Origin of low-chloride fluid in sediments from the eastern continental margin of India, results from the National Gas Hydrate Program Expedition 02
National Gas Hydrate Program Expedition 02 was conducted in 2015 by D/V Chikyu in the western Bay of Bengal, India. Analyses of interstitial water in sediment from four drilling sites along the eastern and western transect in the Krishna–Godavari Basin show that dissolved chloride (Cl−) concentratio...
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Published in | Marine and petroleum geology Vol. 108; no. C; pp. 377 - 388 |
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Main Authors | , , , , , , , |
Format | Journal Article |
Language | English |
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01.10.2019
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Abstract | National Gas Hydrate Program Expedition 02 was conducted in 2015 by D/V Chikyu in the western Bay of Bengal, India. Analyses of interstitial water in sediment from four drilling sites along the eastern and western transect in the Krishna–Godavari Basin show that dissolved chloride (Cl−) concentrations decreased with depth from seawater values (>550 mM) near the sediment surface to 300–400 mM at 350–400 m below seafloor (mbsf), suggesting the upward advection of low-Cl– fluid. Excursions of Cl− concentrations toward low values in gas hydrate zones were attributed to the presence of fresh water released by dissociation of gas hydrate during core recovery. At Sites in the western transect, Cl− concentrations below the gas hydrate reservoir (around 280 mbsf) were ca. 60 mM and ca. 45 mM lower than those from above the reservoir, and δ18O and δD values were 1–2‰ and 0.7–1.3‰ higher than those from above the reservoir, respectively. These results suggest that a fraction of migrating low-Cl– fluid is trapped in the gas hydrate zone, causing decreases of δ18O and δD in the residual water due to isotopic fractionation during gas hydrate formation. From mass-balance calculations, we estimated that 10–20% of the advected fluid is trapped at the gas hydrate zone. At all sites, the δ18O and δD values below the gas hydrate zone, representing relatively unaltered low-Cl– fluid, were 0.5–1‰ higher and ca. 13–15‰ lower than those of seawater, respectively. This trend is consistent with water derived from the dehydration of clay minerals, which generally occurs in deeply buried sediments. The contribution of clay mineral dehydration is relatively large at the western transect compared to that in the eastern transect. Our results imply that fluid advection contributes to the accumulation of gas hydrate in the study area.
•The decrease of Cl– concentration with depth is attributed to upward advection of low-Cl– fluid derived from clay mineral dehydration.•10–20% of migrating fluid is trapped in the thick gas hydrate zone.•The excursions in Cl– concentrations in the gas hydrate zone are attribute to the dissociation of gas hydrate during core recovery. |
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AbstractList | National Gas Hydrate Program Expedition 02 was conducted in 2015 by D/V Chikyu in the western Bay of Bengal, India. Analyses of interstitial water in sediment from four drilling sites along the eastern and western transect in the Krishna–Godavari Basin show that dissolved chloride (Cl−) concentrations decreased with depth from seawater values (>550 mM) near the sediment surface to 300–400 mM at 350–400 m below seafloor (mbsf), suggesting the upward advection of low-Cl– fluid. Excursions of Cl− concentrations toward low values in gas hydrate zones were attributed to the presence of fresh water released by dissociation of gas hydrate during core recovery. At Sites in the western transect, Cl− concentrations below the gas hydrate reservoir (around 280 mbsf) were ca. 60 mM and ca. 45 mM lower than those from above the reservoir, and δ18O and δD values were 1–2‰ and 0.7–1.3‰ higher than those from above the reservoir, respectively. These results suggest that a fraction of migrating low-Cl– fluid is trapped in the gas hydrate zone, causing decreases of δ18O and δD in the residual water due to isotopic fractionation during gas hydrate formation. From mass-balance calculations, we estimated that 10–20% of the advected fluid is trapped at the gas hydrate zone. At all sites, the δ18O and δD values below the gas hydrate zone, representing relatively unaltered low-Cl– fluid, were 0.5–1‰ higher and ca. 13–15‰ lower than those of seawater, respectively. This trend is consistent with water derived from the dehydration of clay minerals, which generally occurs in deeply buried sediments. The contribution of clay mineral dehydration is relatively large at the western transect compared to that in the eastern transect. Our results imply that fluid advection contributes to the accumulation of gas hydrate in the study area.
