Different Adsorption Behaviors of Methane and Carbon Dioxide in the Isotypic Nanoporous Metal Terephthalates MIL-53 and MIL-47
A distinct step in the isotherm occurs during the adsorption of CO2 on MIL-53 at 304 K. Such behavior is neither observed during the adsorption of CH4 on MIL-53 nor during the adsorption on the isostructural MIL-47. This phenomenon seems to be due to a different mechanism than that of previous adsor...
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| Published in | Journal of the American Chemical Society Vol. 127; no. 39; pp. 13519 - 13521 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Washington, DC
American Chemical Society
05.10.2005
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| Subjects | |
| Online Access | Get full text |
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| Abstract | A distinct step in the isotherm occurs during the adsorption of CO2 on MIL-53 at 304 K. Such behavior is neither observed during the adsorption of CH4 on MIL-53 nor during the adsorption on the isostructural MIL-47. This phenomenon seems to be due to a different mechanism than that of previous adsorption steps on MOF samples. It is suggested that a breathing behavior is induced in MIL-53 during CO2 adsorption. |
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| AbstractList | A distinct step in the isotherm occurs during the adsorption of CO2 on MIL-53 at 304 K. Such behavior is neither observed during the adsorption of CH4 on MIL-53 nor during the adsorption on the isostructural MIL-47. This phenomenon seems to be due to a different mechanism than that of previous adsorption steps on MOF samples. It is suggested that a breathing behavior is induced in MIL-53 during CO2 adsorption. A distinct step in the isotherm occurs during the adsorption of CO2 on MIL-53 at 304 K. Such behavior is neither observed during the adsorption of CH4 on MIL-53 nor during the adsorption on the isostructural MIL-47. This phenomenon seems to be due to a different mechanism than that of previous adsorption steps on MOF samples. It is suggested that a breathing behavior is induced in MIL-53 during CO2 adsorption.A distinct step in the isotherm occurs during the adsorption of CO2 on MIL-53 at 304 K. Such behavior is neither observed during the adsorption of CH4 on MIL-53 nor during the adsorption on the isostructural MIL-47. This phenomenon seems to be due to a different mechanism than that of previous adsorption steps on MOF samples. It is suggested that a breathing behavior is induced in MIL-53 during CO2 adsorption. |
| Author | Bourrelly, Sandrine Llewellyn, Philip L Férey, Gérard Millange, Franck Serre, Christian Loiseau, Thierry |
| Author_xml | – sequence: 1 givenname: Sandrine surname: Bourrelly fullname: Bourrelly, Sandrine – sequence: 2 givenname: Philip L surname: Llewellyn fullname: Llewellyn, Philip L – sequence: 3 givenname: Christian surname: Serre fullname: Serre, Christian – sequence: 4 givenname: Franck surname: Millange fullname: Millange, Franck – sequence: 5 givenname: Thierry surname: Loiseau fullname: Loiseau, Thierry – sequence: 6 givenname: Gérard surname: Férey fullname: Férey, Gérard |
| BackLink | http://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=17165243$$DView record in Pascal Francis https://www.ncbi.nlm.nih.gov/pubmed/16190714$$D View this record in MEDLINE/PubMed |
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| Title | Different Adsorption Behaviors of Methane and Carbon Dioxide in the Isotypic Nanoporous Metal Terephthalates MIL-53 and MIL-47 |
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