2D Intrinsic Ferromagnets from van der Waals Antiferromagnets
Intrinsically ferromagnetic 2D semiconductors are essential and highly sought for nanoscale spintronics, but they can only be obtained from ferromagnetic bulk crystals, while the possibility to create 2D intrinsic ferromagnets from bulk antiferromagnets remains unknown. Herein on the basis of ab ini...
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| Published in | Journal of the American Chemical Society Vol. 140; no. 7; pp. 2417 - 2420 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
21.02.2018
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Intrinsically ferromagnetic 2D semiconductors are essential and highly sought for nanoscale spintronics, but they can only be obtained from ferromagnetic bulk crystals, while the possibility to create 2D intrinsic ferromagnets from bulk antiferromagnets remains unknown. Herein on the basis of ab initio calculations, we demonstrate this feasibility with the discovery of intrinsic ferromagnetism in an emerging class of single-layer 2D semiconductors CrOX (CrOCl and CrOBr monolayers), which show robust ferromagnetic ordering, large spin polarization, and high Curie temperature. These 2D crystals promise great dynamical and thermal stabilities as well as easy experimental fabrication from their bulk antiferromagnets. The Curie temperature of 2D CrOCl is 160 K, which exceeds the record (155 K) of the most-studied dilute magnetic GaMnAs materials, and could be further enhanced by appropriate strains. Our study offers an alternative promising way to create 2D intrinsic ferromagnets from their antiferromagnetic bulk counterparts and also renders 2D CrOX monolayers great platform for future spintronics. |
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| AbstractList | Intrinsically ferromagnetic 2D semiconductors are essential and highly sought for nanoscale spintronics, but they can only be obtained from ferromagnetic bulk crystals, while the possibility to create 2D intrinsic ferromagnets from bulk antiferromagnets remains unknown. Herein on the basis of ab initio calculations, we demonstrate this feasibility with the discovery of intrinsic ferromagnetism in an emerging class of single-layer 2D semiconductors CrOX (CrOCl and CrOBr monolayers), which show robust ferromagnetic ordering, large spin polarization, and high Curie temperature. These 2D crystals promise great dynamical and thermal stabilities as well as easy experimental fabrication from their bulk antiferromagnets. The Curie temperature of 2D CrOCl is 160 K, which exceeds the record (155 K) of the most-studied dilute magnetic GaMnAs materials, and could be further enhanced by appropriate strains. Our study offers an alternative promising way to create 2D intrinsic ferromagnets from their antiferromagnetic bulk counterparts and also renders 2D CrOX monolayers great platform for future spintronics.Intrinsically ferromagnetic 2D semiconductors are essential and highly sought for nanoscale spintronics, but they can only be obtained from ferromagnetic bulk crystals, while the possibility to create 2D intrinsic ferromagnets from bulk antiferromagnets remains unknown. Herein on the basis of ab initio calculations, we demonstrate this feasibility with the discovery of intrinsic ferromagnetism in an emerging class of single-layer 2D semiconductors CrOX (CrOCl and CrOBr monolayers), which show robust ferromagnetic ordering, large spin polarization, and high Curie temperature. These 2D crystals promise great dynamical and thermal stabilities as well as easy experimental fabrication from their bulk antiferromagnets. The Curie temperature of 2D CrOCl is 160 K, which exceeds the record (155 K) of the most-studied dilute magnetic GaMnAs materials, and could be further enhanced by appropriate strains. Our study offers an alternative promising way to create 2D intrinsic ferromagnets from their antiferromagnetic bulk counterparts and also renders 2D CrOX monolayers great platform for future spintronics. Intrinsically ferromagnetic 2D semiconductors are essential and highly sought for nanoscale spintronics, but they can only be obtained from ferromagnetic bulk crystals, while the possibility to create 2D intrinsic ferromagnets from bulk antiferromagnets remains unknown. Herein on the basis of ab initio calculations, we demonstrate this feasibility with the discovery of intrinsic ferromagnetism in an emerging class of single-layer 2D semiconductors CrOX (CrOCl and CrOBr monolayers), which show robust ferromagnetic ordering, large spin polarization, and high Curie temperature. These 2D crystals promise great dynamical and thermal stabilities as well as easy experimental fabrication from their bulk antiferromagnets. The Curie temperature of 2D CrOCl is 160 K, which exceeds the record (155 K) of the most-studied dilute magnetic GaMnAs materials, and could be further enhanced by appropriate strains. Our study offers an alternative promising way to create 2D intrinsic ferromagnets from their antiferromagnetic bulk counterparts and also renders 2D CrOX monolayers great platform for future spintronics. |
| Author | Xu, Bin Zhou, Jian Zhu, Linggang Miao, Naihua Sun, Zhimei |
| AuthorAffiliation | Physics Department and Institute for Nanoscience and Engineering School of Materials Science and Engineering Center for Integrated Computational Materials Engineering, International Research Institute for Multidisciplinary Science University of Arkansas Beihang University |
| AuthorAffiliation_xml | – name: Center for Integrated Computational Materials Engineering, International Research Institute for Multidisciplinary Science – name: Beihang University – name: School of Materials Science and Engineering – name: University of Arkansas – name: Physics Department and Institute for Nanoscience and Engineering |
| Author_xml | – sequence: 1 givenname: Naihua orcidid: 0000-0002-5383-9008 surname: Miao fullname: Miao, Naihua organization: Beihang University – sequence: 2 givenname: Bin surname: Xu fullname: Xu, Bin organization: University of Arkansas – sequence: 3 givenname: Linggang orcidid: 0000-0003-2514-4177 surname: Zhu fullname: Zhu, Linggang organization: Beihang University – sequence: 4 givenname: Jian surname: Zhou fullname: Zhou, Jian organization: Beihang University – sequence: 5 givenname: Zhimei orcidid: 0000-0002-4438-5032 surname: Sun fullname: Sun, Zhimei email: zmsun@buaa.edu.cn organization: Beihang University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29400056$$D View this record in MEDLINE/PubMed |
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| Title | 2D Intrinsic Ferromagnets from van der Waals Antiferromagnets |
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