Facile Synthesis of Surfactant-Free Au Cluster/Graphene Hybrids for High-Performance Oxygen Reduction Reaction
Non-Pt noble metal clusters like Au clusters are believed to be promising high performance catalysts for the oxygen reduction reaction (ORR) at the cathode of fuel cells, but they still suffer big problems during the catalysis reactions, such as a large amount of the capping agents being on the surf...
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| Published in | ACS nano Vol. 6; no. 9; pp. 8288 - 8297 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
25.09.2012
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1936-0851 1936-086X 1936-086X |
| DOI | 10.1021/nn302984x |
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| Abstract | Non-Pt noble metal clusters like Au clusters are believed to be promising high performance catalysts for the oxygen reduction reaction (ORR) at the cathode of fuel cells, but they still suffer big problems during the catalysis reactions, such as a large amount of the capping agents being on the surface and easy occurrence of dissolution and aggregation. To overcome these obstacles, here, we present a novel and general strategy to grow ultrafine Au clusters and other metal (Pt, Pd) clusters on the reduced graphene oxide (rGO) sheets without any additional protecting molecule or reductant. Compared with the currently generally adopted nanocatalysts, including commercial Pt/C, rGO sheets, Au nanoparticle/rGO hybrids, and thiol-capped Au clusters of the same sizes, the as-synthesized Au cluster/rGO hybrids display an impressive eletrocatalytic performance toward ORR, for instance, high onset potential, superior methanol tolerance, and excellent stability. |
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| AbstractList | Non-Pt noble metal clusters like Au clusters are believed to be promising high performance catalysts for the oxygen reduction reaction (ORR) at the cathode of fuel cells, but they still suffer big problems during the catalysis reactions, such as a large amount of the capping agents being on the surface and easy occurrence of dissolution and aggregation. To overcome these obstacles, here, we present a novel and general strategy to grow ultrafine Au clusters and other metal (Pt, Pd) clusters on the reduced graphene oxide (rGO) sheets without any additional protecting molecule or reductant. Compared with the currently generally adopted nanocatalysts, including commercial Pt/C, rGO sheets, Au nanoparticle/rGO hybrids, and thiol-capped Au clusters of the same sizes, the as-synthesized Au cluster/rGO hybrids display an impressive eletrocatalytic performance toward ORR, for instance, high onset potential, superior methanol tolerance, and excellent stability. Non-Pt noble metal clusters like Au clusters are believed to be promising high performance catalysts for the oxygen reduction reaction (ORR) at the cathode of fuel cells, but they still suffer big problems during the catalysis reactions, such as a large amount of the capping agents being on the surface and easy occurrence of dissolution and aggregation. To overcome these obstacles, here, we present a novel and general strategy to grow ultrafine Au clusters and other metal (Pt, Pd) clusters on the reduced graphene oxide (rGO) sheets without any additional protecting molecule or reductant. Compared with the currently generally adopted nanocatalysts, including commercial Pt/C, rGO sheets, Au nanoparticle/rGO hybrids, and thiol-capped Au clusters of the same sizes, the as-synthesized Au cluster/rGO hybrids display an impressive eletrocatalytic performance toward ORR, for instance, high onset potential, superior methanol tolerance, and excellent stability.Non-Pt noble metal clusters like Au clusters are believed to be promising high performance catalysts for the oxygen reduction reaction (ORR) at the cathode of fuel cells, but they still suffer big problems during the catalysis reactions, such as a large amount of the capping agents being on the surface and easy occurrence of dissolution and aggregation. To overcome these obstacles, here, we present a novel and general strategy to grow ultrafine Au clusters and other metal (Pt, Pd) clusters on the reduced graphene oxide (rGO) sheets without any additional protecting molecule or reductant. Compared with the currently generally adopted nanocatalysts, including commercial Pt/C, rGO sheets, Au nanoparticle/rGO hybrids, and thiol-capped Au clusters of the same sizes, the as-synthesized Au cluster/rGO hybrids display an impressive eletrocatalytic performance toward ORR, for instance, high onset potential, superior methanol tolerance, and excellent stability. |
| Author | Tang, Zhiyong Gao, Yan Yin, Huajie Tang, Hongjie Wang, Dan |
| AuthorAffiliation | National Center for Nanoscience and Technology Chinese Academy of Sciences |
| AuthorAffiliation_xml | – name: National Center for Nanoscience and Technology – name: Chinese Academy of Sciences |
| Author_xml | – sequence: 1 givenname: Huajie surname: Yin fullname: Yin, Huajie – sequence: 2 givenname: Hongjie surname: Tang fullname: Tang, Hongjie – sequence: 3 givenname: Dan surname: Wang fullname: Wang, Dan – sequence: 4 givenname: Yan surname: Gao fullname: Gao, Yan email: zytang@nanoctr.cn, gaoyan@nanoctr.cn – sequence: 5 givenname: Zhiyong surname: Tang fullname: Tang, Zhiyong email: zytang@nanoctr.cn, gaoyan@nanoctr.cn |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/22931045$$D View this record in MEDLINE/PubMed |
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| Snippet | Non-Pt noble metal clusters like Au clusters are believed to be promising high performance catalysts for the oxygen reduction reaction (ORR) at the cathode of... |
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| SubjectTerms | Catalysis Clusters Crystallization - methods Gold Gold - chemistry Graphene Graphite - chemistry Macromolecular Substances - chemistry Materials Testing Methyl alcohol Molecular Conformation Nanostructure Nanostructures - chemistry Nanostructures - ultrastructure Oxidation-Reduction Oxygen - chemistry Particle Size Platinum Reduction Sheet metal Surface Properties Surface-Active Agents - chemistry |
| Title | Facile Synthesis of Surfactant-Free Au Cluster/Graphene Hybrids for High-Performance Oxygen Reduction Reaction |
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