Solvation Structure Design for Aqueous Zn Metal Batteries
Aqueous Zn batteries are promising energy storage devices for large-scale energy-storage due to low cost and high energy density. However, their lifespan is limited by the water decomposition and Zn dendrite growth. Here, we suppress water reduction and Zn dendrite growth in dilute aqueous electroly...
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| Published in | Journal of the American Chemical Society Vol. 142; no. 51; pp. 21404 - 21409 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
23.12.2020
American Chemical Society (ACS) |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Aqueous Zn batteries are promising energy storage devices for large-scale energy-storage due to low cost and high energy density. However, their lifespan is limited by the water decomposition and Zn dendrite growth. Here, we suppress water reduction and Zn dendrite growth in dilute aqueous electrolyte by adding dimethyl sulfoxide (DMSO) into ZnCl2–H2O, in which DMSO replaces the H2O in Zn2+ solvation sheath due to a higher Gutmann donor number (29.8) of DMSO than that (18) of H2O. The preferential solvation of DMSO with Zn2+ and strong H2O–DMSO interaction inhibit the decomposition of solvated H2O. In addition, the decomposition of solvated DMSO forms Zn12(SO4)3Cl3(OH)15·5H2O, ZnSO3, and ZnS enriched-solid electrolyte interphase (SEI) preventing Zn dendrite and further suppressing water decomposition. The ZnCl2–H2O–DMSO electrolyte enables Zn anodes in Zn||Ti half-cell to achieve a high average Coulombic efficiency of 99.5% for 400 cycles (400 h), and the Zn||MnO2 full cell with a low capacity ratio of Zn:MnO2 at 2:1 to deliver a high energy density of 212 Wh/kg (based on both cathode and anode) and maitain 95.3% of the capacity over 500 cycles at 8 C. |
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| AbstractList | Aqueous Zn batteries are promising energy storage devices for large-scale energy-storage due to low cost and high energy density. However, their lifespan is limited by the water decomposition and Zn dendrite growth. Here, we suppress water reduction and Zn dendrite growth in dilute aqueous electrolyte by adding dimethyl sulfoxide (DMSO) into ZnCl
-H
O, in which DMSO replaces the H
O in Zn
solvation sheath due to a higher Gutmann donor number (29.8) of DMSO than that (18) of H
O. The preferential solvation of DMSO with Zn
and strong H
O-DMSO interaction inhibit the decomposition of solvated H
O. In addition, the decomposition of solvated DMSO forms Zn
(SO
)
Cl
(OH)
·5H
O, ZnSO
, and ZnS enriched-solid electrolyte interphase (SEI) preventing Zn dendrite and further suppressing water decomposition. The ZnCl
-H
O-DMSO electrolyte enables Zn anodes in Zn||Ti half-cell to achieve a high average Coulombic efficiency of 99.5% for 400 cycles (400 h), and the Zn||MnO
full cell with a low capacity ratio of Zn:MnO
at 2:1 to deliver a high energy density of 212 Wh/kg (based on both cathode and anode) and maitain 95.3% of the capacity over 500 cycles at 8 C. Aqueous Zn batteries are promising energy storage devices for large-scale energy-storage due to low cost and high energy density. However, their lifespan is limited by the water decomposition and Zn dendrite growth. Here, we suppress water reduction and Zn dendrite growth in dilute aqueous electrolyte by adding dimethyl sulfoxide (DMSO) into ZnCl2–H2O, in which DMSO replaces the H2O in Zn2+ solvation sheath due to a higher Gutmann donor number (29.8) of DMSO than that (18) of H2O. The preferential solvation of DMSO with Zn2+ and strong H2O–DMSO interaction inhibit the decomposition of solvated H2O. In addition, the decomposition of solvated DMSO forms Zn12(SO4)3Cl3(OH)15·5H2O, ZnSO3, and ZnS