Adsorption of Carbon Dioxide for Post-combustion Capture: A Review

Aiming at meeting the global goals established for carbon dioxide (CO2) reduction, carbon capture and storage (CCS) plays a key role. In this framework, the adsorption-based CO2 post-combustion capture is considered one of the most promising approaches because it can provide remarkable energy saving...

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Published inEnergy & fuels Vol. 35; no. 16; pp. 12845 - 12868
Main Authors Raganati, Federica, Miccio, Francesco, Ammendola, Paola
Format Journal Article
LanguageEnglish
Published American Chemical Society 19.08.2021
Subjects
absorption
adsorbents
adsorption
carbon dioxide
carbon sequestration
energy
heat
hybrids
temperature
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Abstract Aiming at meeting the global goals established for carbon dioxide (CO2) reduction, carbon capture and storage (CCS) plays a key role. In this framework, the adsorption-based CO2 post-combustion capture is considered one of the most promising approaches because it can provide remarkable energy savings with respect to the standard amine-based absorption capture. To date, most of the research effort has been devoted to the development of novel cutting-edge adsorbent materials with the primary purpose of enhancing the adsorption capacity and lifetime while reducing the heat of adsorption, thus lessening the energetic requirement of the sorbent regeneration. Anyway, other factors, beyond the sorbents, greatly affect the competitiveness of the CO2 capture based on the adsorption route, namely, the gas–solid contacting system, impacting the sorbent utilization efficiency, and the regeneration strategies, determining most of the global CO2 capture costs. This review describes the state-of-the-art and most recent progresses of the adsorption-based CO2 post-combustion capture. In particular, the first section describes the CO2 adsorption performances of different classes of solid sorbents on the basis of the most important evaluation parameters (equilibrium adsorption capacity, multi-cyclic stability, etc.). In the second section, the two main gas–solid contacting systems, i.e., fixed beds and fluidized beds, have been reviewed, pointing out their strengths and limitations. Finally, the third section provides a review on the different regeneration modes (temperature, pressure, or hybrid swings), with a focus on the possible strategies available to limit the energy penalty.
AbstractList Aiming at meeting the global goals established for carbon dioxide (CO₂) reduction, carbon capture and storage (CCS) plays a key role. In this framework, the adsorption-based CO₂ post-combustion capture is considered one of the most promising approaches because it can provide remarkable energy savings with respect to the standard amine-based absorption capture. To date, most of the research effort has been devoted to the development of novel cutting-edge adsorbent materials with the primary purpose of enhancing the adsorption capacity and lifetime while reducing the heat of adsorption, thus lessening the energetic requirement of the sorbent regeneration. Anyway, other factors, beyond the sorbents, greatly affect the competitiveness of the CO₂ capture based on the adsorption route, namely, the gas–solid contacting system, impacting the sorbent utilization efficiency, and the regeneration strategies, determining most of the global CO₂ capture costs. This review describes the state-of-the-art and most recent progresses of the adsorption-based CO₂ post-combustion capture. In particular, the first section describes the CO₂ adsorption performances of different classes of solid sorbents on the basis of the most important evaluation parameters (equilibrium adsorption capacity, multi-cyclic stability, etc.). In the second section, the two main gas–solid contacting systems, i.e., fixed beds and fluidized beds, have been reviewed, pointing out their strengths and limitations. Finally, the third section provides a review on the different regeneration modes (temperature, pressure, or hybrid swings), with a focus on the possible strategies available to limit the energy penalty.
Aiming at meeting the global goals established for carbon dioxide (CO2) reduction, carbon capture and storage (CCS) plays a key role. In this framework, the adsorption-based CO2 post-combustion capture is considered one of the most promising approaches because it can provide remarkable energy savings with respect to the standard amine-based absorption capture. To date, most of the research effort has been devoted to the development of novel cutting-edge adsorbent materials with the primary purpose of enhancing the adsorption capacity and lifetime while reducing the heat of adsorption, thus lessening the energetic requirement of the sorbent regeneration. Anyway, other factors, beyond the sorbents, greatly affect the competitiveness of the CO2 capture based on the adsorption route, namely, the gas–solid contacting system, impacting the sorbent utilization efficiency, and the regeneration strategies, determining most of the global CO2 capture costs. This review describes the state-of-the-art and most recent progresses of the adsorption-based CO2 post-combustion capture. In particular, the first section describes the CO2 adsorption performances of different classes of solid sorbents on the basis of the most important evaluation parameters (equilibrium adsorption capacity, multi-cyclic stability, etc.). In the second section, the two main gas–solid contacting systems, i.e., fixed beds and fluidized beds, have been reviewed, pointing out their strengths and limitations. Finally, the third section provides a review on the different regeneration modes (temperature, pressure, or hybrid swings), with a focus on the possible strategies available to limit the energy penalty.
Author Ammendola, Paola
Raganati, Federica
Miccio, Francesco
AuthorAffiliation Istituto di Scienze e Tecnologie per l’Energia e la Mobilità Sostenibili (STEMS)
Istituto di Scienza e Tecnologia dei Materiali Ceramici (ISTEC)
Consiglio Nazionale delle Ricerche (CNR)
AuthorAffiliation_xml – name: Consiglio Nazionale delle Ricerche (CNR)
– name: Istituto di Scienza e Tecnologia dei Materiali Ceramici (ISTEC)
– name: Istituto di Scienze e Tecnologie per l’Energia e la Mobilità Sostenibili (STEMS)
Author_xml – sequence: 1
  givenname: Federica
  surname: Raganati
  fullname: Raganati, Federica
  organization: Istituto di Scienze e Tecnologie per l’Energia e la Mobilità Sostenibili (STEMS)
– sequence: 2
  givenname: Francesco
  orcidid: 0000-0003-0643-6721
  surname: Miccio
  fullname: Miccio, Francesco
  organization: Consiglio Nazionale delle Ricerche (CNR)
– sequence: 3
  givenname: Paola
  orcidid: 0000-0002-2005-3877
  surname: Ammendola
  fullname: Ammendola, Paola
  email: paola.ammendola@stems.cnr.it
  organization: Istituto di Scienze e Tecnologie per l’Energia e la Mobilità Sostenibili (STEMS)
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Snippet Aiming at meeting the global goals established for carbon dioxide (CO2) reduction, carbon capture and storage (CCS) plays a key role. In this framework, the...
Aiming at meeting the global goals established for carbon dioxide (CO₂) reduction, carbon capture and storage (CCS) plays a key role. In this framework, the...
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SubjectTerms absorption
adsorbents
adsorption
carbon dioxide
carbon sequestration
energy
heat
hybrids
temperature
Title Adsorption of Carbon Dioxide for Post-combustion Capture: A Review
URI http://dx.doi.org/10.1021/acs.energyfuels.1c01618
https://www.proquest.com/docview/2636455970
Volume 35
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