Biodegradable and Insoluble Cellulose Photonic Crystals and Metasurfaces
The replacement of plastic with eco-friendly and biodegradable materials is one of the most stringent environmental challenges. In this respect, cellulose stands out as a biodegradable polymer. However, a significant challenge is to obtain biodegradable materials for high-end photonics that are robu...
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| Published in | ACS nano Vol. 14; no. 8; pp. 9502 - 9511 |
|---|---|
| Main Authors | , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
25.08.2020
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The replacement of plastic with eco-friendly and biodegradable materials is one of the most stringent environmental challenges. In this respect, cellulose stands out as a biodegradable polymer. However, a significant challenge is to obtain biodegradable materials for high-end photonics that are robust in humid environments. Here, we demonstrate the fabrication of high-quality micro- and nanoscale photonic and plasmonic structures via replica molding using pure cellulose and a blended version with nonedible agro-wastes. Both materials are biodegradable in soil and seawater according to the ISO 17556 standard. The pure cellulose films are transparent in the vis–NIR spectrum, having a refractive index similar to glass. The microstructured photonic crystals show high-quality diffractive properties that are maintained under extended exposure to water. Nanostructuring the cellulose transforms it to a biodegradable metasurface manifesting bright structural colors. A subsequent deposition of Ag endowed the metasurface with plasmonic properties used to produce plasmonic colors and for surface-enhanced Raman scattering. |
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| AbstractList | The
replacement of plastic with eco-friendly and biodegradable
materials is one of the most stringent environmental challenges. In
this respect, cellulose stands out as a biodegradable polymer. However,
a significant challenge is to obtain biodegradable materials for high-end
photonics that are robust in humid environments. Here, we demonstrate
the fabrication of high-quality micro- and nanoscale photonic and
plasmonic structures
via
replica molding using pure
cellulose and a blended version with nonedible agro-wastes. Both materials
are biodegradable in soil and seawater according to the ISO 17556
standard. The pure cellulose films are transparent in the vis–NIR
spectrum, having a refractive index similar to glass. The microstructured
photonic crystals show high-quality diffractive properties that are
maintained under extended exposure to water. Nanostructuring the cellulose
transforms it to a biodegradable metasurface manifesting bright structural
colors. A subsequent deposition of Ag endowed the metasurface with
plasmonic properties used to produce plasmonic colors and for surface-enhanced
Raman scattering. The replacement of plastic with eco-friendly and biodegradable materials is one of the most stringent environmental challenges. In this respect, cellulose stands out as a biodegradable polymer. However, a significant challenge is to obtain biodegradable materials for high-end photonics that are robust in humid environments. Here, we demonstrate the fabrication of high-quality micro- and nanoscale photonic and plasmonic structures replica molding using pure cellulose and a blended version with nonedible agro-wastes. Both materials are biodegradable in soil and seawater according to the ISO 17556 standard. The pure cellulose films are transparent in the vis-NIR spectrum, having a refractive index similar to glass. The microstructured photonic crystals show high-quality diffractive properties that are maintained under extended exposure to water. Nanostructuring the cellulose transforms it to a biodegradable metasurface manifesting bright structural colors. A subsequent deposition of Ag endowed the metasurface with plasmonic properties used to produce plasmonic colors and for surface-enhanced Raman scattering. The replacement of plastic with eco-friendly and biodegradable materials is one of the most stringent environmental challenges. In this respect, cellulose stands out as a biodegradable polymer. However, a significant challenge is to obtain biodegradable materials for high-end photonics that are robust in humid environments. Here, we demonstrate the fabrication of high-quality