Impact of Reabsorption on the Emission Spectra and Recombination Dynamics of Hybrid Perovskite Single Crystals

Understanding the surface properties of organic–inorganic lead-based perovskites is of high importance to improve the device’s performance. Here, we have investigated the differences between surface and bulk optical properties of CH3NH3PbBr3 single crystals. Depth-resolved cathodoluminescence was us...

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Published inThe journal of physical chemistry letters Vol. 8; no. 13; pp. 2977 - 2983
Main Authors Diab, Hiba, Arnold, Christophe, Lédée, Ferdinand, Trippé-Allard, Gaëlle, Delport, Géraud, Vilar, Christèle, Bretenaker, Fabien, Barjon, Julien, Lauret, Jean-Sébastien, Deleporte, Emmanuelle, Garrot, Damien
Format Journal Article
LanguageEnglish
Published United States American Chemical Society 06.07.2017
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Abstract Understanding the surface properties of organic–inorganic lead-based perovskites is of high importance to improve the device’s performance. Here, we have investigated the differences between surface and bulk optical properties of CH3NH3PbBr3 single crystals. Depth-resolved cathodoluminescence was used to probe the near-surface region on a depth of a few microns. In addition, we have studied the transmitted luminescence through thicknesses between 50 and 600 μm. In both experiments, the expected spectral shift due to the reabsorption effect has been precisely calculated. We demonstrate that reabsorption explains the important variations reported for the emission energy of single crystals. Single crystals are partially transparent to their own luminescence, and radiative transport is the dominant mechanism for propagation of the excitation in thick crystals. The transmitted luminescence dynamics are characterized by a long rise time and a lengthening of their decay due to photon recycling and light trapping.
AbstractList Understanding the surface properties of organic-inorganic lead-based perovskites is of high importance to improve the device's performance. Here, we have investigated the differences between surface and bulk optical properties of CH3NH3PbBr3 single crystals. Depth-resolved cathodoluminescence was used to probe the near-surface region on a depth of a few microns. In addition, we have studied the transmitted luminescence through thicknesses between 50 and 600 μm. In both experiments, the expected spectral shift due to the reabsorption effect has been precisely calculated. We demonstrate that reabsorption explains the important variations reported for the emission energy of single crystals. Single crystals are partially transparent to their own luminescence, and radiative transport is the dominant mechanism for propagation of the excitation in thick crystals. The transmitted luminescence dynamics are characterized by a long rise time and a lengthening of their decay due to photon recycling and light trapping.Understanding the surface properties of organic-inorganic lead-based perovskites is of high importance to improve the device's performance. Here, we have investigated the differences between surface and bulk optical properties of CH3NH3PbBr3 single crystals. Depth-resolved cathodoluminescence was used to probe the near-surface region on a depth of a few microns. In addition, we have studied the transmitted luminescence through thicknesses between 50 and 600 μm. In both experiments, the expected spectral shift due to the reabsorption effect has been precisely calculated. We demonstrate that reabsorption explains the important variations reported for the emission energy of single crystals. Single crystals are partially transparent to their own luminescence, and radiative transport is the dominant mechanism for propagation of the excitation in thick crystals. The transmitted luminescence dynamics are characterized by a long rise time and a lengthening of their decay due to photon recycling and light trapping.
Understanding the surface properties of organic-inorganic lead-based perovskites is of high importance to improve the device's performance. Here, we have investigated the differences between surface and bulk optical properties of CH NH PbBr single crystals. Depth-resolved cathodoluminescence was used to probe the near-surface region on a depth of a few microns. In addition, we have studied the transmitted luminescence through thicknesses between 50 and 600 μm. In both experiments, the expected spectral shift due to the reabsorption effect has been precisely calculated. We demonstrate that reabsorption explains the important variations reported for the emission energy of single crystals. Single crystals are partially transparent to their own luminescence, and radiative transport is the dominant mechanism for propagation of the excitation in thick crystals. The transmitted luminescence dynamics are characterized by a long rise time and a lengthening of their decay due to photon recycling and light trapping.
Understanding the surface properties of organic–inorganic lead-based perovskites is of high importance to improve the device’s performance. Here, we have investigated the differences between surface and bulk optical properties of CH3NH3PbBr3 single crystals. Depth-resolved cathodoluminescence was used to probe the near-surface region on a depth of a few microns. In addition, we have studied the transmitted luminescence through thicknesses between 50 and 600 μm. In both experiments, the expected spectral shift due to the reabsorption effect has been precisely calculated. We demonstrate that reabsorption explains the important variations reported for the emission energy of single crystals. Single crystals are partially transparent to their own luminescence, and radiative transport is the dominant mechanism for propagation of the excitation in thick crystals. The transmitted luminescence dynamics are characterized by a long rise time and a lengthening of their decay due to photon recycling and light trapping.
Author Deleporte, Emmanuelle
Garrot, Damien
Lédée, Ferdinand
Trippé-Allard, Gaëlle
Arnold, Christophe
Vilar, Christèle
Lauret, Jean-Sébastien
Diab, Hiba
Bretenaker, Fabien
Barjon, Julien
Delport, Géraud
AuthorAffiliation CNRS, Univ. Paris-Sud, ENS Paris-Saclay, Université Paris-Saclay
CNRS, Université de Versailles Saint Quentin En Yvelines, Université Paris-Saclay
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BackLink https://www.ncbi.nlm.nih.gov/pubmed/28608691$$D View this record in MEDLINE/PubMed
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Snippet Understanding the surface properties of organic–inorganic lead-based perovskites is of high importance to improve the device’s performance. Here, we have...
Understanding the surface properties of organic-inorganic lead-based perovskites is of high importance to improve the device's performance. Here, we have...
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Title Impact of Reabsorption on the Emission Spectra and Recombination Dynamics of Hybrid Perovskite Single Crystals
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