Chemiresistive Sensor Arrays from Conductive 2D Metal–Organic Frameworks
Applications of porous metal–organic frameworks (MOFs) in electronic devices are rare, owing in large part to a lack of MOFs that display electrical conductivity. Here, we describe the use of conductive two-dimensional (2D) MOFs as a new class of materials for chemiresistive sensing of volatile org...
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| Published in | Journal of the American Chemical Society Vol. 137; no. 43; pp. 13780 - 13783 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
04.11.2015
American Chemical Society (ACS) |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Applications of porous metal–organic frameworks (MOFs) in electronic devices are rare, owing in large part to a lack of MOFs that display electrical conductivity. Here, we describe the use of conductive two-dimensional (2D) MOFs as a new class of materials for chemiresistive sensing of volatile organic compounds (VOCs). We demonstrate that a family of structurally analogous 2D MOFs can be used to construct a cross-reactive sensor array that allows for clear discrimination between different categories of VOCs. Experimental data show that multiple sensing mechanisms are operative with high degrees of orthogonality, establishing that the 2D MOFs used here are mechanistically unique and offer advantages relative to other known chemiresistor materials. |
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| AbstractList | Applications of porous metal–organic frameworks (MOFs) in electronic devices are rare, owing in large part to a lack of MOFs that display electrical conductivity. Here, we describe the use of conductive two-dimensional (2D) MOFs as a new class of materials for chemiresistive sensing of volatile organic compounds (VOCs). We demonstrate that a family of structurally analogous 2D MOFs can be used to construct a cross-reactive sensor array that allows for clear discrimination between different categories of VOCs. Experimental data show that multiple sensing mechanisms are operative with high degrees of orthogonality, establishing that the 2D MOFs used here are mechanistically unique and offer advantages relative to other known chemiresistor materials. Applications of porous metal–organic frameworks (MOFs) in electronic devices are rare, owing in large part to a lack of MOFs that display electrical conductivity. Here, we describe the use of conductive two-dimensional (2D) MOFs as a new class of materials for chemiresistive sensing of volatile organic compounds (VOCs). We demonstrate that a family of structurally analogous 2D MOFs can be used to construct a cross-reactive sensor array that allows for clear discrimination between different categories of VOCs. Lastly, experimental data show that multiple sensing mechanisms are operative with high degrees of orthogonality, establishing that the 2D MOFs used here are mechanistically unique and offer advantages relative to other known chemiresistor materials. Applications of porous metal–organic frameworks (MOFs) in electronic devices are rare, owing in large part to a lack of MOFs that display electrical conductivity. Here, we describe the use of conductive two-dimensional (2D) MOFs as a new class of materials for chemiresistive sensing of volatile organic compounds (VOCs). We demonstrate that a family of structurally analogous 2D MOFs can be used to construct a cross-reactive sensor array that allows for clear discrimination between different categories of VOCs. Experimental data show that multiple sensing mechanisms are operative with high degrees of orthogonality, establishing that the 2D MOFs used here are mechanistically unique and offer advantages relative to other known chemiresistor materials. |
| Author | Campbell, Michael G Dincă, Mircea Liu, Sophie F Swager, Timothy M |
| AuthorAffiliation | Department of Chemistry Massachusetts Institute of Technology |
| AuthorAffiliation_xml | – name: Massachusetts Institute of Technology – name: Department of Chemistry |
| Author_xml | – sequence: 1 givenname: Michael G surname: Campbell fullname: Campbell, Michael G – sequence: 2 givenname: Sophie F surname: Liu fullname: Liu, Sophie F – sequence: 3 givenname: Timothy M surname: Swager fullname: Swager, Timothy M – sequence: 4 givenname: Mircea surname: Dincă fullname: Dincă, Mircea email: mdinca@mit.edu |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/26456526$$D View this record in MEDLINE/PubMed https://www.osti.gov/servlets/purl/1386738$$D View this record in Osti.gov |
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| Snippet | Applications of porous metal–organic frameworks (MOFs) in electronic devices are rare, owing in large part to a lack of MOFs that display electrical... Applications of porous metal-organic frameworks (MOFs) in electronic devices are rare, owing in large part to a lack of MOFs that display electrical... |
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| SubjectTerms | charge transport coordination polymers electrical conductivity electronic equipment INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY optics photosynthesis (natural and artificial) solar (photovoltaic) solid state lighting synthesis (novel materials) synthesis (scalable processing) synthesis (self-assembly) volatile organic compounds |
| Title | Chemiresistive Sensor Arrays from Conductive 2D Metal–Organic Frameworks |
| URI | http://dx.doi.org/10.1021/jacs.5b09600 https://www.ncbi.nlm.nih.gov/pubmed/26456526 https://www.proquest.com/docview/1730685397 https://www.proquest.com/docview/2000343279 https://www.osti.gov/servlets/purl/1386738 |
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