Characterizing Properties and Environmental Behaviors of Dissolved Organic Matter Using Two-Dimensional Correlation Spectroscopic Analysis
Dissolved organic matter (DOM) exists ubiquitously in environments and plays critical roles in pollutant mitigation, transformation, and organic geochemical cycling. Understanding its properties and environmental behaviors is critically important to develop water treatment processes and environmenta...
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| Published in | Environmental science & technology Vol. 53; no. 9; pp. 4683 - 4694 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
07.05.2019
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Dissolved organic matter (DOM) exists ubiquitously in environments and plays critical roles in pollutant mitigation, transformation, and organic geochemical cycling. Understanding its properties and environmental behaviors is critically important to develop water treatment processes and environmental remediation strategies. Generalized two-dimensional correlation spectroscopy (2DCOS), which has numerous advantages, including enhancing spectral resolution and discerning specific order of structural change under an external perturbation, could be used as a powerful tool to interpret a wide range of spectroscopic signatures relating to DOM. A suite of spectroscopic signatures, such as UV–vis, fluorescence, infrared, and Raman spectra that can be analyzed by 2DCOS, is able to provide additional structural information hiding behind the conventional one-dimensional spectra. In this article, the most recent advances in 2DCOS applications for analyzing DOM-related environmental processes are reviewed, and the state-of-the-art novel spectroscopic techniques in 2DCOS are highlighted. Furthermore, the main limitations and requirements of current approaches for exploring DOM-related environmental processes and how these limitations and drawbacks can be addressed are explored. Finally, suggestions and new approaches are proposed to significantly advance the development of 2DCOS in analyzing the properties and behaviors of DOM in natural and engineered environments. |
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| AbstractList | Dissolved organic matter (DOM) exists ubiquitously in environments and plays critical roles in pollutant mitigation, transformation, and organic geochemical cycling. Understanding its properties and environmental behaviors is critically important to develop water treatment processes and environmental remediation strategies. Generalized two-dimensional correlation spectroscopy (2DCOS), which has numerous advantages, including enhancing spectral resolution and discerning specific order of structural change under an external perturbation, could be used as a powerful tool to interpret a wide range of spectroscopic signatures relating to DOM. A suite of spectroscopic signatures, such as UV-vis, fluorescence, infrared, and Raman spectra that can be analyzed by 2DCOS, is able to provide additional structural information hiding behind the conventional one-dimensional spectra. In this article, the most recent advances in 2DCOS applications for analyzing DOM-related environmental processes are reviewed, and the state-of-the-art novel spectroscopic techniques in 2DCOS are highlighted. Furthermore, the main limitations and requirements of current approaches for exploring DOM-related environmental processes and how these limitations and drawbacks can be addressed are explored. Finally, suggestions and new approaches are proposed to significantly advance the development of 2DCOS in analyzing the properties and behaviors of DOM in natural and engineered environments. Dissolved organic matter (DOM) exists ubiquitously in environments and plays critical roles in pollutant mitigation, transformation, and organic geochemical cycling. Understanding its properties and environmental behaviors is critically important to develop water treatment processes and environmental remediation strategies. Generalized two-dimensional correlation spectroscopy (2DCOS), which has numerous advantages, including enhancing spectral resolution and discerning specific order of structural change under an external perturbation, could be used as a powerful tool to interpret a wide range of spectroscopic signatures relating to DOM. A suite of spectroscopic signatures, such as UV-vis, fluorescence, infrared, and Raman spectra that can be analyzed by 2DCOS, is able to provide additional structural information hiding behind the conventional one-dimensional spectra. In this article, the most recent advances in 2DCOS applications for analyzing DOM-related environmental processes are reviewed, and the state-of-the-art novel spectroscopic techniques in 2DCOS are highlighted. Furthermore, the main limitations and requirements of current approaches for exploring DOM-related environmental processes and how these limitations and drawbacks can be addressed are explored. Finally, suggestions and new approaches are proposed to significantly advance the development of 2DCOS in analyzing the properties and behaviors of DOM in natural and engineered environments.Dissolved organic matter (DOM) exists ubiquitously in environments and plays critical roles in pollutant mitigation, transformation, and organic geochemical cycling. Understanding its properties and environmental behaviors is critically important to develop water treatment processes and environmental remediation strategies. Generalized two-dimensional correlation spectroscopy (2DCOS), which has numerous advantages, including enhancing spectral resolution and discerning specific order of structural change under an external perturbation, could be used as a powerful tool to interpret a wide range of spectroscopic signatures relating to DOM. A suite of spectroscopic signatures, such as UV-vis, fluorescence, infrared, and Raman spectra that can be analyzed by 2DCOS, is able to provide additional structural information hiding behind the conventional one-dimensional spectra. In this article, the most recent advances in 2DCOS applications for analyzing DOM-related environmental processes are reviewed, and the state-of-the-art novel spectroscopic techniques in 2DCOS are highlighted. Furthermore, the main limitations and requirements of current approaches for exploring DOM-related environmental processes and how these limitations and drawbacks can be addressed are explored. Finally, suggestions and new approaches are proposed to significantly advance the development of 2DCOS in analyzing the properties and behaviors of DOM in natural and engineered environments. |
| Author | Chen, Wei Teng, Chun-Ying Qian, Chen Yu, Han-Qing |
| AuthorAffiliation | School of Metallurgy and Environment CAS Key Laboratory of Urban Pollutant Conversion, Department of Applied Chemistry |
| AuthorAffiliation_xml | – name: School of Metallurgy and Environment – name: CAS Key Laboratory of Urban Pollutant Conversion, Department of Applied Chemistry |
| Author_xml | – sequence: 1 givenname: Wei surname: Chen fullname: Chen, Wei organization: CAS Key Laboratory of Urban Pollutant Conversion, Department of Applied Chemistry – sequence: 2 givenname: Chun-Ying surname: Teng fullname: Teng, Chun-Ying organization: School of Metallurgy and Environment – sequence: 3 givenname: Chen surname: Qian fullname: Qian, Chen organization: CAS Key Laboratory of Urban Pollutant Conversion, Department of Applied Chemistry – sequence: 4 givenname: Han-Qing orcidid: 0000-0001-5247-6244 surname: Yu fullname: Yu, Han-Qing email: hqyu@ustc.edu.cn organization: CAS Key Laboratory of Urban Pollutant Conversion, Department of Applied Chemistry |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30998320$$D View this record in MEDLINE/PubMed |
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| Snippet | Dissolved organic matter (DOM) exists ubiquitously in environments and plays critical roles in pollutant mitigation, transformation, and organic geochemical... |
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| SubjectTerms | Correlation analysis Dissolved organic matter Environmental behavior Environmental cleanup Environmental Restoration and Remediation Fluorescence Humic Substances Infrared analysis Infrared signatures Infrared spectra pollutants Pollution control Properties (attributes) Raman spectra Raman spectroscopy remediation spectral analysis Spectral resolution Spectrometry, Fluorescence Spectroscopy, Fourier Transform Infrared Spectrum analysis State-of-the-art reviews Two dimensional analysis ultraviolet-visible spectroscopy Water treatment |
| Title | Characterizing Properties and Environmental Behaviors of Dissolved Organic Matter Using Two-Dimensional Correlation Spectroscopic Analysis |
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