Superprotonic Conductivity of Guanidinium Organosulfonate Hydrogen-Bonded Organic Frameworks with Nanotube-Shaped Proton Transport Channels
Grasping proton transport pathways and mechanisms is vital for the application of fuel cell technology. Herein, we screened four guanidinium organosulfonate charge-assisted hydrogen-bonded organic frameworks (HOFs), namely, GBBS, G 3 TSPHB, G 4 TSP, and G 6 HSPB, which possess high hydrogen-bonded d...
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| Published in | Precision Chemistry Vol. 1; no. 10; pp. 608 - 615 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
University of Science and Technology of China and American Chemical Society
25.12.2023
American Chemical Society |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Grasping proton transport pathways and mechanisms is vital for the application of fuel cell technology. Herein, we screened four guanidinium organosulfonate charge-assisted hydrogen-bonded organic frameworks (HOFs), namely, GBBS, G 3 TSPHB, G 4 TSP, and G 6 HSPB, which possess high hydrogen-bonded density proton transport networks shaped like nanotubes. These materials were prepared by self-assembly through charge-assisted interactions between guanidinium cations and organosulfonate anions, as well as by host–guest regulation. At 80 °C and 93% RH, the proton conductivity of GBBS, G 3 TSPHB, G 4 TSP, and G 6 HSPB can reach 4.56 × 10–2, 2.55 × 10–2, 4.01 × 10–2, and 1.2 × 10–1 S cm–1, respectively, with superprotonic conductivity. Doping G 6 HSPB into the Nafion matrix prepared composite membranes for testing the performance of fuel cells. At 80 °C and 98% RH, the proton conductivity of 9%-G 6 HSPB@Nafion reached a maximum value of 1.14 × 10–1 S cm–1, which is 2.8 times higher than recast Nafion. The results showed that charge-assisted HOFs with high proton channel density have better proton transport properties, providing a reference for the design of highly proton-conducting materials. |
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| AbstractList | Grasping proton transport pathways and mechanisms is vital for the application of fuel cell technology. Herein, we screened four guanidinium organosulfonate charge-assisted hydrogen-bonded organic frameworks (HOFs), namely, GBBS, G 3 TSPHB, G 4 TSP, and G 6 HSPB, which possess high hydrogen-bonded density proton transport networks shaped like nanotubes. These materials were prepared by self-assembly through charge-assisted interactions between guanidinium cations and organosulfonate anions, as well as by host-guest regulation. At 80 °C and 93% RH, the proton conductivity of GBBS, G 3 TSPHB, G 4 TSP, and G 6 HSPB can reach 4.56 × 10-2, 2.55 × 10-2, 4.01 × 10-2, and 1.2 × 10-1 S cm-1, respectively, with superprotonic conductivity. Doping G 6 HSPB into the Nafion matrix prepared composite membranes for testing the performance of fuel cells. At 80 °C and 98% RH, the proton conductivity of 9%-G 6 HSPB@Nafion reached a maximum value of 1.14 × 10-1 S cm-1, which is 2.8 times higher than recast Nafion. The results showed that charge-assisted HOFs with high proton channel density have better proton transport properties, providing a reference for the design of highly proton-conducting materials.Grasping proton transport pathways and mechanisms is vital for the application of fuel cell technology. Herein, we screened four guanidinium organosulfonate charge-assisted hydrogen-bonded organic frameworks (HOFs), namely, GBBS, G 3 TSPHB, G 4 TSP, and G 6 HSPB, which possess high hydrogen-bonded density proton transport networks shaped like nanotubes. These materials were prepared by self-assembly through charge-assisted interactions between guanidinium cations and organosulfonate anions, as well as by host-guest regulation. At 80 °C and 93% RH, the proton conductivity of GBBS, G 3 TSPHB, G 4 TSP, and G 6 HSPB can reach 4.56 × 10-2, 2.55 × 10-2, 4.01 × 10-2, and 1.2 × 10-1 S cm-1, respectively, with superprotonic conductivity. Doping G 6 HSPB into the Nafion matrix prepared composite membranes for testing the performance of fuel cells. At 80 °C and 98% RH, the proton conductivity of 9%-G 6 HSPB@Nafion reached a maximum value of 1.14 × 10-1 S cm-1, which is 2.8 times higher than recast Nafion. The results showed that charge-assisted HOFs with high proton channel density have better proton transport properties, providing a reference for the design of highly proton-conducting materials. Grasping proton transport pathways and mechanisms is vital for the application of fuel cell technology. Herein, we screened four guanidinium organosulfonate charge-assisted hydrogen-bonded organic frameworks (HOFs), namely, GBBS, G 3 TSPHB, G 4 TSP, and G 6 HSPB, which possess high hydrogen-bonded density proton transport networks shaped like nanotubes. These materials were