High-Performance Energy Storage and Conversion Materials Derived from a Single Metal–Organic Framework/Graphene Aerogel Composite
Metal oxides and carbon-based materials are the most promising electrode materials for a wide range of low-cost and highly efficient energy storage and conversion devices. Creating unique nanostructures of metal oxides and carbon materials is imperative to the development of a new generation of elec...
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| Published in | Nano letters Vol. 17; no. 5; pp. 2788 - 2795 |
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| Main Authors | , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
10.05.2017
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Metal oxides and carbon-based materials are the most promising electrode materials for a wide range of low-cost and highly efficient energy storage and conversion devices. Creating unique nanostructures of metal oxides and carbon materials is imperative to the development of a new generation of electrodes with high energy and power density. Here we report our findings in the development of a novel graphene aerogel assisted method for preparation of metal oxide nanoparticles (NPs) derived from bulk MOFs (Co-based MOF, Co(mIM)2 (mIM = 2-methylimidazole). The presence of cobalt oxide (CoO x ) hollow NPs with a uniform size of 35 nm monodispersed in N-doped graphene aerogels (NG-A) was confirmed by microscopic analyses. The evolved structure (denoted as CoO x /NG-A) served as a robust Pt-free electrocatalyst with excellent activity for the oxygen reduction reaction (ORR) in an alkaline electrolyte solution. In addition, when Co was removed, the resulting nitrogen-rich porous carbon–graphene composite electrode (denoted as C/NG-A) displayed exceptional capacitance and rate capability in a supercapacitor. Further, this method is readily applicable to creation of functional metal oxide hollow nanoparticles on the surface of other carbon materials such as graphene and carbon nanotubes, providing a good opportunity to tune their physical or chemical activities. |
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| AbstractList | Metal oxides and carbon-based materials are the most promising electrode materials for a wide range of low-cost and highly efficient energy storage and conversion devices. Creating unique nanostructures of metal oxides and carbon materials is imperative to the development of a new generation of electrodes with high energy and power density. Here we report our findings in the development of a novel graphene aerogel assisted method for preparation of metal oxide nanoparticles (NPs) derived from bulk MOFs (Co-based MOF, Co(mIM)2 (mIM = 2-methylimidazole). The presence of cobalt oxide (CoOx) hollow NPs with a uniform size of 35 nm monodispersed in N-doped graphene aerogels (NG-A) was confirmed by microscopic analyses. The evolved structure (denoted as CoOx/NG-A) served as a robust Pt-free electrocatalyst with excellent activity for the oxygen reduction reaction (ORR) in an alkaline electrolyte solution. In addition, when Co was removed, the resulting nitrogen-rich porous carbon-graphene composite electrode (denoted as C/NG-A) displayed exceptional capacitance and rate capability in a supercapacitor. Further, this method is readily applicable to creation of functional metal oxide hollow nanoparticles on the surface of other carbon materials such as graphene and carbon nanotubes, providing a good opportunity to tune their physical or chemical activities.Metal oxides and carbon-based materials are the most promising electrode materials for a wide range of low-cost and highly efficient energy storage and conversion devices. Creating unique nanostructures of metal oxides and carbon materials is imperative to the development of a new generation of electrodes with high energy and power density. Here we report our findings in the development of a novel graphene aerogel assisted method for preparation of metal oxide nanoparticles (NPs) derived from bulk MOFs (Co-based MOF, Co(mIM)2 (mIM = 2-methylimidazole). The presence of cobalt oxide (CoOx) hollow NPs with a uniform size of 35 nm monodispersed in N-doped graphene aerogels (NG-A) was confirmed by microscopic analyses. The evolved structure (denoted as CoOx/NG-A) served as a robust Pt-free electrocatalyst with excellent activity for the oxygen reduction reaction (ORR) in an alkaline electrolyte solution. In addition, when Co was removed, the resulting nitrogen-rich porous carbon-graphene composite electrode (denoted as C/NG-A) displayed exceptional capacitance and rate capability in a supercapacitor. Further, this method is readily applicable to creation of functional metal oxide hollow nanoparticles on the surface of other carbon materials such as graphene and carbon nanotubes, providing a good opportunity to tune their physical or chemical activities. Metal oxides and carbon-based materials are the most promising electrode materials for a wide range of low-cost and highly efficient energy storage and conversion devices. Creating unique nanostructures of metal oxides and carbon materials is imperative to the development of a new generation of electrodes with high energy and power density. Here we report our findings in the development of a novel graphene aerogel assisted method for preparation of metal oxide nanoparticles (NPs) derived from bulk MOFs (Co-based MOF, Co(mIM)2 (mIM = 2-methylimidazole). The presence of cobalt oxide (CoO x ) hollow NPs with a uniform size of 35 nm monodispersed in N-doped graphene aerogels (NG-A) was confirmed by microscopic analyses. The evolved structure (denoted as CoO x /NG-A) served as a robust Pt-free