Space-Confined Seeded Growth of Black Silver Nanostructures for Solar Steam Generation
Plasmonic metal nanostructures have attracted considerable attention for solar energy harvesting due to their capability in photothermal conversion. However, the narrow resonant band of the conventional plasmonic nanoparticles greatly limits their application as only a small fraction of the solar en...
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| Published in | Nano letters Vol. 19; no. 1; pp. 400 - 407 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
09.01.2019
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Plasmonic metal nanostructures have attracted considerable attention for solar energy harvesting due to their capability in photothermal conversion. However, the narrow resonant band of the conventional plasmonic nanoparticles greatly limits their application as only a small fraction of the solar energy can be utilized. Herein, a unique confined seeded growth strategy is developed to synthesize black silver nanostructures with broadband absorption in the visible and near-infrared spectrum. Through this novel strategy, assemblages of silver nanoparticles with widely distributed interparticle distances are generated in rod-shaped tubular spaces, leading to strong random plasmonic coupling and accordingly broadband absorption for significantly improved utilization of solar energy. With excellent efficiency in converting solar energy to heat, the resulting black Ag nanostructures can be made into thin films floating at the air/water interface for efficient generation of clean water steam through localized interfacial heating. |
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| AbstractList | Plasmonic metal nanostructures have attracted considerable attention for solar energy harvesting due to their capability in photothermal conversion. However, the narrow resonant band of the conventional plasmonic nanoparticles greatly limits their application as only a small fraction of the solar energy can be utilized. Herein, a unique confined seeded growth strategy is developed to synthesize black silver nanostructures with broadband absorption in the visible and near-infrared spectrum. Through this novel strategy, assemblages of silver nanoparticles with widely distributed interparticle distances are generated in rod-shaped tubular spaces, leading to strong random plasmonic coupling and accordingly broadband absorption for significantly improved utilization of solar energy. With excellent efficiency in converting solar energy to heat, the resulting black Ag nanostructures can be made into thin films floating at the air/water interface for efficient generation of clean water steam through localized interfacial heating. Plasmonic metal nanostructures have attracted considerable attention for solar energy harvesting due to their capability in photothermal conversion. However, the narrow resonant band of the conventional plasmonic nanoparticles greatly limits their application as only a small fraction of the solar energy can be utilized. Herein, a unique confined seeded growth strategy is developed to synthesize black silver nanostructures with broadband absorption in the visible and near-infrared spectrum. Through this novel strategy, assemblages of silver nanoparticles with widely distributed interparticle distances are generated in rod-shaped tubular spaces, leading to strong random plasmonic coupling and accordingly broadband absorption for significantly improved utilization of solar energy. With excellent efficiency in converting solar energy to heat, the resulting black Ag nanostructures can be made into thin films floating at the air/water interface for efficient generation of clean water steam through localized interfacial heating.Plasmonic metal nanostructures have attracted considerable attention for solar energy harvesting due to their capability in photothermal conversion. However, the narrow resonant band of the conventional plasmonic nanoparticles greatly limits their application as only a small fraction of the solar energy can be utilized. Herein, a unique confined seeded growth strategy is developed to synthesize black silver nanostructures with broadband absorption in the visible and near-infrared spectrum. Through this novel strategy, assemblages of silver nanoparticles with widely distributed interparticle distances are generated in rod-shaped tubular spaces, leading to strong random plasmonic coupling and accordingly broadband absorption for significantly improved utilization of solar energy. With excellent efficiency in converting solar energy to heat, the resulting black Ag nanostructures can be made into thin films floating at the air/water interface for efficient generation of clean water steam through localized interfacial heating. |
| Author | Chen, Jinxing Wang, Mozhen Feng, Ji Yin, Yadong Li, Zhiwei Ge, Xuewu Wang, Xiaojing Xu, Panpan Yin, Wenwen |
| AuthorAffiliation | Department of Polymer Science and Engineering Department of Chemistry |
| AuthorAffiliation_xml | – name: Department of Polymer Science and Engineering – name: Department of Chemistry |
| Author_xml | – sequence: 1 givenname: Jinxing surname: Chen fullname: Chen, Jinxing organization: Department of Chemistry – sequence: 2 givenname: Ji surname: Feng fullname: Feng, Ji organization: Department of Chemistry – sequence: 3 givenname: Zhiwei surname: Li fullname: Li, Zhiwei organization: Department of Chemistry – sequence: 4 givenname: Panpan surname: Xu fullname: Xu, Panpan organization: Department of Chemistry – sequence: 5 givenname: Xiaojing surname: Wang fullname: Wang, Xiaojing organization: Department of Chemistry – sequence: 6 givenname: Wenwen surname: Yin fullname: Yin, Wenwen organization: Department of Chemistry – sequence: 7 givenname: Mozhen orcidid: 0000-0003-2408-1805 surname: Wang fullname: Wang, Mozhen email: pstwmz@ustc.edu.cn organization: Department of Polymer Science and Engineering – sequence: 8 givenname: Xuewu surname: Ge fullname: Ge, Xuewu organization: Department of Polymer Science and Engineering – sequence: 9 givenname: Yadong orcidid: 0000-0003-0218-3042 surname: Yin fullname: Yin, Yadong email: yadong.yin@ucr.edu organization: Department of Chemistry |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30561210$$D View this record in MEDLINE/PubMed |
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