kg−1. On the other hand, the 238U activity concentrations of these soil samples ranged from 5.2 to 22.4 Bq kg−1 with a mean of 13.2 Bq kg−1. The activity ratios of 234U/238U ranged from 0.973 to 1.023. The 235U/238U isotope ratios of these exclusion zone soil samples varied from 0.007246 to 0.007260, and they were similar to the natural terrestrial ratio confirming the natural origin. Using isotope dilution technique, the 235U/137Cs activity ratio was theoretically estimated for highly 137Cs contaminated soil samples from Fukushima exclusion zone ranged from 5.01 × 10−8 - 6.16 × 10−7 with a mean value of 2.51 × 10−7.
•137Cs activity concentration ranged from 29.9 to 4780 kBq kg−1.•The activity ratio of 234U/238U were in the range of 0.973–1.023.•The 235U/238U isotope ratios indicate natural in origin for Fukushima soil samples.•The 235U/137Cs activity ratio ranged from 5.01 × 10−8 - 6.16 × 10−7 for Fukushima exclusion zone soil samples. |
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| AbstractList | In the present study, 137Cs and 238U activity concentrations, 234U/238U activity ratio, and 235U/238U isotope ratio were measured in fifteen soil samples collected from the exclusion zone around the Fukushima Daiichi Nuclear Power Station (FDNPS). The 137Cs activity concentrations of Fukushima-accident contaminated soil samples ranged from 29.9 to 4780 kBq kg-1 with a mean of 2007 kBq kg-1. On the other hand, the 238U activity concentrations of these soil samples ranged from 5.2 to 22.4 Bq kg-1 with a mean of 13.2 Bq kg-1. The activity ratios of 234U/238U ranged from 0.973 to 1.023. The 235U/238U isotope ratios of these exclusion zone soil samples varied from 0.007246 to 0.007260, and they were similar to the natural terrestrial ratio confirming the natural origin. Using isotope dilution technique, the 235U/137Cs activity ratio was theoretically estimated for highly 137Cs contaminated soil samples from Fukushima exclusion zone ranged from 5.01 × 10-8 - 6.16 × 10-7 with a mean value of 2.51 × 10-7.In the present study, 137Cs and 238U activity concentrations, 234U/238U activity ratio, and 235U/238U isotope ratio were measured in fifteen soil samples collected from the exclusion zone around the Fukushima Daiichi Nuclear Power Station (FDNPS). The 137Cs activity concentrations of Fukushima-accident contaminated soil samples ranged from 29.9 to 4780 kBq kg-1 with a mean of 2007 kBq kg-1. On the other hand, the 238U activity concentrations of these soil samples ranged from 5.2 to 22.4 Bq kg-1 with a mean of 13.2 Bq kg-1. The activity ratios of 234U/238U ranged from 0.973 to 1.023. The 235U/238U isotope ratios of these exclusion zone soil samples varied from 0.007246 to 0.007260, and they were similar to the natural terrestrial ratio confirming the natural origin. Using isotope dilution technique, the 235U/137Cs activity ratio was theoretically estimated for highly 137Cs contaminated soil samples from Fukushima exclusion zone ranged from 5.01 × 10-8 - 6.16 × 10-7 with a mean value of 2.51 × 10-7. In the present study, Cs and U activity concentrations, U/ U activity ratio, and U/ U isotope ratio were measured in fifteen soil samples collected from the exclusion zone around the Fukushima Daiichi Nuclear Power Station (FDNPS). The Cs activity concentrations of Fukushima-accident contaminated soil samples ranged from 29.9 to 4780 kBq kg with a mean of 2007 kBq kg . On the other hand, the U activity concentrations of these soil samples ranged from 5.2 to 22.4 Bq kg with a mean of 13.2 Bq kg . The activity ratios of U/ U ranged from 0.973 to 1.023. The U/ U isotope ratios of these exclusion zone soil samples varied from 0.007246 to 0.007260, and they were similar to the natural terrestrial ratio confirming the natural origin. Using isotope dilution technique, the U/ Cs activity ratio was theoretically estimated for highly Cs contaminated soil samples from Fukushima exclusion zone ranged from 5.01 × 10 - 6.16 × 10 with a mean value of 2.51 × 10 . In the present study, 137Cs and 238U activity concentrations, 234U/238U activity ratio, and 235U/238U isotope ratio were measured in fifteen soil samples collected from the exclusion zone around the Fukushima Daiichi Nuclear Power Station (FDNPS). The 137Cs activity concentrations of Fukushima-accident contaminated soil samples ranged from 29.9 to 4780 kBq kg−1 with a mean of 2007 kBq kg−1. On the other hand, the 238U activity concentrations of these soil samples ranged from 5.2 to 22.4 Bq kg−1 with a mean of 13.2 Bq kg−1. The activity ratios of 234U/238U ranged from 0.973 to 1.023. The 235U/238U isotope ratios of these exclusion zone soil samples varied from 0.007246 to 0.007260, and they were similar to the natural terrestrial ratio confirming the natural origin. Using isotope dilution technique, the 235U/137Cs activity ratio was theoretically estimated for highly 137Cs contaminated soil samples from Fukushima exclusion zone ranged from 5.01 × 10−8 - 6.16 × 10−7 with a mean value of 2.51 × 10−7. •137Cs activity concentration ranged from 29.9 to 4780 kBq kg−1.