enriched-solid electrolyte interphase (SEI) preventing Zn dendrite and further suppressing water decomposition. The ZnCl2–H2O–DMSO electrolyte enables Zn anodes in Zn||Ti half-cell to achieve a high average Coulombic efficiency of 99.5% for 400 cycles (400 h), and the Zn||MnO2 full cell with a low capacity ratio of Zn:MnO2 at 2:1 to deliver a high energy density of 212 Wh/kg (based on both cathode and anode) and maitain 95.3% of the capacity over 500 cycles at 8 C. Aqueous Zn batteries are promising energy storage devices for large-scale energy-storage due to low cost and high energy density. However, their lifespan is limited by the water decomposition and Zn dendrite growth. Here, we suppress water reduction and Zn dendrite growth in dilute aqueous electrolyte by adding dimethyl sulfoxide (DMSO) into ZnCl2-H2O, in which DMSO replaces the H2O in Zn2+ solvation sheath due to a higher Gutmann donor number (29.8) of DMSO than that (18) of H2O. The preferential solvation of DMSO with Zn2+ and strong H2O-DMSO interaction inhibit the decomposition of solvated H2O. In addition, the decomposition of solvated DMSO forms Zn12(SO4)3Cl3(OH)15·5H2O, ZnSO3, and ZnS enriched-solid electrolyte interphase (SEI) preventing Zn dendrite and further suppressing water decomposition. The ZnCl2-H2O-DMSO electrolyte enables Zn anodes in Zn||Ti half-cell to achieve a high average Coulombic efficiency of 99.5% for 400 cycles (400 h), and the Zn||MnO2 full cell with a low capacity ratio of Zn:MnO2 at 2:1 to deliver a high energy density of 212 Wh/kg (based on both cathode and anode) and maitain 95.3% of the capacity over 500 cycles at 8 C.Aqueous Zn batteries are promising energy storage devices for large-scale energy-storage due to low cost and high energy density. However, their lifespan is limited by the water decomposition and Zn dendrite growth. Here, we suppress water reduction and Zn dendrite growth in dilute aqueous electrolyte by adding dimethyl sulfoxide (DMSO) into ZnCl2-H2O, in which DMSO replaces the H2O in Zn2+ solvation sheath due to a higher Gutmann donor number (29.8) of DMSO than that (18) of H2O. The preferential solvation of DMSO with Zn2+ and strong H2O-DMSO interaction inhibit the decomposition of solvated H2O. In addition, the decomposition of solvated DMSO forms Zn12(SO4)3Cl3(OH)15·5H2O, ZnSO3, and ZnS enriched-solid electrolyte interphase (SEI) preventing Zn dendrite and further suppressing water decomposition. The ZnCl2-H2O-DMSO electrolyte enables Zn anodes in Zn||Ti half-cell to achieve a high average Coulombic efficiency of 99.5% for 400 cycles (400 h), and the Zn||MnO2 full cell with a low capacity ratio of Zn:MnO2 at 2:1 to deliver a high energy density of 212 Wh/kg (based on both cathode and anode) and maitain 95.3% of the capacity over 500 cycles at 8 C. Aqueous Zn batteries are promising energy storage devices for large-scale energy-storage due to low cost and high energy density. However, their lifespan is limited by the water decomposition and Zn dendrite growth. In this study, we suppress water reduction and Zn dendrite growth in dilute aqueous electrolyte by adding dimethyl sulfoxide (DMSO) into ZnCl2–H2O, in which DMSO replaces the H2O in Zn2+ solvation sheath due to a higher Gutmann donor number (29.8) of DMSO than that (18) of H2O. The preferential solvation of DMSO with Zn2+ and strong H2O–DMSO interaction inhibit the decomposition of solvated H2O. In addition, the decomposition of solvated DMSO forms Zn12(SO4)3Cl3(OH)15·5H2O, ZnSO3, and ZnS enriched-solid electrolyte interphase (SEI) preventing Zn dendrite and further suppressing water decomposition. The ZnCl2–H2O–DMSO electrolyte enables Zn anodes in Zn||Ti half-cell to achieve a high average Coulombic efficiency of 99.5% for 400 cycles (400 