Ultrathin and Ion-Selective Janus Membranes for High-Performance Osmotic Energy Conversion
The osmotic energy existing in fluids is recognized as a promising “blue” energy source that can help solve the global issues of energy shortage and environmental pollution. Recently, nanofluidic channels have shown great potential for capturing this worldwide energy because of their novel transport...
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| Published in | Journal of the American Chemical Society Vol. 139; no. 26; pp. 8905 - 8914 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
05.07.2017
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The osmotic energy existing in fluids is recognized as a promising “blue” energy source that can help solve the global issues of energy shortage and environmental pollution. Recently, nanofluidic channels have shown great potential for capturing this worldwide energy because of their novel transport properties contributed by nanoconfinement. However, with respect to membrane-scale porous systems, high resistance and undesirable ion selectivity remain bottlenecks, impeding their applications. The development of thinner, low-resistance membranes, meanwhile promoting their ion selectivity, is a necessity. Here, we engineered ultrathin and ion-selective Janus membranes prepared via the phase separation of two block copolymers, which enable osmotic energy conversion with power densities of approximately 2.04 W/m2 by mixing natural seawater and river water. Both experiments and continuum simulation help us to understand the mechanism for how membrane thickness and channel structure dominate the ion transport process and overall device performance, which can serve as a general guiding principle for the future design of nanochannel membranes for high-energy concentration cells. |
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| AbstractList | The osmotic energy existing in fluids is recognized as a promising "blue" energy source that can help solve the global issues of energy shortage and environmental pollution. Recently, nanofluidic channels have shown great potential for capturing this worldwide energy because of their novel transport properties contributed by nanoconfinement. However, with respect to membrane-scale porous systems, high resistance and undesirable ion selectivity remain bottlenecks, impeding their applications. The development of thinner, low-resistance membranes, meanwhile promoting their ion selectivity, is a necessity. Here, we engineered ultrathin and ion-selective Janus membranes prepared via the phase separation of two block copolymers, which enable osmotic energy conversion with power densities of approximately 2.04 W/m
by mixing natural seawater and river water. Both experiments and continuum simulation help us to understand the mechanism for how membrane thickness and channel structure dominate the ion transport process and overall device performance, which can serve as a general guiding principle for the future design of nanochannel membranes for high-energy concentration cells. The osmotic energy existing in fluids is recognized as a promising “blue” energy source that can help solve the global issues of energy shortage and environmental pollution. Recently, nanofluidic channels have shown great potential for capturing this worldwide energy because of their novel transport properties contributed by nanoconfinement. However, with respect to membrane-scale porous systems, high resistance and undesirable ion selectivity remain bottlenecks, impeding their applications. The development of thinner, low-resistance membranes, meanwhile promoting their ion selectivity, is a necessity. Here, we engineered ultrathin and ion-selective Janus membranes prepared via the phase separation of two block copolymers, which enable osmotic energy conversion with power densities of approximately 2.04 W/m² by mixing natural seawater and river water. Both experiments and continuum simulation help us to understand the mechanism for how membrane thickness and channel structure dominate the ion transport process and overall device performance, which can serve as a general guiding principle for the future design of nanochannel membranes for high-energy concentration cells. The osmotic energy existing in fluids is recognized as a promising “blue” energy source that can help solve the global issues of energy shortage and environmental pollution. Recently, nanofluidic channels have shown great potential for capturing this worldwide energy because of their novel transport properties contributed by nanoconfinement. However, with respect to membrane-scale porous systems, high resistance and undesirable ion selectivity remain bottlenecks, impeding their applications. The development of thinner, low-resistance membranes, meanwhile promoting their ion selectivity, is a necessity. Here, we engineered ultrathin and ion-selective Janus membranes prepared via the phase separation of two block copolymers, which enable osmotic energy conversion with power densities of approximately 