prepared by self-assembly through charge-assisted interactions between guanidinium cations and organosulfonate anions, as well as by host–guest regulation. At 80 °C and 93% RH, the proton conductivity of GBBS, G 3 TSPHB, G 4 TSP, and G 6 HSPB can reach 4.56 × 10–2, 2.55 × 10–2, 4.01 × 10–2, and 1.2 × 10–1 S cm–1, respectively, with superprotonic conductivity. Doping G 6 HSPB into the Nafion matrix prepared composite membranes for testing the performance of fuel cells. At 80 °C and 98% RH, the proton conductivity of 9%-G 6 HSPB@Nafion reached a maximum value of 1.14 × 10–1 S cm–1, which is 2.8 times higher than recast Nafion. The results showed that charge-assisted HOFs with high proton channel density have better proton transport properties, providing a reference for the design of highly proton-conducting materials. Grasping proton transport pathways and mechanisms is vital for the application of fuel cell technology. Herein, we screened four guanidinium organosulfonate charge-assisted hydrogen-bonded organic frameworks (HOFs), namely, , , , and , which possess high hydrogen-bonded density proton transport networks shaped like nanotubes. These materials were prepared by self-assembly through charge-assisted interactions between guanidinium cations and organosulfonate anions, as well as by host-guest regulation. At 80 °C and 93% RH, the proton conductivity of , , , and can reach 4.56 × 10 , 2.55 × 10 , 4.01 × 10 , and 1.2 × 10 S cm , respectively, with superprotonic conductivity. Doping into the Nafion matrix prepared composite membranes for testing the performance of fuel cells. At 80 °C and 98% RH, the proton conductivity of reached a maximum value of 1.14 × 10 S cm , which is 2.8 times higher than recast Nafion. The results showed that charge-assisted HOFs with high proton channel density have better proton transport properties, providing a reference for the design of highly proton-conducting materials. Grasping proton transport pathways and mechanisms is vital for the application of fuel cell technology. Herein, we screened four guanidinium organosulfonate charge-assisted hydrogen-bonded organic frameworks (HOFs), namely, GBBS , G 3 TSPHB , G 4 TSP , and G 6 HSPB , which possess high hydrogen-bonded density proton transport networks shaped like nanotubes. These materials were prepared by self-assembly through charge-assisted interactions between guanidinium cations and organosulfonate anions, as well as by host–guest regulation. At 80 °C and 93% RH, the proton conductivity of GBBS , G 3 TSPHB , G 4 TSP , and G 6 HSPB can reach 4.56 × 10 –2 , 2.55 × 10 –2 , 4.01 × 10 –2 , and 1.2 × 10 –1 S cm –1 , respectively, with superprotonic conductivity. Doping G 6 HSPB into the Nafion matrix prepared composite membranes for testing the performance of fuel cells. At 80 °C and 98% RH, the proton conductivity of 9%-G 6 HSPB@Nafion reached a maximum value of 1.14 × 10 –1 S cm –1 , which is 2.8 times higher than recast Nafion. The results showed that charge-assisted HOFs with high proton channel density have better proton transport properties, providing a reference for the design of highly proton-conducting materials. |
| Author | Bai, Xiang-Tian Cao, Li-Hui Chen, Xu-Yong Cao, Xiao-Jie Gao, Yi-Da Yang, Dan |
| AuthorAffiliation | Shaanxi Key Laboratory of Chemical Additives for Industry, College of Chemistry and Chemical Engineering |
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| Author_xml | – sequence: 1 givenname: Xu-Yong surname: Chen fullname: Chen, Xu-Yong – sequence: 2 givenname: Li-Hui orcidid: 0000-0002-3676-0242 surname: Cao fullname: Cao, Li-Hui email: caolihui@sust.edu.cn – sequence: 3 givenname: Xiang-Tian surname: Bai fullname: Bai, Xiang-Tian – sequence: 4 givenname: Xiao-Jie surname: Cao fullname: Cao, Xiao-Jie – sequence: 5 givenname: Dan surname: Yang fullname: Yang, Dan – sequence: 6 givenname: Yi-Da surname: Gao fullname: Gao, Yi-Da |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/39473576$$D View this record in MEDLINE/PubMed |
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| Keywords | proton conduction charge-assisted proton exchange membrane hydrogen-bonded organic frameworks nanotubular |
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| Snippet | Grasping proton transport pathways and mechanisms is vital for the application of fuel cell technology. Herein, we screened four guanidinium organosulfonate... Grasping proton transport pathways and mechanisms is vital for the application of fuel cell technology. Herein, we screened four guanidinium organosulfonate... |
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| Title | Superprotonic Conductivity of Guanidinium Organosulfonate Hydrogen-Bonded Organic Frameworks with Nanotube-Shaped Proton Transport Channels |
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