Polycyclic aromatic hydrocarbons (PAH) and polychlorinated biphenyls (PCB) in urban soils of Greater London, UK

•London soil PAH concentrations are comparable with other cities.•London soil PCB concentrations are higher than other cities.•London soils contain multiple pryrogenic PAH sources.•Normal background PAH concentrations exceed land management assessment criteria. Surface soils from a 19km2 area in eas...

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Published inApplied geochemistry Vol. 51; pp. 303 - 314
Main Authors Vane, Christopher H., Kim, Alexander W., Beriro, Darren J., Cave, Mark R., Knights, Katherine, Moss-Hayes, Vicky, Nathanail, Paul C.
Format Journal Article
LanguageEnglish
Published Kidlington Elsevier Ltd 01.12.2014
Elsevier
Subjects
benzo(a)pyrene
cities
Earth sciences
Earth, ocean, space
Engineering and environment geology. Geothermics
Exact sciences and technology
Geochemistry
human health
Pollution, environment geology
polychlorinated biphenyls
polycyclic aromatic hydrocarbons
United Kingdom
urban soils
United Kingdom
Europe
Western Europe
PCBs
concentration
polycyclic aromatic hydrocarbons
soils
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Abstract •London soil PAH concentrations are comparable with other cities.•London soil PCB concentrations are higher than other cities.•London soils contain multiple pryrogenic PAH sources.•Normal background PAH concentrations exceed land management assessment criteria. Surface soils from a 19km2 area in east London, UK were analysed for polycyclic aromatic hydrocarbons (PAH) and polychlorinated biphenyls (PCB) (n=76). ∑16 PAH ranged from 4 to 67mg/kg (mean, 18mg/kg) and ∑50 PAH ranged from 6 to 88mg/kg (mean, 25mg/kg). ∑7 PCB ranged from 1 to 750μg/kg (mean, 22μg/kg) and ∑tri-hepta PCB ranged 9 to 2600μg/kg (mean, 120μg/kg). Compared to other international cities concentrations were similar for PAH but higher for PCB. Normal background concentrations (NBC) were calculated and compared to risk-based human health generic assessment criteria (GAC). Benzo[a]pyrene NBC for urban (6.9mg/kg), semi-urban (4.4mg/kg) and urban+semi urban (6mg/kg) domains exceed residential (1mg/kg) and allotment (2.2mg/kg) LQM/CIEH GAC (at 6% SOM) and the Indeno[1,2,3-cd]pyrene NBC for urban (6.8mg/kg) and urban+semi-urban (5.2mg/kg) domains exceed the residential (4.2mg/kg) LQM/CIEH GAC (at 6% SOM). Capsule Abstract: Normal background concentrations of polycyclic aromatic hydrocarbons and polychlorinated biphenyls are elevated in east London soils and in some cases exceed regulatory assessment criteria.
AbstractList Surface soils from a 19km2 area in east London, UK were analysed for polycyclic aromatic hydrocarbons (PAH) and polychlorinated biphenyls (PCB) (n=76). ∑16 PAH ranged from 4 to 67mg/kg (mean, 18mg/kg) and ∑50 PAH ranged from 6 to 88mg/kg (mean, 25mg/kg). ∑7 PCB ranged from 1 to 750μg/kg (mean, 22μg/kg) and ∑tri-hepta PCB ranged 9 to 2600μg/kg (mean, 120μg/kg). Compared to other international cities concentrations were similar for PAH but higher for PCB. Normal background concentrations (NBC) were calculated and compared to risk-based human health generic assessment criteria (GAC). Benzo[a]pyrene NBC for urban (6.9mg/kg), semi-urban (4.4mg/kg) and urban+semi urban (6mg/kg) domains exceed residential (1mg/kg) and allotment (2.2mg/kg) LQM/CIEH GAC (at 6% SOM) and the Indeno[1,2,3-cd]pyrene NBC for urban (6.8mg/kg) and urban+semi-urban (5.2mg/kg) domains exceed the residential (4.2mg/kg) LQM/CIEH GAC (at 6% SOM).Capsule Abstract: Normal background concentrations of polycyclic aromatic hydrocarbons and polychlorinated biphenyls are elevated in east London soils and in some cases exceed regulatory assessment criteria.
