Recent Progress in Electrocatalytic Conversion of Lignin: From Monomers, Dimers, to Raw Lignin

Lignin, as the second largest renewable biomass resource in nature, has increasingly received significant interest for its potential to be transformed into valuable chemicals, potentially contributing to carbon neutrality. Among different approaches, renewable electricity-driven biomass conversion h...

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Published inPrecision Chemistry Vol. 2; no. 9; pp. 428 - 446
Main Authors Liu, Xiang, Wang, Ye, Duan, Haohong
Format Journal Article
LanguageEnglish
Published United States University of Science and Technology of China and American Chemical Society 23.09.2024
American Chemical Society
Subjects
Review
Lignin
Electrocatalytic oxidation
Electrocatalyst design
Electrocatalytic reduction
Selectivity regulation
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Abstract Lignin, as the second largest renewable biomass resource in nature, has increasingly received significant interest for its potential to be transformed into valuable chemicals, potentially contributing to carbon neutrality. Among different approaches, renewable electricity-driven biomass conversion holds great promise to substitute a petroleum resource-driven one, owing to its characteristics of environmental friendliness, high energy efficiency, and tunable reactivity. The challenges lie on the polymeric structure and complex functional groups in lignin, requiring the development of efficient electrocatalysts for lignin valorization with enhanced activity and selectivity toward targeted chemicals. In this Review, we focus on the advancement of electrocatalytic valorization of lignin, from monomers, to dimers and to raw lignin, toward various value-added chemicals, with emphasis on catalyst design, reaction innovation, and mechanistic study. The general strategies for catalyst design are also summarized, offering insights into enhancing the activity and selectivity. Finally, challenges and perspectives for the electrocatalytic conversion of lignin are proposed.
AbstractList Lignin, as the second largest renewable biomass resource in nature, has increasingly received significant interest for its potential to be transformed into valuable chemicals, potentially contributing to carbon neutrality. Among different approaches, renewable electricity-driven biomass conversion holds great promise to substitute a petroleum resource-driven one, owing to its characteristics of environmental friendliness, high energy efficiency, and tunable reactivity. The challenges lie on the polymeric structure and complex functional groups in lignin, requiring the development of efficient electrocatalysts for lignin valorization with enhanced activity and selectivity toward targeted chemicals. In this Review, we focus on the advancement of electrocatalytic valorization of lignin, from monomers, to dimers and to raw lignin, toward various value-added chemicals, with emphasis on catalyst design, reaction innovation, and mechanistic study. The general strategies for catalyst design are also summarized, offering insights into enhancing the activity and selectivity. Finally, challenges and perspectives for the electrocatalytic conversion of lignin are proposed.Lignin, as the second largest renewable biomass resource in nature, has increasingly received significant interest for its potential to be transformed into valuable chemicals, potentially contributing to carbon neutrality. Among different approaches, renewable electricity-driven biomass conversion holds great promise to substitute a petroleum resource-driven one, owing to its characteristics of environmental friendliness, high energy efficiency, and tunable reactivity. The challenges lie on the polymeric structure and complex functional groups in lignin, requiring the development of efficient electrocatalysts for lignin valorization with enhanced activity and selectivity toward targeted chemicals. In this Review, we focus on the advancement of electrocatalytic valorization of lignin, from monomers, to dimers and to raw lignin, toward various value-added chemicals, with emphasis on catalyst design, reaction innovation, and mechanistic study. The general strategies for catalyst design are also summarized, offering insights into enhancing the activity and selectivity. Finally, challenges and perspectives for the electrocatalytic conversion of lignin are proposed.
Lignin, as the second largest renewable biomass resource in nature, has increasingly received significant interest for its potential to be transformed into valuable chemicals, potentially contributing to carbon neutrality. Among different approaches, renewable electricity-driven biomass conversion holds great promise to substitute a petroleum resource-driven one, owing to its characteristics of environmental friendliness, high energy efficiency, and tunable reactivity. The challenges lie on the polymeric structure and complex functional groups in lignin, requiring the development of efficient electrocatalysts for lignin valorization with enhanced activity and selectivity toward targeted chemicals. In this Review, we focus on the advancement of electrocatalytic valorization of lignin, from monomers, to dimers and to raw lignin, toward various value-added chemicals, with emphasis on catalyst design, reaction innovation, and mechanistic study. The general strategies for catalyst design are also summarized, offering insights into enhancing the activity and selectivity. Finally, challenges and perspectives for the electrocatalytic conversion of lignin are proposed.
Lignin, as the second largest renewable biomass resource in nature, has increasingly received significant interest for its potential to be transformed into valuable chemicals, potentially contributing to carbon neutrality. Among different approaches, renewable electricity-driven biomass conversion holds great promise to substitute a petroleum resource-driven one, owing to its characteristics of environmental friendliness, high energy efficiency, and tunable reactivity. The challenges lie on the polymeric structure and complex functional groups in lignin, requiring the development of efficient electrocatalysts for lignin valorization with enhanced activity and selectivity toward targeted chemicals. In this Review, we focus on the advancement of electrocatalytic valorization of lignin, from monomers, to dimers and to raw lignin, toward various value-added chemicals, with emphasis on catalyst design, reaction innovation, and mechanistic study. The general strategies for catalyst design are also summarized, offering insights into enhancing the activity and selectivity. Finally, challenges and perspectives for the electrocatalytic conversion of lignin are proposed.
Author Wang, Ye
Duan, Haohong
Liu, Xiang
AuthorAffiliation Department of Chemistry
Haihe Laboratory of Sustainable Chemical Transformations
Engineering Research Center of Advanced Rare Earth Materials, (Ministry of Education), Department of Chemistry
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Issue 9
Keywords Lignin
Electrocatalytic oxidation
Electrocatalyst design
Electrocatalytic reduction
Selectivity regulation
Language English
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Snippet Lignin, as the second largest renewable biomass resource in nature, has increasingly received significant interest for its potential to be transformed into...
Lignin, as the second largest renewable biomass resource in nature, has increasingly received significant interest for its potential to be transformed into...
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Title Recent Progress in Electrocatalytic Conversion of Lignin: From Monomers, Dimers, to Raw Lignin
URI http://dx.doi.org/10.1021/prechem.4c00024
https://www.ncbi.nlm.nih.gov/pubmed/39478938
https://www.proquest.com/docview/3122645545
https://pubmed.ncbi.nlm.nih.gov/PMC11524326
https://doaj.org/article/781d345ca4d943a0b5f26cf3ed347a9e
Volume 2
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