2.04 W/m2 by mixing natural seawater and river water. Both experiments and continuum simulation help us to understand the mechanism for how membrane thickness and channel structure dominate the ion transport process and overall device performance, which can serve as a general guiding principle for the future design of nanochannel membranes for high-energy concentration cells. The osmotic energy existing in fluids is recognized as a promising "blue" energy source that can help solve the global issues of energy shortage and environmental pollution. Recently, nanofluidic channels have shown great potential for capturing this worldwide energy because of their novel transport properties contributed by nanoconfinement. However, with respect to membrane-scale porous systems, high resistance and undesirable ion selectivity remain bottlenecks, impeding their applications. The development of thinner, low-resistance membranes, meanwhile promoting their ion selectivity, is a necessity. Here, we engineered ultrathin and ion-selective Janus membranes prepared via the phase separation of two block copolymers, which enable osmotic energy conversion with power densities of approximately 2.04 W/m2 by mixing natural seawater and river water. Both experiments and continuum simulation help us to understand the mechanism for how membrane thickness and channel structure dominate the ion transport process and overall device performance, which can serve as a general guiding principle for the future design of nanochannel membranes for high-energy concentration cells.The osmotic energy existing in fluids is recognized as a promising "blue" energy source that can help solve the global issues of energy shortage and environmental pollution. Recently, nanofluidic channels have shown great potential for capturing this worldwide energy because of their novel transport properties contributed by nanoconfinement. However, with respect to membrane-scale porous systems, high resistance and undesirable ion selectivity remain bottlenecks, impeding their applications. The development of thinner, low-resistance membranes, meanwhile promoting their ion selectivity, is a necessity. Here, we engineered ultrathin and ion-selective Janus membranes prepared via the phase separation of two block copolymers, which enable osmotic energy conversion with power densities of approximately 2.04 W/m2 by mixing natural seawater and river water. Both experiments and continuum simulation help us to understand the mechanism for how membrane thickness and channel structure dominate the ion transport process and overall device performance, which can serve as a general guiding principle for the future design of nanochannel membranes for high-energy concentration cells. |
| Author | Sui, Xin Li, Pei Xie, Ganhua Wen, Liping Xiao, Kai Zhang, Zhen Gao, Longcheng Kong, Xiang-Yu Jiang, Lei |
| AuthorAffiliation | Chinese Academy of Sciences School of Chemistry and Environment Key Laboratory of Bio-inspired Materials and Interfacial Science, Technical Institute of Physics and Chemistry Beijing National Laboratory for Molecular Sciences (BNLMS), Key Laboratory of Green Printing, Institute of Chemistry University of Chinese Academy of Sciences |
| AuthorAffiliation_xml | – name: Beijing National Laboratory for Molecular Sciences (BNLMS), Key Laboratory of Green Printing, Institute of Chemistry – name: Key Laboratory of Bio-inspired Materials and Interfacial Science, Technical Institute of Physics and Chemistry – name: School of Chemistry and Environment – name: University of Chinese Academy of Sciences – name: Chinese Academy of Sciences |
| Author_xml | – sequence: 1 givenname: Zhen surname: Zhang fullname: Zhang, Zhen organization: University of Chinese Academy of Sciences – sequence: 2 givenname: Xin surname: Sui fullname: Sui, Xin organization: School of Chemistry and Environment – sequence: 3 givenname: Pei surname: Li fullname: Li, Pei organization: School of Chemistry and Environment – sequence: 4 givenname: Ganhua surname: Xie fullname: Xie, Ganhua organization: University of Chinese Academy of Sciences – sequence: 5 givenname: Xiang-Yu surname: Kong fullname: Kong, Xiang-Yu organization: Chinese Academy of Sciences – sequence: 6 givenname: Kai surname: Xiao fullname: Xiao, Kai organization: University of Chinese Academy of Sciences – sequence: 7 givenname: Longcheng surname: Gao fullname: Gao, Longcheng email: lcgao@buaa.edu.cn organization: School of Chemistry and Environment – sequence: 8 givenname: Liping surname: Wen fullname: Wen, Liping email: wen@mail.ipc.ac.cn organization: University of Chinese Academy of Sciences – sequence: 9 givenname: Lei orcidid: 0000-0003-4579-728X surname: Jiang fullname: Jiang, Lei organization: University of Chinese Academy of Sciences |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28602079$$D View this record in MEDLINE/PubMed |
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| Title | Ultrathin and Ion-Selective Janus Membranes for High-Performance Osmotic Energy Conversion |
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