electrocatalyst with excellent activity for the oxygen reduction reaction (ORR) in an alkaline electrolyte solution. In addition, when Co was removed, the resulting nitrogen-rich porous carbon–graphene composite electrode (denoted as C/NG-A) displayed exceptional capacitance and rate capability in a supercapacitor. Further, this method is readily applicable to creation of functional metal oxide hollow nanoparticles on the surface of other carbon materials such as graphene and carbon nanotubes, providing a good opportunity to tune their physical or chemical activities. Metal oxides and carbon-based materials are the most promising electrode materials for a wide range of low-cost and highly efficient energy storage and conversion devices. Creating unique nanostructures of metal oxides and carbon materials is imperative to the development of a new generation of electrodes with high energy and power density. Here we report our findings in the development of a novel graphene aerogel assisted method for preparation of metal oxide nanoparticles (NPs) derived from bulk MOFs (Co-based MOF, Co(mIM) (mIM = 2-methylimidazole). The presence of cobalt oxide (CoO ) hollow NPs with a uniform size of 35 nm monodispersed in N-doped graphene aerogels (NG-A) was confirmed by microscopic analyses. The evolved structure (denoted as CoO /NG-A) served as a robust Pt-free electrocatalyst with excellent activity for the oxygen reduction reaction (ORR) in an alkaline electrolyte solution. In addition, when Co was removed, the resulting nitrogen-rich porous carbon-graphene composite electrode (denoted as C/NG-A) displayed exceptional capacitance and rate capability in a supercapacitor. Further, this method is readily applicable to creation of functional metal oxide hollow nanoparticles on the surface of other carbon materials such as graphene and carbon nanotubes, providing a good opportunity to tune their physical or chemical activities. |
| Author | Xia, Wei Liu, Meilin Dai, Shuge Qiu, Bin Zhang, Qiaobao Dang, Dai Zou, Ruqiang Zhao, Bote Xia, Dingguo Xu, Qiang Qu, Chong Liang, Zibin Jiao, Yang Guo, Wenhan Huang, Xinyu |
| AuthorAffiliation | School of Chemical and Biomolecular Engineering School of Materials Science and Engineering Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Department of Materials Science and Engineering, College of Engineering National Institute of Advanced Industrial Science and Technology (AIST) Georgia Institute of Technology |
| AuthorAffiliation_xml | – name: School of Chemical and Biomolecular Engineering – name: National Institute of Advanced Industrial Science and Technology (AIST) – name: School of Materials Science and Engineering – name: Georgia Institute of Technology – name: Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Department of Materials Science and Engineering, College of Engineering |
| Author_xml | – sequence: 1 givenname: Wei surname: Xia fullname: Xia, Wei organization: Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Department of Materials Science and Engineering, College of Engineering – sequence: 2 givenname: Chong surname: Qu fullname: Qu, Chong organization: School of Materials Science and Engineering – sequence: 3 givenname: Zibin surname: Liang fullname: Liang, Zibin organization: Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Department of Materials Science and Engineering, College of Engineering – sequence: 4 givenname: Bote orcidid: 0000-0003-1236-6862 surname: Zhao fullname: Zhao, Bote organization: School of Materials Science and Engineering – sequence: 5 givenname: Shuge surname: Dai fullname: Dai, Shuge organization: School of Materials Science and Engineering – sequence: 6 givenname: Bin surname: Qiu fullname: Qiu, Bin organization: Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Department of Materials Science and Engineering, College of Engineering – sequence: 7 givenname: Yang surname: Jiao fullname: Jiao, Yang organization: Georgia Institute of Technology – sequence: 8 givenname: Qiaobao surname: Zhang fullname: Zhang, Qiaobao organization: School of Materials Science and Engineering – sequence: 9 givenname: Xinyu surname: Huang fullname: Huang, Xinyu organization: Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Department of Materials Science and Engineering, College of Engineering – sequence: 10 givenname: Wenhan surname: Guo fullname: Guo, Wenhan organization: Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Department of Materials Science and Engineering, College of Engineering – sequence: 11 givenname: Dai surname: Dang fullname: Dang, Dai organization: School of Materials Science and Engineering – sequence: 12 givenname: Ruqiang orcidid: 0000-0003-0456-4615 surname: Zou fullname: Zou, Ruqiang email: rzou@pku.edu.cn organization: Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Department of Materials Science and Engineering, College of Engineering – sequence: 13 givenname: Dingguo orcidid: 0000-0003-2191-236X surname: Xia fullname: Xia, Dingguo email: dgxia@pku.edu.cn organization: Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Department of Materials Science and Engineering, College of Engineering – sequence: 14 givenname: Qiang orcidid: 0000-0001-5385-9650 surname: Xu fullname: Xu, Qiang email: q.xu@aist.go.jp organization: National Institute of Advanced Industrial Science and Technology (AIST) – sequence: 15 givenname: Meilin orcidid: 0000-0002-6188-2372 surname: Liu fullname: Liu, Meilin email: meilin.liu@mse.gatech.edu organization: School of Materials Science and Engineering |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28394621$$D View this record in MEDLINE/PubMed |
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