•The activity ratio of 234U/238U were in the range of 0.973–1.023.•The 235U/238U isotope ratios indicate natural in origin for Fukushima soil samples.•The 235U/137Cs activity ratio ranged from 5.01 × 10−8 - 6.16 × 10−7 for Fukushima exclusion zone soil samples. In the present study, ¹³⁷Cs and ²³⁸U activity concentrations, ²³⁴U/²³⁸U activity ratio, and ²³⁵U/²³⁸U isotope ratio were measured in fifteen soil samples collected from the exclusion zone around the Fukushima Daiichi Nuclear Power Station (FDNPS). The ¹³⁷Cs activity concentrations of Fukushima-accident contaminated soil samples ranged from 29.9 to 4780 kBq kg⁻¹ with a mean of 2007 kBq kg⁻¹. On the other hand, the ²³⁸U activity concentrations of these soil samples ranged from 5.2 to 22.4 Bq kg⁻¹ with a mean of 13.2 Bq kg⁻¹. The activity ratios of ²³⁴U/²³⁸U ranged from 0.973 to 1.023. The ²³⁵U/²³⁸U isotope ratios of these exclusion zone soil samples varied from 0.007246 to 0.007260, and they were similar to the natural terrestrial ratio confirming the natural origin. Using isotope dilution technique, the ²³⁵U/¹³⁷Cs activity ratio was theoretically estimated for highly ¹³⁷Cs contaminated soil samples from Fukushima exclusion zone ranged from 5.01 × 10⁻⁸ - 6.16 × 10⁻⁷ with a mean value of 2.51 × 10⁻⁷. |
| ArticleNumber | 106568 |
| Author | Sorimachi, A. Sahoo, S.K. Omori, Y. Aono, T. Kavasi, N. Takahashi, H. Murugan, R. |
| Author_xml | – sequence: 1 givenname: R. surname: Murugan fullname: Murugan, R. organization: National Institutes for Quantum and Radiological Sciences and Technology (QST), 4-9-1 Anagawa, Inage-ku, Chiba, 263-8555, Japan – sequence: 2 givenname: N. surname: Kavasi fullname: Kavasi, N. organization: National Institutes for Quantum and Radiological Sciences and Technology (QST), 4-9-1 Anagawa, Inage-ku, Chiba, 263-8555, Japan – sequence: 3 givenname: S.K. surname: Sahoo fullname: Sahoo, S.K. email: sahoo.sarata@qst.go.jp organization: National Institutes for Quantum and Radiological Sciences and Technology (QST), 4-9-1 Anagawa, Inage-ku, Chiba, 263-8555, Japan – sequence: 4 givenname: Y. surname: Omori fullname: Omori, Y. organization: Fukushima Medical University, Hikarigaoka, Fukushima, 960-1295, Japan – sequence: 5 givenname: A. surname: Sorimachi fullname: Sorimachi, A. organization: Fukushima Medical University, Hikarigaoka, Fukushima, 960-1295, Japan – sequence: 6 givenname: H. surname: Takahashi fullname: Takahashi, H. organization: National Institutes for Quantum and Radiological Sciences and Technology (QST), 4-9-1 Anagawa, Inage-ku, Chiba, 263-8555, Japan – sequence: 7 givenname: T. surname: Aono fullname: Aono, T. organization: National Institutes for Quantum and Radiological Sciences and Technology (QST), 4-9-1 Anagawa, Inage-ku, Chiba, 263-8555, Japan |
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| Keywords | 235U/238U FDNPS 234U/238U activity ratio Fukushima soils MC-ICP-MS 137Cs Cs U/U U/U activity ratio |
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| Snippet | In the present study, 137Cs and 238U activity concentrations, 234U/238U activity ratio, and 235U/238U isotope ratio were measured in fifteen soil samples... In the present study, Cs and U activity concentrations, U/ U activity ratio, and U/ U isotope ratio were measured in fifteen soil samples collected from the... In the present study, ¹³⁷Cs and ²³⁸U activity concentrations, ²³⁴U/²³⁸U activity ratio, and ²³⁵U/²³⁸U isotope ratio were measured in fifteen soil samples... |
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| SubjectTerms | 137Cs 234U/238U activity ratio 235U/238U atomic absorption spectrometry cesium radioisotopes Cesium Radioisotopes - analysis FDNPS Fukushima Nuclear Accident Fukushima soils isotope dilution technique isotopes Japan Mass Spectrometry MC-ICP-MS nuclear power Plasma - chemistry polluted soils power plants Radiation Monitoring radioactivity Soil Soil Pollutants, Radioactive - analysis uranium Uranium - analysis |
| Title | Measurement of uranium isotope ratios in Fukushima-accident contaminated soil samples using multi collector inductively coupled plasma mass spectrometry |
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