Supramolecular Assembly-Induced Emission Enhancement for Efficient Mercury(II) Detection and Removal

New strategies that can simultaneously detect and remove highly toxic environmental pollutants such as heavy metal ions are still in urgent need. Herein, through supramolecular host–guest interactions, a fluorescent supramolecular polymer has been facilely constructed from a newly designed [2]­biphe...

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Published inJournal of the American Chemical Society Vol. 141; no. 11; pp. 4756 - 4763
Main Authors Dai, Dihua, Li, Zheng, Yang, Jie, Wang, Chunyu, Wu, Jia-Rui, Wang, Yan, Zhang, Dongmei, Yang, Ying-Wei
Format Journal Article
LanguageEnglish
Published WASHINGTON American Chemical Society 20.03.2019
Amer Chemical Soc
Subjects
adsorption
aromatic hydrocarbons
Chemistry
Chemistry, Multidisciplinary
environmental sustainability
fluorescence
heavy metals
mercury
metal ions
nanoparticles
Physical Sciences
pollutants
pollution
polymers
quaternary ammonium compounds
Science & Technology
sodium sulfide
thymine
toxicity
HOSTS
DESIGN
HG2
METAL-ORGANIC FRAMEWORKS
CONVERSION
POLYMER
AGGREGATION-INDUCED-EMISSION
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Abstract New strategies that can simultaneously detect and remove highly toxic environmental pollutants such as heavy metal ions are still in urgent need. Herein, through supramolecular host–guest interactions, a fluorescent supramolecular polymer has been facilely constructed from a newly designed [2]­biphenyl-extended pillar[6]­arene equipped with two thymine sites as arms (H) and a tetraphenylethylene (TPE)-bridged bis­(quaternary ammonium) guest (G) with aggregation-induced emission (AIE) property. Interestingly, supramolecular assembly-induced emission enhancement (SAIEE) could be switched on upon addition of Hg2+ into the above-mentioned supramolecular polymer system to generate spherical-like supramolecular nanoparticles, due to the restriction of intramolecular rotation (RIR)-related AIE feature of G. Significantly, this supramolecular polymer with integrated modalities has been successfully used for real-time detection and removal of toxic heavy metal Hg2+ ions from water with quick response, high selectivity, and rapid adsorption rates, which could be efficiently regenerated and recycled without any loss via a simple treatment with Na2S. The newly developed supramolecular polymer system combines the inherent rigid and spacious cavity of novel extended-pillarene host with the AIE characteristics of TPE-based guest, suggesting a great potential in the treatment of heavy metal pollution and environmental sustainability.
AbstractList New strategies that can simultaneously detect and remove highly toxic environmental pollutants such as heavy metal ions are still in urgent need. Herein, through supramolecular host–guest interactions, a fluorescent supramolecular polymer has been facilely constructed from a newly designed [2]biphenyl-extended pillar[6]arene equipped with two thymine sites as arms (H) and a tetraphenylethylene (TPE)-bridged bis(quaternary ammonium) guest (G) with aggregation-induced emission (AIE) property. Interestingly, supramolecular assembly-induced emission enhancement (SAIEE) could be switched on upon addition of Hg²⁺ into the above-mentioned supramolecular polymer system to generate spherical-like supramolecular nanoparticles, due to the restriction of intramolecular rotation (RIR)-related AIE feature of G. Significantly, this supramolecular polymer with integrated modalities has been successfully used for real-time detection and removal of toxic heavy metal Hg²⁺ ions from water with quick response, high selectivity, and rapid adsorption rates, which could be efficiently regenerated and recycled without any loss via a simple treatment with Na₂S. The newly developed supramolecular polymer system combines the inherent rigid and spacious cavity of novel extended-pillarene host with the AIE characteristics of TPE-based guest, suggesting a great potential in the treatment of heavy metal pollution and environmental sustainability.
