Cyclic Formation Stability of 1,1,1,2-Tetrafluoroethane Hydrate in Different SDS Solution Systems and Dissociation Characteristics Using Thermal Stimulation Combined with Depressurization
Cold storage using hydrates for cooling is a high-efficiency technology. However, this technology suffers from problems such as the stochastic nature of hydrate nucleation, cyclic hydrate formation instability, and a low cold discharge rate. To solve these problems, it is necessary to further clarif...
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| Published in | ACS omega Vol. 4; no. 7; pp. 11397 - 11407 |
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| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
31.07.2019
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| Abstract | Cold storage using hydrates for cooling is a high-efficiency technology. However, this technology suffers from problems such as the stochastic nature of hydrate nucleation, cyclic hydrate formation instability, and a low cold discharge rate. To solve these problems, it is necessary to further clarify the characteristics of hydrate formation and dissociation in different systems. First, a comparative experimental study in pure water and sodium dodecyl sulfate (SDS) solution systems was conducted to explore the influence of SDS on the morphology of the hydrate and the time needed for its formation under visualization conditions. Subsequently, the cyclic hydrate formation stability was investigated at different test temperatures with two types of SDS solution systemswith or without a porous medium. The induction time, full time, and energy consumption time ratio of the first hydrate formation process and the cyclic hydrate reformation process were analyzed. Finally, thermal stimulation combined with depressurization was used to intensify hydrate dissociation compared with single thermal stimulation. The results showed that the growth morphology of hydrate and the time required for its formation in the SDS solution system were obviously different than those in pure water. In addition, the calculation and comparison results revealed that the induction time and full time of cyclic hydrate reformation were shorter and the energy consumption time ratio was smaller in the porous medium. The results indicated that a porous medium could improve the cyclic hydrate formation process by making it more stable and by decreasing time and energy costs. Thermal stimulation combined with depressurization at different backpressures (0.1, 0.2, 0.3, and 0.4 MPa) effectively promoted the decomposition of hydrates, and with the decrease in backpressure, the dissociation time decreased gradually. At a backpressure of 0.1 MPa, the dissociation time was reduced by 150 min. The experimental results presented the formation and dissociation characteristics of 1,1,1,2-tetrafluoroethane hydrates in different systems, which could accelerate the application of gas hydrates in cold storage. |
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| AbstractList | Cold storage using hydrates for cooling is a high-efficiency technology. However, this technology suffers from problems such as the stochastic nature of hydrate nucleation, cyclic hydrate formation instability, and a low cold discharge rate. To solve these problems, it is necessary to further clarify the characteristics of hydrate formation and dissociation in different systems. First, a comparative experimental study in pure water and sodium dodecyl sulfate (SDS) solution systems was conducted to explore the influence of SDS on the morphology of the hydrate and the time needed for its formation under visualization conditions. Subsequently, the cyclic hydrate formation stability was investigated at different test temperatures with two types of SDS solution systemswith or without a porous medium. The induction time, full time, and energy consumption time ratio of the first hydrate formation process and the cyclic hydrate reformation process were analyzed. Finally, thermal stimulation combined with depressurization was used to intensify hydrate dissociation compared with single thermal stimulation. The results showed that the growth morphology of hydrate and the time required for its formation in the SDS solution system were obviously different than those in pure water. In addition, the calculation and comparison results revealed that the induction time and full time of cyclic hydrate reformation were shorter and the energy consumption time ratio was smaller in the porous medium. The results indicated that a porous medium could improve the cyclic hydrate formation process by making it more stable and by decreasing time and energy costs. Thermal stimulation combined with depressurization at different backpressures (0.1, 0.2, 0.3, and 0.4 MPa) effectively promoted the decomposition of hydrates, and with the decrease in backpressure, the dissociation time decreased gradually. At a backpressure of 0.1 MPa, the dissociation time was reduced by 150 min. The experimental results presented the formation and dissociation characteristics of 1,1,1,2-tetrafluoroethane hydrates in different systems, which could accelerate the application of gas hydrates in cold storage. Cold storage using hydrates for cooling is a high-efficiency technology. However, this technology suffers from problems such as the stochastic nature of hydrate nucleation, cyclic hydrate formation instability, and a low cold discharge rate. To solve these problems, it is necessary to further clarify the characteristics of hydrate formation and dissociation in different systems. First, a comparative experimental study in pure water and sodium dodecyl sulfate (SDS) solution systems was conducted to explore the influence of SDS on the morphology of the hydrate and the time needed for its formation under visualization conditions. Subsequently, the cyclic hydrate formation stability was investigated at different test temperatures with two types of SDS solution systems-with or without a porous medium. The induction time, full time, and energy consumption time ratio of the first hydrate formation process and the cyclic hydrate reformation process were analyzed. Finally, thermal stimulation combined with depressurization was used to intensify hydrate dissociation compared with single thermal stimulation. The results showed that the growth morphology of hydrate and the time required for its formation in the SDS solution