h), and the Zn||MnO2 full cell with a low capacity ratio of Zn:MnO2 at 2:1 to deliver a high energy density of 212 Wh/kg (based on both cathode and anode) and maitain 95.3% of the capacity over 500 cycles at 8 C. Aqueous Zn batteries are promising energy storage devices for large-scale energy-storage due to low cost and high energy density. However, their lifespan is limited by the water decomposition and Zn dendrite growth. Here, we suppress water reduction and Zn dendrite growth in dilute aqueous electrolyte by adding dimethyl sulfoxide (DMSO) into ZnCl₂–H₂O, in which DMSO replaces the H₂O in Zn²⁺ solvation sheath due to a higher Gutmann donor number (29.8) of DMSO than that (18) of H₂O. The preferential solvation of DMSO with Zn²⁺ and strong H₂O–DMSO interaction inhibit the decomposition of solvated H₂O. In addition, the decomposition of solvated DMSO forms Zn₁₂(SO₄)₃Cl₃(OH)₁₅·5H₂O, ZnSO₃, and ZnS enriched-solid electrolyte interphase (SEI) preventing Zn dendrite and further suppressing water decomposition. The ZnCl₂–H₂O–DMSO electrolyte enables Zn anodes in Zn||Ti half-cell to achieve a high average Coulombic efficiency of 99.5% for 400 cycles (400 h), and the Zn||MnO₂ full cell with a low capacity ratio of Zn:MnO₂ at 2:1 to deliver a high energy density of 212 Wh/kg (based on both cathode and anode) and maitain 95.3% of the capacity over 500 cycles at 8 C. |
| Author | Wang, Yi Wang, Chunsheng Li, Dan Deng, Tao Cao, Longsheng Yang, Xiao-Qing Ma, Lin Xu, Jijian Hu, Enyuan |
| AuthorAffiliation | Chemistry Division Department of Chemical and Biomolecular Engineering |
| AuthorAffiliation_xml | – name: Department of Chemical and Biomolecular Engineering – name: Chemistry Division |
| Author_xml | – sequence: 1 givenname: Longsheng surname: Cao fullname: Cao, Longsheng organization: Department of Chemical and Biomolecular Engineering – sequence: 2 givenname: Dan surname: Li fullname: Li, Dan organization: Department of Chemical and Biomolecular Engineering – sequence: 3 givenname: Enyuan orcidid: 0000-0002-1881-4534 surname: Hu fullname: Hu, Enyuan organization: Chemistry Division – sequence: 4 givenname: Jijian orcidid: 0000-0001-7727-0488 surname: Xu fullname: Xu, Jijian organization: Department of Chemical and Biomolecular Engineering – sequence: 5 givenname: Tao surname: Deng fullname: Deng, Tao organization: Department of Chemical and Biomolecular Engineering – sequence: 6 givenname: Lin orcidid: 0000-0003-1183-1347 surname: Ma fullname: Ma, Lin organization: Department of Chemical and Biomolecular Engineering – sequence: 7 givenname: Yi surname: Wang fullname: Wang, Yi organization: Department of Chemical and Biomolecular Engineering – sequence: 8 givenname: Xiao-Qing orcidid: 0000-0002-3625-3478 surname: Yang fullname: Yang, Xiao-Qing organization: Chemistry Division – sequence: 9 givenname: Chunsheng orcidid: 0000-0002-8626-6381 surname: Wang fullname: Wang, Chunsheng email: cswang@umd.edu organization: Department of Chemical and Biomolecular Engineering |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/33290658$$D View this record in MEDLINE/PubMed https://www.osti.gov/servlets/purl/1737441$$D View this record in Osti.gov |
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| Snippet | Aqueous Zn batteries are promising energy storage devices for large-scale energy-storage due to low cost and high energy density. However, their lifespan is... |
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| SubjectTerms | anodes cathodes dimethyl sulfoxide Electrochemical cells Electrodes Electrolytes energy energy density ENERGY STORAGE longevity Solvation Surface chemistry |
| Title | Solvation Structure Design for Aqueous Zn Metal Batteries |
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