•London soil PAH concentrations are comparable with other cities.•London soil PCB concentrations are higher than other cities.•London soils contain multiple pryrogenic PAH sources.•Normal background PAH concentrations exceed land management assessment criteria. Surface soils from a 19km2 area in east London, UK were analysed for polycyclic aromatic hydrocarbons (PAH) and polychlorinated biphenyls (PCB) (n=76). ∑16 PAH ranged from 4 to 67mg/kg (mean, 18mg/kg) and ∑50 PAH ranged from 6 to 88mg/kg (mean, 25mg/kg). ∑7 PCB ranged from 1 to 750μg/kg (mean, 22μg/kg) and ∑tri-hepta PCB ranged 9 to 2600μg/kg (mean, 120μg/kg). Compared to other international cities concentrations were similar for PAH but higher for PCB. Normal background concentrations (NBC) were calculated and compared to risk-based human health generic assessment criteria (GAC). Benzo[a]pyrene NBC for urban (6.9mg/kg), semi-urban (4.4mg/kg) and urban+semi urban (6mg/kg) domains exceed residential (1mg/kg) and allotment (2.2mg/kg) LQM/CIEH GAC (at 6% SOM) and the Indeno[1,2,3-cd]pyrene NBC for urban (6.8mg/kg) and urban+semi-urban (5.2mg/kg) domains exceed the residential (4.2mg/kg) LQM/CIEH GAC (at 6% SOM). Capsule Abstract: Normal background concentrations of polycyclic aromatic hydrocarbons and polychlorinated biphenyls are elevated in east London soils and in some cases exceed regulatory assessment criteria.
Author Moss-Hayes, Vicky
Nathanail, Paul C.
Vane, Christopher H.
Beriro, Darren J.
Knights, Katherine
Cave, Mark R.
Kim, Alexander W.
Author_xml – sequence: 1
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– sequence: 2
  givenname: Alexander W.
  surname: Kim
  fullname: Kim, Alexander W.
  organization: British Geological Survey, Centre for Environmental Geochemistry, Keyworth, Nottingham NG12 5GG, UK
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  givenname: Darren J.
  surname: Beriro
  fullname: Beriro, Darren J.
  organization: British Geological Survey, Centre for Environmental Geochemistry, Keyworth, Nottingham NG12 5GG, UK
– sequence: 4
  givenname: Mark R.
  surname: Cave
  fullname: Cave, Mark R.
  organization: British Geological Survey, Centre for Environmental Geochemistry, Keyworth, Nottingham NG12 5GG, UK
– sequence: 5
  givenname: Katherine
  surname: Knights
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  organization: British Geological Survey, Centre for Environmental Geochemistry, Keyworth, Nottingham NG12 5GG, UK
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  surname: Moss-Hayes
  fullname: Moss-Hayes, Vicky
  organization: British Geological Survey, Centre for Environmental Geochemistry, Keyworth, Nottingham NG12 5GG, UK
– sequence: 7
  givenname: Paul C.
  surname: Nathanail
  fullname: Nathanail, Paul C.
  organization: University of Nottingham, School of Geography, University of Nottingham, Nottingham NG7 2RD, UK
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Keywords PCBs
concentration
polycyclic aromatic hydrocarbons
soils
Language English
License http://creativecommons.org/licenses/by/3.0
CC BY 4.0
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  year: 2014
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PublicationTitle Applied geochemistry
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Snippet •London soil PAH concentrations are comparable with other cities.•London soil PCB concentrations are higher than other cities.•London soils contain multiple...
Surface soils from a 19km2 area in east London, UK were analysed for polycyclic aromatic hydrocarbons (PAH) and polychlorinated biphenyls (PCB) (n=76). ∑16 PAH...
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SubjectTerms benzo(a)pyrene
cities
Earth sciences
Earth, ocean, space
Engineering and environment geology. Geothermics
Exact sciences and technology
Geochemistry
human health
Pollution, environment geology
polychlorinated biphenyls
polycyclic aromatic hydrocarbons
United Kingdom
urban soils
Title Polycyclic aromatic hydrocarbons (PAH) and polychlorinated biphenyls (PCB) in urban soils of Greater London, UK
URI https://dx.doi.org/10.1016/j.apgeochem.2014.09.013
https://www.proquest.com/docview/2000135196
Volume 51
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