system were obviously different than those in pure water. In addition, the calculation and comparison results revealed that the induction time and full time of cyclic hydrate reformation were shorter and the energy consumption time ratio was smaller in the porous medium. The results indicated that a porous medium could improve the cyclic hydrate formation process by making it more stable and by decreasing time and energy costs. Thermal stimulation combined with depressurization at different backpressures (0.1, 0.2, 0.3, and 0.4 MPa) effectively promoted the decomposition of hydrates, and with the decrease in backpressure, the dissociation time decreased gradually. At a backpressure of 0.1 MPa, the dissociation time was reduced by 150 min. The experimental results presented the formation and dissociation characteristics of 1,1,1,2-tetrafluoroethane hydrates in different systems, which could accelerate the application of gas hydrates in cold storage. Cold storage using hydrates for cooling is a high-efficiency technology. However, this technology suffers from problems such as the stochastic nature of hydrate nucleation, cyclic hydrate formation instability, and a low cold discharge rate. To solve these problems, it is necessary to further clarify the characteristics of hydrate formation and dissociation in different systems. First, a comparative experimental study in pure water and sodium dodecyl sulfate (SDS) solution systems was conducted to explore the influence of SDS on the morphology of the hydrate and the time needed for its formation under visualization conditions. Subsequently, the cyclic hydrate formation stability was investigated at different test temperatures with two types of SDS solution systems—with or without a porous medium. The induction time, full time, and energy consumption time ratio of the first hydrate formation process and the cyclic hydrate reformation process were analyzed. Finally, thermal stimulation combined with depressurization was used to intensify hydrate dissociation compared with single thermal stimulation. The results showed that the growth morphology of hydrate and the time required for its formation in the SDS solution system were obviously different than those in pure water. In addition, the calculation and comparison results revealed that the induction time and full time of cyclic hydrate reformation were shorter and the energy consumption time ratio was smaller in the porous medium. The results indicated that a porous medium could improve the cyclic hydrate formation process by making it more stable and by decreasing time and energy costs. Thermal stimulation combined with depressurization at different backpressures (0.1, 0.2, 0.3, and 0.4 MPa) effectively promoted the decomposition of hydrates, and with the decrease in backpressure, the dissociation time decreased gradually. At a backpressure of 0.1 MPa, the dissociation time was reduced by 150 min. The experimental results presented the formation and dissociation characteristics of 1,1,1,2-tetrafluoroethane hydrates in different systems, which could accelerate the application of gas hydrates in cold storage. |
| Author | Jin, Tingxiang Lv, Shuai Cheng, Chuanxiao Qi, Tian Li, Lun Zhao, Jiafei Zheng, Jili Wang, Fan Zhang, Jun Li, Lingjuan Yang, Penglin |
| AuthorAffiliation | School of Energy and Power Engineering Henan Muxiang Veterinary Pharmaceutical Company Limited Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education |
| AuthorAffiliation_xml | – name: Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education – name: Henan Muxiang Veterinary Pharmaceutical Company Limited – name: School of Energy and Power Engineering |
| Author_xml | – sequence: 1 givenname: Chuanxiao orcidid: 0000-0001-5057-6364 surname: Cheng fullname: Cheng, Chuanxiao organization: School of Energy and Power Engineering – sequence: 2 givenname: Fan orcidid: 0000-0001-5068-5309 surname: Wang fullname: Wang, Fan organization: School of Energy and Power Engineering – sequence: 3 givenname: Jun surname: Zhang fullname: Zhang, Jun organization: School of Energy and Power Engineering – sequence: 4 givenname: Tian surname: Qi fullname: Qi, Tian organization: School of Energy and Power Engineering – sequence: 5 givenname: Tingxiang orcidid: 0000-0001-8883-8294 surname: Jin fullname: Jin, Tingxiang email: txjin@126.com organization: School of Energy and Power Engineering – sequence: 6 givenname: Jiafei orcidid: 0000-0001-8401-4204 surname: Zhao fullname: Zhao, Jiafei email: jfzhao@dlut.edu.cn organization: Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education – sequence: 7 givenname: Jili surname: Zheng fullname: Zheng, Jili organization: School of Energy and Power Engineering – sequence: 8 givenname: Lingjuan surname: Li fullname: Li, Lingjuan organization: Henan Muxiang Veterinary Pharmaceutical Company Limited – sequence: 9 givenname: Lun surname: Li fullname: Li, Lun organization: School of Energy and Power Engineering – sequence: 10 givenname: Penglin surname: Yang fullname: Yang, Penglin organization: School of Energy and Power Engineering – sequence: 11 givenname: Shuai surname: Lv fullname: Lv, Shuai organization: School of Energy and Power Engineering |
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| CitedBy_id | crossref_primary_10_1021_acs_jced_1c00139 crossref_primary_10_1016_j_est_2022_103980 crossref_primary_10_1021_acsomega_3c04578 crossref_primary_10_1021_acs_energyfuels_3c03559 crossref_primary_10_1016_j_rser_2019_109492 crossref_primary_10_1021_acsomega_9b02497 crossref_primary_10_1016_j_fuel_2023_129249 crossref_primary_10_1016_j_fuel_2020_118908 crossref_primary_10_1016_j_applthermaleng_2022_118462 crossref_primary_10_1016_j_est_2024_111127 crossref_primary_10_1016_j_fuel_2021_122080 crossref_primary_10_1016_j_energy_2020_119374 crossref_primary_10_1016_j_fuel_2023_130483 crossref_primary_10_1016_j_energy_2022_124647 |
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| Title | Cyclic Formation Stability of 1,1,1,2-Tetrafluoroethane Hydrate in Different SDS Solution Systems and Dissociation Characteristics Using Thermal Stimulation Combined with Depressurization |
| URI | http://dx.doi.org/10.1021/acsomega.9b01187 https://www.ncbi.nlm.nih.gov/pubmed/31460244 https://search.proquest.com/docview/2281841308 https://pubmed.ncbi.nlm.nih.gov/PMC6682015 https://doaj.org/article/c3865abe4c2e4889b3517d95e1b1f474 |
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