Shape-Dependent Oriented Trapping and Scaffolding of Plasmonic Nanoparticles by Topological Defects for Self-Assembly of Colloidal Dimers in Liquid Crystals

We demonstrate scaffolding of plasmonic nanoparticles by topological defects induced by colloidal microspheres to match their surface boundary conditions with a uniform far-field alignment in a liquid crystal host. Displacing energetically costly liquid crystal regions of reduced order, anisotropic...

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Published inNano letters Vol. 12; no. 2; pp. 955 - 963
Main Authors Senyuk, Bohdan, Evans, Julian S, Ackerman, Paul J, Lee, Taewoo, Manna, Pramit, Vigderman, Leonid, Zubarev, Eugene R, van de Lagemaat, Jao, Smalyukh, Ivan I
Format Journal Article
LanguageEnglish
Published Washington, DC American Chemical Society 08.02.2012
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Abstract We demonstrate scaffolding of plasmonic nanoparticles by topological defects induced by colloidal microspheres to match their surface boundary conditions with a uniform far-field alignment in a liquid crystal host. Displacing energetically costly liquid crystal regions of reduced order, anisotropic nanoparticles with concave or convex shapes not only stably localize in defects but also self-orient with respect to the microsphere surface. Using laser tweezers, we manipulate the ensuing nanoparticle-microsphere colloidal dimers, probing the strength of elastic binding and demonstrating self-assembly of hierarchical colloidal superstructures such as chains and arrays.
AbstractList We demonstrate scaffolding of plasmonic nanoparticles by topological defects induced by colloidal microspheres to match their surface boundary conditions with a uniform far-field alignment in a liquid crystal host. Displacing energetically costly liquid crystal regions of reduced order, anisotropic nanoparticles with concave or convex shapes not only stably localize in defects but also self-orient with respect to the microsphere surface. Using laser tweezers, we manipulate the ensuing nanoparticle-microsphere colloidal dimers, probing the strength of elastic binding and demonstrating self-assembly of hierarchical colloidal superstructures such as chains and arrays.
Author Evans, Julian S
Vigderman, Leonid
van de Lagemaat, Jao
Zubarev, Eugene R
Ackerman, Paul J
Senyuk, Bohdan
Manna, Pramit
Lee, Taewoo
Smalyukh, Ivan I
AuthorAffiliation University of Colorado at Boulder
National Renewable Energy Laboratory and University of Colorado at Boulder
National Renewable Energy Laboratory
Rice University
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  fullname: Ackerman, Paul J
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  surname: Smalyukh
  fullname: Smalyukh, Ivan I
  email: ivan.smalyukh@colorado.edu
  organization: National Renewable Energy Laboratory and University of Colorado at Boulder
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Issue 2
Keywords nanoscale self-assembly
liquid crystal elasticity
colloids
topological defects
optical trapping
Plasmonic nanoparticles
Gold
Topological defect
Uniform field
Boundary conditions
Nanoplasmonics
Liquid crystals
Nanoparticles
Microspheres
Optical trapping
Self-assembly
Anisotropy
Transition elements
Superstructure
Surface plasmon resonance
Arrays
Language English
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2012 American Chemical Society
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Snippet We demonstrate scaffolding of plasmonic nanoparticles by topological defects induced by colloidal microspheres to match their surface boundary conditions with...
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SubjectTerms Collective excitations (including excitons, polarons, plasmons and other charge-density excitations)
Colloids
Colloids - chemical synthesis
Colloids - chemistry
Condensed matter: electronic structure, electrical, magnetic, and optical properties
Crystal defects
Dimerization
Electronic structure and electrical properties of surfaces, interfaces, thin films and low-dimensional structures
Exact sciences and technology
Liquid crystals
Liquid Crystals - chemistry
Microspheres
Nanoparticles
Nanoparticles - chemistry
Nanostructure
Particle Size
Physics
Plasmonics
Scaffolding
Self assembly
Surface and interface electron states
Surface Plasmon Resonance
Surface Properties
Title Shape-Dependent Oriented Trapping and Scaffolding of Plasmonic Nanoparticles by Topological Defects for Self-Assembly of Colloidal Dimers in Liquid Crystals
URI http://dx.doi.org/10.1021/nl204030t
https://www.ncbi.nlm.nih.gov/pubmed/22233163
https://search.proquest.com/docview/1762052890
https://search.proquest.com/docview/920785978
Volume 12
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