Comparison of nickel and vanadyl porphyrin distributions of sediments
The distributions of nickel and vanadyl porphyrins of Toarcian shale, northern Germany, and the Monterey Formation, California, were examined. The compositions of nickel and vanadyl porphyrin fractions of extracts from the same sample show substantial differences. The nickel porphyrin distribution i...
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| Published in | Geochimica et cosmochimica acta Vol. 57; no. 6; pp. 1367 - 1377 |
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| Main Authors | , |
| Format | Journal Article |
| Language | English |
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United States
Elsevier Ltd
01.03.1993
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| Abstract | The distributions of nickel and vanadyl porphyrins of Toarcian shale, northern Germany, and the Monterey Formation, California, were examined. The compositions of nickel and vanadyl porphyrin fractions of extracts from the same sample show substantial differences. The nickel porphyrin distribution is more complex than the vanadyl porphyrin distribution. While the vanadyl porphyrin distributions of samples from a core are the same, their nickel porphyrin compositions show wide variations. The nickel porphyrins are enriched in “etio” and 3-nor C
30DPEP structures. The vanadyl porphyrins are enriched in the C
33DiDPEP structure. Methylpropano porphyrins are found only in the vanadyl porphyrin fraction, whereas the cycloheptano structural type is predominant in the nickel fraction. C
31DPEP and C
32DPEP are found both in the nickel and vanadyl fractions. Their relative abundance in the two fractions is proportional to the
Ni
VO
porphyrin ratio. The observed differences in the compositions of nickel and vanadyl porphyrin fractions are due to differences in the rate constants for their formation from the pheopigments. |
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| AbstractList | The distributions of nickel and vanadyl porphyrins of Toarcian shale, northern Germany, and the Monterey Formation, California, were examined. The compositions of nickel and vanadyl porphyrin fractions of extracts from the same sample show substantial differences. The nickel porphyrin distribution is more complex than the vanadyl porphyrin distribution. While the vanadyl porphyrin distributions of samples from a core are the same, their nickel porphyrin compositions show wide variations. The nickel porphyrins are enriched in [open quotes]etio[close quotes] and 3-nor C[sub 30]DPEP structures. The vanadyl porphyrins are enriched in the C[sub 33]DiDPEP structure. Methylpropano porphyrins are found only in the vanadyl porphyrin fraction, whereas the cycloheptano structural type is predominant in the nickel fraction. C[sub 31]DPEP and C[sub 32]DPEP are found both in the nickel and vanadyl fractions. Their relative abundance in the two fractions is proportional to the Ni/VO porphyrin ratio. The observed differences in the compositions of nickel and vanadyl porphyrin fractions are due to differences in the rate constants for their formation from the pheopigments. 25 refs., 9 figs. The distributions of nickel and vanadyl porphyrins of Toarcian shale, northern Germany, and the Monterey Formation, California, were examined. The compositions of nickel and vanadyl porphyrin fractions of extracts from the same sample show substantial differences. The nickel porphyrin distribution is more complex than the vanadyl porphyrin distribution. While the vanadyl porphyrin distributions of samples from a core are the same, their nickel porphyrin compositions show wide variations. The nickel porphyrins are enriched in “etio” and 3-nor C 30DPEP structures. The vanadyl porphyrins are enriched in the C 33DiDPEP structure. Methylpropano porphyrins are found only in the vanadyl porphyrin fraction, whereas the cycloheptano structural type is predominant in the nickel fraction. C 31DPEP and C 32DPEP are found both in the nickel and vanadyl fractions. Their relative abundance in the two fractions is proportional to the Ni VO porphyrin ratio. The observed differences in the compositions of nickel and vanadyl porphyrin fractions are due to differences in the rate constants for their formation from the pheopigments. |
| Author | Boreham, Christopher J. Sundararaman, Padmanabhan |
| Author_xml | – sequence: 1 givenname: Padmanabhan surname: Sundararaman fullname: Sundararaman, Padmanabhan organization: Chevron Oil Field Research Company, PO Box 446, La Habra, CA 90631, USA – sequence: 2 givenname: Christopher J. surname: Boreham fullname: Boreham, Christopher J. organization: Bureau of Mineral Resources, Geology and Geophysics, GPO Box 378, Canberra, ACT 2601, Australia |
| BackLink | https://www.osti.gov/biblio/6342508$$D View this record in Osti.gov |
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| Cites_doi | 10.1016/S0040-4039(00)84480-9 10.1016/S0040-4039(00)85030-3 10.1016/0009-2541(82)90019-5 10.1016/0016-7037(88)90136-6 10.1016/S0040-4039(00)92250-0 10.1016/0016-7037(84)90219-9 10.1016/0146-6380(84)90038-X 10.1016/S0021-9673(01)93964-0 10.1021/ef00032a017 10.1016/0146-6380(90)90003-I 10.1021/ef00024a003 10.1016/S0040-4039(00)88754-7 10.1021/ac00289a007 10.1021/ef00024a001 10.1016/0016-7037(82)90377-5 10.1002/ange.19360493803 |
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| Snippet | The distributions of nickel and vanadyl porphyrins of Toarcian shale, northern Germany, and the Monterey Formation, California, were examined. The compositions... |
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| SubjectTerms | 400100 - Analytical & Separations Chemistry CALIFORNIA CARBOXYLIC ACIDS CHEMICAL ANALYSIS CHLOROPHYLL CHROMATOGRAPHY COMPLEXES DEVELOPED COUNTRIES DIAGENESIS DISTRIBUTION HETEROCYCLIC ACIDS HETEROCYCLIC COMPOUNDS INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY LIQUID COLUMN CHROMATOGRAPHY NICKEL COMPLEXES NORTH AMERICA ORGANIC ACIDS ORGANIC COMPOUNDS ORGANIC NITROGEN COMPOUNDS PHYTOCHROMES PIGMENTS PORPHYRINS PROTEINS QUANTITATIVE CHEMICAL ANALYSIS SEDIMENTS SEPARATION PROCESSES SPATIAL DISTRIBUTION TRANSITION ELEMENT COMPLEXES USA VANADIUM COMPLEXES |
| Title | Comparison of nickel and vanadyl porphyrin distributions of sediments |
| URI | https://dx.doi.org/10.1016/0016-7037(93)90078-B https://www.osti.gov/biblio/6342508 |
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