New strategies that can simultaneously detect and remove highly toxic environmental pollutants such as heavy metal ions are still in urgent need. Herein, through supramolecular host-guest interactions, a fluorescent supramolecular polymer has been facilely constructed from a newly designed [2]biphenyl-extended pillar[6]arene equipped with two thymine sites as arms (H) and a tetraphenylethylene (TPE)-bridged bis(quaternary ammonium) guest (G) with aggregation-induced emission (AIE) property. Interestingly, supramolecular assembly-induced emission enhancement (SAIEE) could be switched on upon addition of Hg2+ into the above-mentioned supramolecular polymer system to generate spherical-like supramolecular nanoparticles, due to the restriction of intramolecular rotation (RIR)-related AIE feature of G. Significantly, this supramolecular polymer with integrated modalities has been successfully used for real-time detection and removal of toxic heavy metal Hg2+ ions from water with quick response, high selectivity, and rapid adsorption rates, which could be efficiently regenerated and recycled without any loss via a simple treatment with Na2S. The newly developed supramolecular polymer system combines the inherent rigid and spacious cavity of novel extended-pillarene host with the AIE characteristics of TPE-based guest, suggesting a great potential in the treatment of heavy metal pollution and environmental sustainability.
New strategies that can simultaneously detect and remove highly toxic environmental pollutants such as heavy metal ions are still in urgent need. Herein, through supramolecular host-guest interactions, a fluorescent supramolecular polymer has been facilely constructed from a newly designed [2]biphenyl-extended pillar[6]arene equipped with two thymine sites as arms (H) and a tetraphenylethylene (TPE)-bridged bis(quaternary ammonium) guest (G) with aggregation-induced emission (AIE) property. Interestingly, supramolecular assembly-induced emission enhancement (SAIEE) could be switched on upon addition of Hg into the above-mentioned supramolecular polymer system to generate spherical-like supramolecular nanoparticles, due to the restriction of intramolecular rotation (RIR)-related AIE feature of G. Significantly, this supramolecular polymer with integrated modalities has been successfully used for real-time detection and removal of toxic heavy metal Hg ions from water with quick response, high selectivity, and rapid adsorption rates, which could be efficiently regenerated and recycled without any loss via a simple treatment with Na S. The newly developed supramolecular polymer system combines the inherent rigid and spacious cavity of novel extended-pillarene host with the AIE characteristics of TPE-based guest, suggesting a great potential in the treatment of heavy metal pollution and environmental sustainability.
New strategies that can simultaneously detect and remove highly toxic environmental pollutants such as heavy metal ions are still in urgent need. Herein, through supramolecular host–guest interactions, a fluorescent supramolecular polymer has been facilely constructed from a newly designed [2]­biphenyl-extended pillar[6]­arene equipped with two thymine sites as arms (H) and a tetraphenylethylene (TPE)-bridged bis­(quaternary ammonium) guest (G) with aggregation-induced emission (AIE) property. Interestingly, supramolecular assembly-induced emission enhancement (SAIEE) could be switched on upon addition of Hg2+ into the above-mentioned supramolecular polymer system to generate spherical-like supramolecular nanoparticles, due to the restriction of intramolecular rotation (RIR)-related AIE feature of G. Significantly, this supramolecular polymer with integrated modalities has been successfully used for real-time detection and removal of toxic heavy metal Hg2+ ions from water with quick response, high selectivity, and rapid adsorption rates, which could be efficiently regenerated and recycled without any loss via a simple treatment with Na2S. The newly developed supramolecular polymer system combines the inherent rigid and spacious cavity of novel extended-pillarene host with the AIE characteristics of TPE-based guest, suggesting a great potential in the treatment of heavy metal pollution and environmental sustainability.