micro- and nanoscale photonic and plasmonic structures via replica molding using pure cellulose and a blended version with nonedible agro-wastes. Both materials are biodegradable in soil and seawater according to the ISO 17556 standard. The pure cellulose films are transparent in the vis–NIR spectrum, having a refractive index similar to glass. The microstructured photonic crystals show high-quality diffractive properties that are maintained under extended exposure to water. Nanostructuring the cellulose transforms it to a biodegradable metasurface manifesting bright structural colors. A subsequent deposition of Ag endowed the metasurface with plasmonic properties used to produce plasmonic colors and for surface-enhanced Raman scattering. |
| Author | Heredia-Guerrero, José Alejandro Martin-Garcia, Beatriz Cingolani, Roberto Hedayati, Mehdi Keshavarz Guzman-Puyol, Susana Palei, Milan Caligiuri, Vincenzo Athanassiou, Athanassia Bonaccorso, Francesco Salerno, Marco Miscuglio, Mario Krahne, Roman Tedeschi, Giacomo Sorger, Volker J Kristensen, Anders |
| AuthorAffiliation | Dipartimento di Fisica Department of Health Technology Department of Electrical Engineering Materials Characterization Facility Department of Electrical and Computer Engineering BeDimensional Srl Istituto Italiano di Tecnologia Università della Calabria IHSM La Mayora, Departamento de Mejora Genética y Biotecnología Department of Engineering CNR Nanotec |
| AuthorAffiliation_xml | – name: Istituto Italiano di Tecnologia – name: CNR Nanotec – name: Materials Characterization Facility – name: Dipartimento di Fisica – name: Università della Calabria – name: Department of Electrical and Computer Engineering – name: Department of Health Technology – name: Department of Electrical Engineering – name: IHSM La Mayora, Departamento de Mejora Genética y Biotecnología – name: Department of Engineering – name: BeDimensional Srl |
| Author_xml | – sequence: 1 givenname: Vincenzo orcidid: 0000-0003-1035-4702 surname: Caligiuri fullname: Caligiuri, Vincenzo email: vincenzo.caligiuri@unical.it organization: Università della Calabria – sequence: 2 givenname: Giacomo orcidid: 0000-0002-7232-7235 surname: Tedeschi fullname: Tedeschi, Giacomo – sequence: 3 givenname: Milan orcidid: 0000-0003-4387-5184 surname: Palei fullname: Palei, Milan organization: Department of Electrical Engineering – sequence: 4 givenname: Mario orcidid: 0000-0001-5953-8452 surname: Miscuglio fullname: Miscuglio, Mario organization: Department of Electrical and Computer Engineering – sequence: 5 givenname: Beatriz orcidid: 0000-0001-7065-856X surname: Martin-Garcia fullname: Martin-Garcia, Beatriz – sequence: 6 givenname: Susana surname: Guzman-Puyol fullname: Guzman-Puyol, Susana organization: IHSM La Mayora, Departamento de Mejora Genética y Biotecnología – sequence: 7 givenname: Mehdi Keshavarz surname: Hedayati fullname: Hedayati, Mehdi Keshavarz organization: Department of Engineering – sequence: 8 givenname: Anders surname: Kristensen fullname: Kristensen, Anders organization: Department of Health Technology – sequence: 9 givenname: Athanassia orcidid: 0000-0002-6533-3231 surname: Athanassiou fullname: Athanassiou, Athanassia – sequence: 10 givenname: Roberto surname: Cingolani fullname: Cingolani, Roberto – sequence: 11 givenname: Volker J orcidid: 0000-0002-5152-4766 surname: Sorger fullname: Sorger, Volker J organization: Department of Electrical and Computer Engineering – sequence: 12 givenname: Marco surname: Salerno fullname: Salerno, Marco organization: Istituto Italiano di Tecnologia – sequence: 13 givenname: Francesco orcidid: 0000-0001-7238-9420 surname: Bonaccorso fullname: Bonaccorso, Francesco organization: BeDimensional Srl – sequence: 14 givenname: Roman orcidid: 0000-0003-0066-7019 surname: Krahne fullname: Krahne, Roman – sequence: 15 givenname: José Alejandro orcidid: 0000-0002-8251-7577 surname: Heredia-Guerrero fullname: Heredia-Guerrero, José Alejandro email: ja.heredia@csic.es organization: IHSM La Mayora, Departamento de Mejora Genética y Biotecnología |
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| Keywords | biodegradability cellulose SERS cocoa agro-waste plasmonic colors water insolubility photonic crystals meta-structures |
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| Title | Biodegradable and Insoluble Cellulose Photonic Crystals and Metasurfaces |
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