Regionalization of soil base cation weathering for evaluating stream water acidification in the Appalachian Mountains, USA
Estimation of base cation supply from mineral weathering (BC w ) is useful for watershed research and management. Existing regional approaches for estimating BC w require generalized assumptions and availability of stream chemistry data. We developed an approach for estimating BC w using regionally...
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Published in | Environmental pollution (1987) Vol. 162; pp. 338 - 344 |
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Main Authors | , , |
Format | Journal Article |
Language | English |
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Elsevier Ltd
01.03.2012
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Abstract | Estimation of base cation supply from mineral weathering (BC
w
) is useful for watershed research and management. Existing regional approaches for estimating BC
w
require generalized assumptions and availability of stream chemistry data. We developed an approach for estimating BC
w
using regionally specific empirical relationships. The dynamic model MAGIC was used to calibrate BC
w
in 92 watersheds distributed across three ecoregions. Empirical relationships between MAGIC-simulated BC
w
and watershed characteristics were developed to provide the basis for regionalization of BC
w
throughout the entire study region. BC
w
estimates extracted from MAGIC calibrations compared reasonably well with BC
w
estimated by regression based on landscape characteristics. Approximately one-third of the study region was predicted to exhibit BC
w
rates less than 100 meq/m
2/yr. Estimates were especially low for some locations within national park and wilderness areas. The regional BC
w
results are discussed in the context of critical loads (CLs) of acidic deposition for aquatic ecosystem protection.
► Base cation weathering (BC
w
) estimates are needed to model critical load of acidity. ► Estimating BC
w
formerly required generalized assumptions and stream chemistry data. ► We describe a high-resolution approach for estimating BC
w
for regional application.
A new approach is described for deriving regional estimates of effective base cation weathering using empirical relationships with landscape characteristics. |
---|---|
AbstractList | Estimation of base cation supply from mineral weathering (BC(w)) is useful for watershed research and management. Existing regional approaches for estimating BC(w) require generalized assumptions and availability of stream chemistry data. We developed an approach for estimating BC(w) using regionally specific empirical relationships. The dynamic model MAGIC was used to calibrate BC(w) in 92 watersheds distributed across three ecoregions. Empirical relationships between MAGIC-simulated BC(w) and watershed characteristics were developed to provide the basis for regionalization of BC(w) throughout the entire study region. BC(w) estimates extracted from MAGIC calibrations compared reasonably well with BC(w) estimated by regression based on landscape characteristics. Approximately one-third of the study region was predicted to exhibit BC(w) rates less than 100 meq/m(2)/yr. Estimates were especially low for some locations within national park and wilderness areas. The regional BC(w) results are discussed in the context of critical loads (CLs) of acidic deposition for aquatic ecosystem protection. Estimation of base cation supply from mineral weathering (BC sub(w)) is useful for watershed research and management. Existing regional approaches for estimating BC sub(w) require generalized assumptions and availability of stream chemistry data. We developed an approach for estimating BC sub(w) using regionally specific empirical relationships. The dynamic model MAGIC was used to calibrate BC sub(w) in 92 watersheds distributed across three ecoregions. Empirical relationships between MAGIC-simulated BC sub(w) and watershed characteristics were developed to provide the basis for regionalization of BC sub(w) throughout the entire study region. BC sub(w) estimates extracted from MAGIC calibrations compared reasonably well with BC sub(w) estimated by regression based on landscape characteristics. Approximately one-third of the study region was predicted to exhibit BC sub(w) rates less than 100 meq/m super(2)/yr. Estimates were especially low for some locations within national park and wilderness areas. The regional BC sub(w) results are discussed in the context of critical loads (CLs) of acidic deposition for aquatic ecosystem protection. Estimation of base cation supply from mineral weathering (BCw) is useful for watershed research and management. Existing regional approaches for estimating BCw require generalized assumptions and availability of stream chemistry data. We developed an approach for estimating BCw using regionally specific empirical relationships. The dynamic model MAGIC was used to calibrate BCw in 92 watersheds distributed across three ecoregions. Empirical relationships between MAGIC-simulated BCw and watershed characteristics were developed to provide the basis for regionalization of BCw throughout the entire study region. BCw estimates extracted from MAGIC calibrations compared reasonably well with BCw estimated by regression based on landscape characteristics. Approximately one-third of the study region was predicted to exhibit BCw rates less than 100 meq/m²/yr. Estimates were especially low for some locations within national park and wilderness areas. The regional BCw results are discussed in the context of critical loads (CLs) of acidic deposition for aquatic ecosystem protection. Estimation of base cation supply from mineral weathering (BC w ) is useful for watershed research and management. Existing regional approaches for estimating BC w require generalized assumptions and availability of stream chemistry data. We developed an approach for estimating BC w using regionally specific empirical relationships. The dynamic model MAGIC was used to calibrate BC w in 92 watersheds distributed across three ecoregions. Empirical relationships between MAGIC-simulated BC w and watershed characteristics were developed to provide the basis for regionalization of BC w throughout the entire study region. BC w estimates extracted from MAGIC calibrations compared reasonably well with BC w estimated by regression based on landscape characteristics. Approximately one-third of the study region was predicted to exhibit BC w rates less than 100 meq/m 2/yr. Estimates were especially low for some locations within national park and wilderness areas. The regional BC w results are discussed in the context of critical loads (CLs) of acidic deposition for aquatic ecosystem protection. ► Base cation weathering (BC w ) estimates are needed to model critical load of acidity. ► Estimating BC w formerly required generalized assumptions and stream chemistry data. ► We describe a high-resolution approach for estimating BC w for regional application. A new approach is described for deriving regional estimates of effective base cation weathering using empirical relationships with landscape characteristics. |
Author | Cosby, B.J. Sullivan, T.J. McDonnell, T.C. |
Author_xml | – sequence: 1 givenname: T.C. surname: McDonnell fullname: McDonnell, T.C. email: todd.mcdonnell@esenvironmental.com organization: E&S Environmental Chemistry, Inc., P.O. Box 609, Corvallis, OR 97339, USA – sequence: 2 givenname: B.J. surname: Cosby fullname: Cosby, B.J. organization: Department of Environmental Science, University of Virginia, Charlottesville, VA 22903, USA – sequence: 3 givenname: T.J. surname: Sullivan fullname: Sullivan, T.J. organization: E&S Environmental Chemistry, Inc., P.O. Box 609, Corvallis, OR 97339, USA |
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Keywords | Weathering Acidification Critical load Base cation Acidic deposition Atmospheric fallout Geochemistry Environmental management Acid precipitation Hydrochemistry Watershed Surface water Stream Water pollution |
Language | English |
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References | Henriksen, Dillon, Aherne (bib13) 2002; 59 Jenkins, Whitehead, Musgrove, Cosby (bib17) 1990; 116 Sullivan, Cosby, Herlihy, Webb, Bulger, Snyder, Brewer, Gilbert, Moore (bib30) 2004; 40 Henriksen, Posch (bib11) 2001; 1 Henriksen, Kämäri, Posch, Wilander (bib12) 1992; 21 McDonnell, Cosby, Sullivan, McNulty, Cohen (bib20) 2010; 158 Cosby, Ferrier, Jenkins, Wright (bib6) 2001; 5 Lepistö, Whitehead, Neal, Cosby (bib18) 1988; 19 Cosby, Wright, Hornberger, Galloway (bib2) 1985; 21 Wright, Cosby, Flaten, Reuss (bib40) 1990; 343 Li, McNulty (bib19) 2007; 149 NRCS (Natural Resources Conservation Service) (bib22) 2009 Hall, Wright, Sparks, Ullyett, Allott, Hornung (bib8) 1995; 85 (bib26) 2003 U. S. EPA (U.S. Environmental Protection Agency) (bib35) 2009 U. S. EPA (U.S. Environmental Protection Agency), USGS (U.S. Geological Survey) (bib36) 2005 Omernik (bib25) 1987; 77 Hornberger, Cosby, Wright (bib14) 1989; 25 Harris, Fotheringham, Juggins (bib9) 2010; 100 Jenkins, Cosby, Ferrier, Walker, Miller (bib15) 1990; 120 Whitehead, Bird, Hornung, Cosby, Neal, Parcios (bib39) 1988; 101 Sullivan, Cosby (bib28) 1995; 85 Gregor, Werner, Spranger (bib7) 2004 Cosby, Norton, Kahl (bib5) 1996; 183 Rapp, Bishop (bib27) 2009; 13 Cosby, Ryan, Webb, Hornberger, Galloway, Charles (bib4) 1991 Jenkins, Whitehead, Cosby, Birks (bib16) 1990; 327 Turner, Cook, van Miegroet, Johnson, Elwood, Bricker, Lindberg, Hornberger (bib33) 1990 Norton, Wright, Kahl, Schofield (bib24) 1992; 77 USGS (U.S. Geological Survey) (bib37) 1999 Sullivan, Cosby, Driscoll, Charles, Hemond (bib29) 1996; 91 (bib23) 1988; vol. 15 Sverdrup, De Vries (bib32) 1994; 72 Verdin, Worstell (bib38) 2008; 44 Aherne, Posch, Dillon, Henriksen (bib1) 2004; 4 Henriksen (bib10) 1984; 22 NRCS (Natural Resources Conservation Service) (bib21) 2009 Umweltbundesamt (bib34) 2004 Wright, Cosby, Ferrier, Jenkins, Bulger, Harriman (bib41) 1994; 161 Cosby, Jenkins, Ferrier, Miller, Walker (bib3) 1990; 120 Sullivan, Webb, Snyder, Herlihy, Cosby (bib31) 2007; 182 Cosby (10.1016/j.envpol.2011.11.025_bib4) 1991 Sullivan (10.1016/j.envpol.2011.11.025_bib28) 1995; 85 (10.1016/j.envpol.2011.11.025_bib23) 1988; vol. 15 Norton (10.1016/j.envpol.2011.11.025_bib24) 1992; 77 Henriksen (10.1016/j.envpol.2011.11.025_bib11) 2001; 1 Omernik (10.1016/j.envpol.2011.11.025_bib25) 1987; 77 Lepistö (10.1016/j.envpol.2011.11.025_bib18) 1988; 19 Gregor (10.1016/j.envpol.2011.11.025_bib7) 2004 Turner (10.1016/j.envpol.2011.11.025_bib33) 1990 Sullivan (10.1016/j.envpol.2011.11.025_bib31) 2007; 182 Sverdrup (10.1016/j.envpol.2011.11.025_bib32) 1994; 72 Hall (10.1016/j.envpol.2011.11.025_bib8) 1995; 85 U. S. EPA (U.S. Environmental Protection Agency) (10.1016/j.envpol.2011.11.025_bib35) 2009 NRCS (Natural Resources Conservation Service) (10.1016/j.envpol.2011.11.025_bib22) 2009 Sullivan (10.1016/j.envpol.2011.11.025_bib29) 1996; 91 Aherne (10.1016/j.envpol.2011.11.025_bib1) 2004; 4 Wright (10.1016/j.envpol.2011.11.025_bib40) 1990; 343 Li (10.1016/j.envpol.2011.11.025_bib19) 2007; 149 Harris (10.1016/j.envpol.2011.11.025_bib9) 2010; 100 Rapp (10.1016/j.envpol.2011.11.025_bib27) 2009; 13 Jenkins (10.1016/j.envpol.2011.11.025_bib16) 1990; 327 McDonnell (10.1016/j.envpol.2011.11.025_bib20) 2010; 158 Henriksen (10.1016/j.envpol.2011.11.025_bib13) 2002; 59 USGS (U.S. Geological Survey) (10.1016/j.envpol.2011.11.025_bib37) 1999 Cosby (10.1016/j.envpol.2011.11.025_bib3) 1990; 120 Jenkins (10.1016/j.envpol.2011.11.025_bib15) 1990; 120 Sullivan (10.1016/j.envpol.2011.11.025_bib30) 2004; 40 Henriksen (10.1016/j.envpol.2011.11.025_bib10) 1984; 22 Henriksen (10.1016/j.envpol.2011.11.025_bib12) 1992; 21 (10.1016/j.envpol.2011.11.025_bib26) 2003 Hornberger (10.1016/j.envpol.2011.11.025_bib14) 1989; 25 Verdin (10.1016/j.envpol.2011.11.025_bib38) 2008; 44 Jenkins (10.1016/j.envpol.2011.11.025_bib17) 1990; 116 NRCS (Natural Resources Conservation Service) (10.1016/j.envpol.2011.11.025_bib21) 2009 Cosby (10.1016/j.envpol.2011.11.025_bib2) 1985; 21 Cosby (10.1016/j.envpol.2011.11.025_bib6) 2001; 5 Whitehead (10.1016/j.envpol.2011.11.025_bib39) 1988; 101 Umweltbundesamt (10.1016/j.envpol.2011.11.025_bib34) 2004 Wright (10.1016/j.envpol.2011.11.025_bib41) 1994; 161 U. S. EPA (U.S. Environmental Protection Agency) (10.1016/j.envpol.2011.11.025_bib36) 2005 Cosby (10.1016/j.envpol.2011.11.025_bib5) 1996; 183 |
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) is useful for watershed research and management. Existing regional approaches for estimating... Estimation of base cation supply from mineral weathering (BCw) is useful for watershed research and management. Existing regional approaches for estimating BCw... Estimation of base cation supply from mineral weathering (BC(w)) is useful for watershed research and management. Existing regional approaches for estimating... Estimation of base cation supply from mineral weathering (BC sub(w)) is useful for watershed research and management. Existing regional approaches for... |
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SubjectTerms | Acidic deposition Acidification Acids - analysis Appalachian Region Applied sciences Base cation Calibration Cations Cations - analysis Continental surface waters Critical load Earth sciences Earth, ocean, space ecoregions ecosystems Empirical analysis Engineering and environment geology. Geothermics Environmental Monitoring - methods Estimates Estimating Exact sciences and technology landscapes national parks Natural water pollution Pollution Pollution, environment geology Rivers - chemistry soil Soil - chemistry Streams United States Water treatment and pollution Watersheds Weathering wilderness |
Title | Regionalization of soil base cation weathering for evaluating stream water acidification in the Appalachian Mountains, USA |
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