Seasonal variation of biogenic VOC emissions above a mixed hardwood forest in northern Michigan

Fluxes of biogenic volatile organic compounds (VOCs) were measured at a hardwood forest in northern Michigan (UMBS, Prophet research site) over the course of the growing and senescing season. Methanol, acetaldehyde, acetone and isoprene were found to be the most abundant biogenic VOCs with maximum f...

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Published inGeophysical research letters Vol. 30; no. 23; pp. 2186 - n/a
Main Authors Karl, T., Guenther, A., Spirig, C., Hansel, A., Fall, R.
Format Journal Article
LanguageEnglish
Published American Geophysical Union 01.12.2003
Blackwell Publishing Ltd
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Abstract Fluxes of biogenic volatile organic compounds (VOCs) were measured at a hardwood forest in northern Michigan (UMBS, Prophet research site) over the course of the growing and senescing season. Methanol, acetaldehyde, acetone and isoprene were found to be the most abundant biogenic VOCs with maximum fluxes (mixing ratios in ppbv) of 2.0 mg m−2 h−1 (21.0), 1.0 mg m−2 h−1 (2.7), 1.6 mg m−2 h−1 (5.6) and 7.6 mg m−2 h−1 (6), respectively. The emission patterns show distinct seasonal changes and indicate a spring peak for methanol due to rapid leaf expansion and a fall peak for acetone and acetaldehyde most likely attributed to senescing and decaying biomass; isoprene emissions peaked as expected in the summer. We estimate potential source strengths of 8.9 Tg (C) y−1 methanol, 2.7 Tg (C) y−1 acetaldehyde and 7.0 Tg (C) y−1 acetone for deciduous temperate forests, which is a substantial contribution to the global atmospheric VOC budget.
AbstractList Fluxes of biogenic volatile organic compounds (VOCs) were measured at a hardwood forest in northern Michigan (UMBS, Prophet research site) over the course of the growing and senescing season. Methanol, acetaldehyde, acetone and isoprene were found to be the most abundant biogenic VOCs with maximum fluxes (mixing ratios in ppbv) of 2.0 mg m super(-2) h super(-1) (21.0), 1.0 mg m super(-2) h super(-1) (2.7), 1.6 mg m super(-2) h super(-1) (5.6) and 7.6 mg m super(-2) h super(-1) (6), respectively. The emission patterns show distinct seasonal changes and indicate a spring peak for methanol due to rapid leaf expansion and a fall peak for acetone and acetaldehyde most likely attributed to senescing and decaying biomass; isoprene emissions peaked as expected in the summer. We estimate potential source strengths of 8.9 Tg (C) y super(-1) methanol, 2.7 Tg (C) y super(-1) acetaldehyde and 7.0 Tg (C) y super(-1) acetone for deciduous temperate forests, which is a substantial contribution to the global atmospheric VOC budget.
Fluxes of biogenic volatile organic compounds (VOCs) were measured at a hardwood forest in northern Michigan (UMBS, Prophet research site) over the course of the growing and senescing season. Methanol, acetaldehyde, acetone and isoprene were found to be the most abundant biogenic VOCs with maximum fluxes (mixing ratios in ppbv) of 2.0 mg/sq m/h (21.0), 1.0 mg/sq m/h (2.7), 1.6 mg/sq m/h (5.6) and 7.6 mg/sq m/h (6), respectively. The emission patterns show distinct seasonal changes and indicate a spring peak for methanol due to rapid leaf expansion and a fall peak for acetone and acetaldehyde most likely attributed to senescing and decaying biomass; isoprene emissions peaked as expected in the summer. We estimate potential source strengths of 8.9 Tg (C)/y methanol, 2.7 Tg (C)/y acetaldehyde and 7.0 Tg (C)/y acetone for deciduous temperate forests, which is a substantial contribution to the global atmospheric VOC budget.
Fluxes of biogenic volatile organic compounds (VOCs) were measured at a hardwood forest in northern Michigan (UMBS, Prophet research site) over the course of the growing and senescing season. Methanol, acetaldehyde, acetone and isoprene were found to be the most abundant biogenic VOCs with maximum fluxes (mixing ratios in ppbv) of 2.0 mg m −2 h −1 (21.0), 1.0 mg m −2 h −1 (2.7), 1.6 mg m −2 h −1 (5.6) and 7.6 mg m −2 h −1 (6), respectively. The emission patterns show distinct seasonal changes and indicate a spring peak for methanol due to rapid leaf expansion and a fall peak for acetone and acetaldehyde most likely attributed to senescing and decaying biomass; isoprene emissions peaked as expected in the summer. We estimate potential source strengths of 8.9 Tg (C) y −1 methanol, 2.7 Tg (C) y −1 acetaldehyde and 7.0 Tg (C) y −1 acetone for deciduous temperate forests, which is a substantial contribution to the global atmospheric VOC budget.
Fluxes of biogenic volatile organic compounds (VOCs) were measured at a hardwood forest in northern Michigan (UMBS, Prophet research site) over the course of the growing and senescing season. Methanol, acetaldehyde, acetone and isoprene were found to be the most abundant biogenic VOCs with maximum fluxes (mixing ratios in ppbv) of 2.0 mg m−2 h−1 (21.0), 1.0 mg m−2 h−1 (2.7), 1.6 mg m−2 h−1 (5.6) and 7.6 mg m−2 h−1 (6), respectively. The emission patterns show distinct seasonal changes and indicate a spring peak for methanol due to rapid leaf expansion and a fall peak for acetone and acetaldehyde most likely attributed to senescing and decaying biomass; isoprene emissions peaked as expected in the summer. We estimate potential source strengths of 8.9 Tg (C) y−1 methanol, 2.7 Tg (C) y−1 acetaldehyde and 7.0 Tg (C) y−1 acetone for deciduous temperate forests, which is a substantial contribution to the global atmospheric VOC budget.
Author Guenther, A.
Fall, R.
Hansel, A.
Karl, T.
Spirig, C.
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  surname: Fall
  fullname: Fall, R.
  organization: CIRES, University of Colorado, Colorado, Boulder, USA
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Snippet Fluxes of biogenic volatile organic compounds (VOCs) were measured at a hardwood forest in northern Michigan (UMBS, Prophet research site) over the course of...
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SubjectTerms Atmospheric Composition and Structure
Biosphere/atmosphere interactions
Constituent sources and sinks
Troposphere—composition and chemistry
Title Seasonal variation of biogenic VOC emissions above a mixed hardwood forest in northern Michigan
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https://onlinelibrary.wiley.com/doi/abs/10.1029%2F2003GL018432
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