Effect of Electrolyte Concentration on the Viscosity and Voltammetry of Supercritical Solutions
The viscosity of a supercritical electrolyte solution is measured for the first time using a modified quartz crystal microbalance, and it is shown that ionic solvation leads to a significant structuring of the solvent and an appreciable increase in solution viscosity. Voltammetric investigations in...
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| Published in | Analytical chemistry (Washington) Vol. 77; no. 20; pp. 6702 - 6708 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Washington, DC
American Chemical Society
15.10.2005
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The viscosity of a supercritical electrolyte solution is measured for the first time using a modified quartz crystal microbalance, and it is shown that ionic solvation leads to a significant structuring of the solvent and an appreciable increase in solution viscosity. Voltammetric investigations in the electrolyte solutions are used to confirm the magnitude of the viscosity changes, and these account for the appreciably lower than expected peak currents. |
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| AbstractList | The viscosity of a supercritical electrolyte solution is measured for the first time using a modified quartz crystal microbalance, and it is shown that ionic solvation leads to a significant structuring of the solvent and an appreciable increase in solution viscosity. Voltammetric investigations in the electrolyte solutions are used to confirm the magnitude of the viscosity changes, and these account for the appreciably lower than expected peak currents. The viscosity of a supercritical electrolyte solution is measured for the first time using a modified quartz crystal microbalance, and it is shown that ionic solvation leads to a significant structuring of the solvent and an appreciable increase in solution viscosity. Voltammetric investigations in the electrolyte solutions are used to confirm the magnitude of the viscosity changes, and these account for the appreciably lower than expected peak currents.[PUBLICATION ABSTRACT] |
| Author | Hope, Eric G Palmer, Donna J Abbott, Andrew P |
| Author_xml | – sequence: 1 givenname: Andrew P surname: Abbott fullname: Abbott, Andrew P – sequence: 2 givenname: Eric G surname: Hope fullname: Hope, Eric G – sequence: 3 givenname: Donna J surname: Palmer fullname: Palmer, Donna J |
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| CitedBy_id | crossref_primary_10_1021_jp066620p crossref_primary_10_1016_j_colsurfa_2021_126688 crossref_primary_10_1039_C1CP22555C crossref_primary_10_1039_B918981E crossref_primary_10_1039_C0CP01202E crossref_primary_10_1016_j_jphotochem_2017_12_014 crossref_primary_10_1039_C6CP00466K crossref_primary_10_1098_rsta_2015_0007 crossref_primary_10_1016_j_elecom_2014_04_008 crossref_primary_10_1039_C4CP04545A crossref_primary_10_1039_c3cp54955k crossref_primary_10_1016_j_jelechem_2009_01_027 crossref_primary_10_1016_j_supflu_2015_03_007 crossref_primary_10_1002_elan_201500515 crossref_primary_10_1039_c004227g |
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| Keywords | Viscosity Solvation Electrolyte solution Concentration effect Lead Voltammetry Quartz microbalance |
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| Snippet | The viscosity of a supercritical electrolyte solution is measured for the first time using a modified quartz crystal microbalance, and it is shown that ionic... |
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| SubjectTerms | Analytical chemistry Borates - chemistry Calibration Chemistry Crystal structure Electrochemical methods Electrochemistry Electrodes Electrolytes - chemistry Exact sciences and technology Ferrous Compounds - chemistry General, instrumentation Hydrocarbons, Fluorinated - chemistry Ions Metallocenes Quartz - chemistry Quaternary Ammonium Compounds - chemistry Solutions - chemistry Viscosity |
| Title | Effect of Electrolyte Concentration on the Viscosity and Voltammetry of Supercritical Solutions |
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