Sodium-Ion Hybrid Capacitor of High Power and Energy Density
Sodium-ion hybrid capacitors (NHCs) have been attracting research interest in recent years. However, NHCs suffer from slower redox reaction kinetics of electrodes as compared to non-Faradaic capacitive counterparts. Herein, a high-performance NHC using porous NaBi as anode, activated carbon (AC) as...
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| Published in | ACS central science Vol. 4; no. 9; pp. 1261 - 1265 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
26.09.2018
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| Online Access | Get full text |
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| Abstract | Sodium-ion hybrid capacitors (NHCs) have been attracting research interest in recent years. However, NHCs suffer from slower redox reaction kinetics of electrodes as compared to non-Faradaic capacitive counterparts. Herein, a high-performance NHC using porous NaBi as anode, activated carbon (AC) as cathode, and 1.5 M of NaPF6 in diglyme as electrolyte is reported. In a charging process, Na+ is inserted into NaBi to form Na3Bi, and PF6 – is stored in the electric double layers of the AC cathode; in a reverse process, the Na3Bi is desodiated to NaBi and eventually Bi, and the adsorbed PF6 – is released into the electrolyte in the first cycle. The NHC exhibits a capacity of ∼298 mA h gBi –1, capacity retention of 98.6% after 1000 cycles at 2 A gBi –1, and Coulombic efficiency of >99.4%. The achievable power and energy density are as high as 11.1 kW kgtotal –1 and 106.5 W h kgtotal –1, respectively. The superior electrochemical performance is ascribed to the gradually formed three-dimensional (3D) porous and stable networks of the anode, ensuring its comparable fast reaction kinetics and cycle stability to the AC cathode. |
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| AbstractList | Sodium-ion hybrid
capacitors (NHCs) have been attracting research
interest in recent years. However, NHCs suffer from slower redox reaction
kinetics of electrodes as compared to non-Faradaic capacitive counterparts.
Herein, a high-performance NHC using porous NaBi as anode, activated
carbon (AC) as cathode, and 1.5 M of NaPF
6
in diglyme as
electrolyte is reported. In a charging process, Na
+
is
inserted into NaBi to form Na
3
Bi, and PF
6
–
is stored in the electric double layers of the AC
cathode; in a reverse process, the Na
3
Bi is desodiated
to NaBi and eventually Bi, and the adsorbed PF
6
–
is released into the electrolyte in the first cycle. The NHC exhibits
a capacity of ∼298 mA h g
Bi
–1
,
capacity retention of 98.6% after 1000 cycles at 2 A g
Bi
–1
, and Coulombic efficiency of >99.4%. The
achievable
power and energy density are as high as 11.1 kW kg
total
–1
and 106.5 W h kg
total
–1
, respectively. The superior electrochemical performance is ascribed
to the gradually formed three-dimensional (3D) porous and stable networks
of the anode, ensuring its comparable fast reaction kinetics and cycle
stability to the AC cathode.
A sodium-ion hybrid capacitor
with high power and energy
density is reported on the basis of a NaBi anode with fast kinetics,
which bridges the performance gap between batteries and supercapacitors. Sodium-ion hybrid capacitors (NHCs) have been attracting research interest in recent years. However, NHCs suffer from slower redox reaction kinetics of electrodes as compared to non-Faradaic capacitive counterparts. Herein, a high-performance NHC using porous NaBi as anode, activated carbon (AC) as cathode, and 1.5 M of NaPF6 in diglyme as electrolyte is reported. In a charging process, Na+ is inserted into NaBi to form Na3Bi, and PF6 – is stored in the electric double layers of the AC cathode; in a reverse process, the Na3Bi is desodiated to NaBi and eventually Bi, and the adsorbed PF6 – is released into the electrolyte in the first cycle. The NHC exhibits a capacity of ∼298 mA h gBi –1, capacity retention of 98.6% after 1000 cycles at 2 A gBi –1, and Coulombic efficiency of >99.4%. The achievable power and energy density are as high as 11.1 kW kgtotal –1 and 106.5 W h kgtotal –1, respectively. The superior electrochemical performance is ascribed to the gradually formed three-dimensional (3D) porous and stable networks of the anode, ensuring its comparable fast reaction kinetics and cycle stability to the AC cathode. Sodium-ion hybrid capacitors (NHCs) have been attracting research interest in recent years. However, NHCs suffer from slower redox reaction kinetics of electrodes as compared to non-Faradaic capacitive counterparts. Herein, a high-performance NHC using porous NaBi as anode, activated carbon (AC) as cathode, and 1.5 M of NaPF in diglyme as electrolyte is reported. In a charging process, Na is inserted into NaBi to form Na Bi, and PF is stored in the electric double layers of the AC cathode; in a reverse process, the Na Bi is desodiated to NaBi and eventually Bi, and the adsorbed PF is released into the electrolyte in the first cycle. The NHC exhibits a capacity of ∼298 mA h g , capacity retention of 98.6% after 1000 cycles at 2 A g , and Coulombic efficiency of >99.4%. The achievable power and energy density are as high as 11.1 kW kg and 106.5 W h kg , respectively. The superior electrochemical performance is ascribed to the gradually formed three-dimensional (3D) porous and stable networks of the anode, ensuring its comparable fast reaction kinetics and cycle stability to the AC cathode. |
| Author | Chen, Jun Li, Fujun Wang, Chenchen Yuan, Yue Lei, Kaixiang Li, Haixia |
| AuthorAffiliation | Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education), College of Chemistry |
| AuthorAffiliation_xml | – name: Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education), College of Chemistry |
| Author_xml | – sequence: 1 givenname: Yue surname: Yuan fullname: Yuan, Yue – sequence: 2 givenname: Chenchen surname: Wang fullname: Wang, Chenchen – sequence: 3 givenname: Kaixiang surname: Lei fullname: Lei, Kaixiang – sequence: 4 givenname: Haixia surname: Li fullname: Li, Haixia – sequence: 5 givenname: Fujun orcidid: 0000-0002-1298-0267 surname: Li fullname: Li, Fujun email: fujunli@nankai.edu.cn – sequence: 6 givenname: Jun orcidid: 0000-0001-8604-9689 surname: Chen fullname: Chen, Jun |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30276261$$D View this record in MEDLINE/PubMed |
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| Snippet | Sodium-ion hybrid capacitors (NHCs) have been attracting research interest in recent years. However, NHCs suffer from slower redox reaction kinetics of... Sodium-ion hybrid capacitors (NHCs) have been attracting research interest in recent years. However, NHCs suffer from slower redox reaction kinetics of... |
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| Title | Sodium-Ion Hybrid Capacitor of High Power and Energy Density |
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