Design and Mechanisms of Asymmetric Supercapacitors

Ongoing technological advances in diverse fields including portable electronics, transportation, and green energy are often hindered by the insufficient capability of energy-storage devices. By taking advantage of two different electrode materials, asymmetric supercapacitors can extend their operati...

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Published in	Chemical reviews Vol. 118; no. 18; pp. 9233 - 9280
Main Authors	Shao, Yuanlong, El-Kady, Maher F, Sun, Jingyu, Li, Yaogang, Zhang, Qinghong, Zhu, Meifang, Wang, Hongzhi, Dunn, Bruce, Kaner, Richard B
Format	Journal Article
Language	English
Published	United States American Chemical Society 26.09.2018
Subjects	Asymmetry Clean energy Component parts Design Electric potential Electrochemical analysis Electrochemistry Electrode materials Electrodes Electrolytes electronics Energy storage Fabrication Green energy Performance evaluation renewable energy sources Supercapacitors Thermodynamics transportation
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Abstract	Ongoing technological advances in diverse fields including portable electronics, transportation, and green energy are often hindered by the insufficient capability of energy-storage devices. By taking advantage of two different electrode materials, asymmetric supercapacitors can extend their operating voltage window beyond the thermodynamic decomposition voltage of electrolytes while enabling a solution to the energy storage limitations of symmetric supercapacitors. This review provides comprehensive knowledge to this field. We first look at the essential energy-storage mechanisms and performance evaluation criteria for asymmetric supercapacitors to understand the wide-ranging research conducted in this area. Then we move to the recent progress made for the design and fabrication of electrode materials and the overall structure of asymmetric supercapacitors in different categories. We also highlight several key scientific challenges and present our perspectives on enhancing the electrochemical performance of future asymmetric supercapacitors.
AbstractList	Ongoing technological advances in diverse fields including portable electronics, transportation, and green energy are often hindered by the insufficient capability of energy-storage devices. By taking advantage of two different electrode materials, asymmetric supercapacitors can extend their operating voltage window beyond the thermodynamic decomposition voltage of electrolytes while enabling a solution to the energy storage limitations of symmetric supercapacitors. This review provides comprehensive knowledge to this field. We first look at the essential energy-storage mechanisms and performance evaluation criteria for asymmetric supercapacitors to understand the wide-ranging research conducted in this area. Then we move to the recent progress made for the design and fabrication of electrode materials and the overall structure of asymmetric supercapacitors in different categories. We also highlight several key scientific challenges and present our perspectives on enhancing the electrochemical performance of future asymmetric supercapacitors. Ongoing technological advances in diverse fields including portable electronics, transportation, and green energy are often hindered by the insufficient capability of energy-storage devices. By taking advantage of two different electrode materials, asymmetric supercapacitors can extend their operating voltage window beyond the thermodynamic decomposition voltage of electrolytes while enabling a solution to the energy storage limitations of symmetric supercapacitors. This review provides comprehensive knowledge to this field. We first look at the essential energy-storage mechanisms and performance evaluation criteria for asymmetric supercapacitors to understand the wide-ranging research conducted in this area. Then we move to the recent progress made for the design and fabrication of electrode materials and the overall structure of asymmetric supercapacitors in different categories. We also highlight several key scientific challenges and present our perspectives on enhancing the electrochemical performance of future asymmetric supercapacitors.Ongoing technological advances in diverse fields including portable electronics, transportation, and green energy are often hindered by the insufficient capability of energy-storage devices. By taking advantage of two different electrode materials, asymmetric supercapacitors can extend their operating voltage window beyond the thermodynamic decomposition voltage of electrolytes while enabling a solution to the energy storage limitations of symmetric supercapacitors. This review provides comprehensive knowledge to this field. We first look at the essential energy-storage mechanisms and performance evaluation criteria for asymmetric supercapacitors to understand the wide-ranging research conducted in this area. Then we move to the recent progress made for the design and fabrication of electrode materials and the overall structure of asymmetric supercapacitors in different categories. We also highlight several key scientific challenges and present our perspectives on enhancing the electrochemical performance of future asymmetric supercapacitors.
Author	Li, Yaogang El-Kady, Maher F Zhang, Qinghong Kaner, Richard B Zhu, Meifang Dunn, Bruce Shao, Yuanlong Wang, Hongzhi Sun, Jingyu
AuthorAffiliation	Engineering Research Center of Advanced Glasses Manufacturing Technology, Ministry of Education California NanoSystems Institute, UCLA Soochow University Donghua University Department of Chemistry and Biochemistry Cambridge Graphene Center, Department of Engineering College of Energy, Soochow Institute for Energy and Materials InnovationS (SIEMIS) State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Material Science and Engineering Department of Materials Science and Engineering University of Cambridge
AuthorAffiliation_xml	– name: College of Energy, Soochow Institute for Energy and Materials InnovationS (SIEMIS) – name: Soochow University – name: State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Material Science and Engineering – name: Engineering Research Center of Advanced Glasses Manufacturing Technology, Ministry of Education – name: California NanoSystems Institute, UCLA – name: Donghua University – name: University of Cambridge – name: Department of Chemistry and Biochemistry – name: Department of Materials Science and Engineering – name: Cambridge Graphene Center, Department of Engineering
Author_xml	– sequence: 1 givenname: Yuanlong orcidid: 0000-0002-4950-9911 surname: Shao fullname: Shao, Yuanlong email: yuanlong.shao@gmail.com organization: University of Cambridge – sequence: 2 givenname: Maher F surname: El-Kady fullname: El-Kady, Maher F – sequence: 3 givenname: Jingyu orcidid: 0000-0002-9812-3046 surname: Sun fullname: Sun, Jingyu organization: Soochow University – sequence: 4 givenname: Yaogang surname: Li fullname: Li, Yaogang organization: Donghua University – sequence: 5 givenname: Qinghong surname: Zhang fullname: Zhang, Qinghong organization: State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Material Science and Engineering – sequence: 6 givenname: Meifang surname: Zhu fullname: Zhu, Meifang organization: State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Material Science and Engineering – sequence: 7 givenname: Hongzhi orcidid: 0000-0002-5469-2327 surname: Wang fullname: Wang, Hongzhi email: wanghz@dhu.edu.cn organization: State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Material Science and Engineering – sequence: 8 givenname: Bruce orcidid: 0000-0001-5669-4740 surname: Dunn fullname: Dunn, Bruce email: bdunn@ucla.edu organization: California NanoSystems Institute, UCLA – sequence: 9 givenname: Richard B orcidid: 0000-0003-0345-4924 surname: Kaner fullname: Kaner, Richard B email: kaner@chem.ucla.edu organization: California NanoSystems Institute, UCLA
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/30204424$$D View this record in MEDLINE/PubMed
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Snippet	Ongoing technological advances in diverse fields including portable electronics, transportation, and green energy are often hindered by the insufficient...
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SubjectTerms	Asymmetry Clean energy Component parts Design Electric potential Electrochemical analysis Electrochemistry Electrode materials Electrodes Electrolytes electronics Energy storage Fabrication Green energy Performance evaluation renewable energy sources Supercapacitors Thermodynamics transportation
Title	Design and Mechanisms of Asymmetric Supercapacitors
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