•The decrease of Cl– concentration with depth is attributed to upward advection of low-Cl– fluid derived from clay mineral dehydration.•10–20% of migrating fluid is trapped in the thick gas hydrate zone.•The excursions in Cl– concentrations in the gas hydrate zone are attribute to the dissociation of gas hydrate during core recovery. |
Author | Kinoshita, Masataka Suga, Hisami Jiménez-Espejo, Francisco Jose Komai, Nobuharu Ijiri, Akira Haraguchi, Satoru Inagaki, Fumio Yamada, Yasuhiro |
Author_xml | – sequence: 1 givenname: Akira orcidid: 0000-0001-7140-1491 surname: Ijiri fullname: Ijiri, Akira email: ijiri@jamstec.go.jp organization: Kochi Institute for Core Sample Research, Japan Agency for Marine-Earth Science and Technology (JAMSTEC), 200 Monobe Otsu, Nankoku 783-8502, Japan – sequence: 2 givenname: Satoru surname: Haraguchi fullname: Haraguchi, Satoru organization: Department of Solid Earth Geochemistry, JAMSTEC, Natsushima-cho 2-15, Yokosuka 237-0061, Japan – sequence: 3 givenname: Francisco Jose orcidid: 0000-0002-0335-8580 surname: Jiménez-Espejo fullname: Jiménez-Espejo, Francisco Jose organization: Department of Biogeochemistry, JAMSTEC, Natsushima-cho 2-15, Yokosuka 237-0061, Japan – sequence: 4 givenname: Nobuharu surname: Komai fullname: Komai, Nobuharu organization: Marine Works Japan Ltd., 3-54-1 Oppamahigashi, Yokosuka 237-0063, Japan – sequence: 5 givenname: Hisami surname: Suga fullname: Suga, Hisami organization: Department of Biogeochemistry, JAMSTEC, Natsushima-cho 2-15, Yokosuka 237-0061, Japan – sequence: 6 givenname: Masataka orcidid: 0000-0003-1144-3651 surname: Kinoshita fullname: Kinoshita, Masataka organization: Earthquake Research Institute, The University of Tokyo, 1-1-1 Yayoi, Bunkyo-ku, Tokyo 113-0032, Japan – sequence: 7 givenname: Fumio surname: Inagaki fullname: Inagaki, Fumio organization: Kochi Institute for Core Sample Research, Japan Agency for Marine-Earth Science and Technology (JAMSTEC), 200 Monobe Otsu, Nankoku 783-8502, Japan – sequence: 8 givenname: Yasuhiro surname: Yamada fullname: Yamada, Yasuhiro organization: R & D Center for Ocean Drilling Science, JAMSTEC, 3173-25 Showa-machi, Yokohama 236-0001, Japan |
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CitedBy_id | crossref_primary_10_1016_j_marpetgeo_2019_03_032 crossref_primary_10_1016_j_marpetgeo_2018_07_026 crossref_primary_10_1016_j_marpetgeo_2018_12_049 crossref_primary_10_1016_j_marpetgeo_2023_106370 crossref_primary_10_1016_j_marpetgeo_2019_05_023 crossref_primary_10_1016_j_marpetgeo_2018_11_014 crossref_primary_10_1016_j_marpetgeo_2018_11_047 crossref_primary_10_1016_j_marpetgeo_2020_104856 crossref_primary_10_1190_INT_2019_0026_1 |
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Keywords | Oxygen and hydrogen isotopic compositions Gas hydrate Chloride concentration Clay mineral dehydration Fluid advection |
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SubjectTerms | Chloride concentration Clay mineral dehydration Fluid advection Gas hydrate Oxygen and hydrogen isotopic compositions |
Title | Origin of low-chloride fluid in sediments from the eastern continental margin of India, results from the National Gas Hydrate Program Expedition 02 |
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