New strategies that can simultaneously detect and remove highly toxic environmental pollutants such as heavy metal ions are still in urgent need. Herein, through supramolecular host-guest interactions, a fluorescent supramolecular polymer has been facilely constructed from a newly designed [2]biphenyl-extended pillar[6]arene equipped with two thymine sites as arms (H) and a tetraphenylethylene (TPE)-bridged bis(quaternary ammonium) guest (G) with aggregation-induced emission (AIE) property. Interestingly, supramolecular assembly-induced emission enhancement (SAIEE) could be switched on upon addition of Hg2+ into the above-mentioned supramolecular polymer system to generate spherical-like supramolecular nanoparticles, due to the restriction of intramolecular rotation (RIR)-related AIE feature of G. Significantly, this supramolecular polymer with integrated modalities has been successfully used for real-time detection and removal of toxic heavy metal Hg2+ ions from water with quick response, high selectivity, and rapid adsorption rates, which could be efficiently regenerated and recycled without any loss via a simple treatment with Na2S. The newly developed supramolecular polymer system combines the inherent rigid and spacious cavity of novel extended-pillarene host with the AIE characteristics of TPE-based guest, suggesting a great potential in the treatment of heavy metal pollution and environmental sustainability.New strategies that can simultaneously detect and remove highly toxic environmental pollutants such as heavy metal ions are still in urgent need. Herein, through supramolecular host-guest interactions, a fluorescent supramolecular polymer has been facilely constructed from a newly designed [2]biphenyl-extended pillar[6]arene equipped with two thymine sites as arms (H) and a tetraphenylethylene (TPE)-bridged bis(quaternary ammonium) guest (G) with aggregation-induced emission (AIE) property. Interestingly, supramolecular assembly-induced emission enhancement (SAIEE) could be switched on upon addition of Hg2+ into the above-mentioned supramolecular polymer system to generate spherical-like supramolecular nanoparticles, due to the restriction of intramolecular rotation (RIR)-related AIE feature of G. Significantly, this supramolecular polymer with integrated modalities has been successfully used for real-time detection and removal of toxic heavy metal Hg2+ ions from water with quick response, high selectivity, and rapid adsorption rates, which could be efficiently regenerated and recycled without any loss via a simple treatment with Na2S. The newly developed supramolecular polymer system combines the inherent rigid and spacious cavity of novel extended-pillarene host with the AIE characteristics of TPE-based guest, suggesting a great potential in the treatment of heavy metal pollution and environmental sustainability.
Author Zhang, Dongmei
Li, Zheng
Wu, Jia-Rui
Dai, Dihua
Yang, Ying-Wei
Yang, Jie
Wang, Chunyu
Wang, Yan
AuthorAffiliation California NanoSystems Institute and Departments of Chemistry & Biochemistry
University of California
School of Environment
State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, International Joint Research Laboratory of Nano-Micro Architecture Chemistry (NMAC), College of Chemistry
State Key Laboratory of Supramolecular Structure and Materials, Institute of Theoretical Chemistry
AuthorAffiliation_xml – name: State Key Laboratory of Supramolecular Structure and Materials, Institute of Theoretical Chemistry
– name: School of Environment
– name: University of California
– name: State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, International Joint Research Laboratory of Nano-Micro Architecture Chemistry (NMAC), College of Chemistry
– name: California NanoSystems Institute and Departments of Chemistry & Biochemistry
Author_xml – sequence: 1
  givenname: Dihua
  surname: Dai
  fullname: Dai, Dihua
– sequence: 2
  givenname: Zheng
  surname: Li
  fullname: Li, Zheng
– sequence: 3
  givenname: Jie
  surname: Yang
  fullname: Yang, Jie
– sequence: 4
  givenname: Chunyu
  surname: Wang
  fullname: Wang, Chunyu
– sequence: 5
  givenname: Jia-Rui
  surname: Wu
  fullname: Wu, Jia-Rui
– sequence: 6
  givenname: Yan
  surname: Wang
  fullname: Wang, Yan
– sequence: 7
  givenname: Dongmei
  surname: Zhang
  fullname: Zhang, Dongmei
  organization: School of Environment
– sequence: 8
  givenname: Ying-Wei
  orcidid: 0000-0001-8839-8161
  surname: Yang
  fullname: Yang, Ying-Wei
  email: ywyang@jlu.edu.cn
  organization: University of California
BackLink https://www.ncbi.nlm.nih.gov/pubmed/30807128$$D View this record in MEDLINE/PubMed
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Snippet New strategies that can simultaneously detect and remove highly toxic environmental pollutants such as heavy metal ions are still in urgent need. Herein,...
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SubjectTerms adsorption
aromatic hydrocarbons
Chemistry
Chemistry, Multidisciplinary
environmental sustainability
fluorescence
heavy metals
mercury
metal ions
nanoparticles
Physical Sciences
pollutants
pollution
polymers
quaternary ammonium compounds
Science & Technology
sodium sulfide
thymine
toxicity
Title Supramolecular Assembly-Induced Emission Enhancement for Efficient Mercury(II) Detection and Removal
URI http://dx.doi.org/10.1021/jacs.9b01546
http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=Summon&SrcAuth=ProQuest&DestApp=WOS&DestLinkType=FullRecord&UT=000462260400035
https://www.ncbi.nlm.nih.gov/pubmed/30807128
https://www.proquest.com/docview/2186617645
https://www.proquest.com/docview/2237512827
Volume 141
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