Near Field of Strongly Coupled Plasmons: Uncovering Dark Modes
Strongly coupled plasmons in a system of individual gold nanoparticles placed at subnanometer distance to a gold film (nanoparticle-on-plane, NPOP) are investigated using two complementary single particle spectroscopy techniques. Optical scattering spectroscopy exclusively detects plasmon modes that...
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Published in | Nano letters Vol. 12; no. 4; pp. 1885 - 1890 |
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Main Authors | , , , , , |
Format | Journal Article |
Language | English |
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Washington, DC
American Chemical Society
11.04.2012
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Abstract | Strongly coupled plasmons in a system of individual gold nanoparticles placed at subnanometer distance to a gold film (nanoparticle-on-plane, NPOP) are investigated using two complementary single particle spectroscopy techniques. Optical scattering spectroscopy exclusively detects plasmon modes that couple to the far field via their dipole moment (bright modes). By using photoemission electron microscopy (PEEM), we detect in the identical NPOPs near-field modes that do not couple to the scattered far field (dark modes) and are characterized by a strongly enhanced nonlinear electron emission process. To our knowledge, this is the first time that both far- and near-field spectroscopy are carried out for identical individual nanostructures interacting via a subnanometer gap. Strongly resonant electron emission occurs at excitation wavelengths far off-resonant in the scattering spectra. |
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AbstractList | Strongly coupled plasmons in a system of individual gold nanoparticles placed at subnanometer distance to a gold film (nanoparticle-on-plane, NPOP) are investigated using two complementary single particle spectroscopy techniques. Optical scattering spectroscopy exclusively detects plasmon modes that couple to the far field via their dipole moment (bright modes). By using photoemission electron microscopy (PEEM), we detect in the identical NPOPs near-field modes that do not couple to the scattered far field (dark modes) and are characterized by a strongly enhanced nonlinear electron emission process. To our knowledge, this is the first time that both far- and near-field spectroscopy are carried out for identical individual nanostructures interacting via a subnanometer gap. Strongly resonant electron emission occurs at excitation wavelengths far off-resonant in the scattering spectra. |
Author | Mohammadi, Reza Schönhense, Gerd Schertz, Florian Elmers, Hans-Joachim Schmelzeisen, Marcus Kreiter, Maximilian |
AuthorAffiliation | Technische Universität Darmstadt Max-Planck-Institut für Polymerforschung Johannes Gutenberg-Universität |
AuthorAffiliation_xml | – name: Technische Universität Darmstadt – name: Max-Planck-Institut für Polymerforschung – name: Johannes Gutenberg-Universität |
Author_xml | – sequence: 1 givenname: Florian surname: Schertz fullname: Schertz, Florian email: scherfl@uni-mainz.de – sequence: 2 givenname: Marcus surname: Schmelzeisen fullname: Schmelzeisen, Marcus – sequence: 3 givenname: Reza surname: Mohammadi fullname: Mohammadi, Reza – sequence: 4 givenname: Maximilian surname: Kreiter fullname: Kreiter, Maximilian – sequence: 5 givenname: Hans-Joachim surname: Elmers fullname: Elmers, Hans-Joachim – sequence: 6 givenname: Gerd surname: Schönhense fullname: Schönhense, Gerd |
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Keywords | subnanometer gap gap resonance near field dark mode sphere-on-plane Plasmon coupling Thin films Nanoparticles Gold Photoemission Far field Plasmons Dipole moments Electron emission Nanostructures Gallium phosphide Electron microscopy Nanostructured materials |
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Snippet | Strongly coupled plasmons in a system of individual gold nanoparticles placed at subnanometer distance to a gold film (nanoparticle-on-plane, NPOP) are... |
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SubjectTerms | Collective excitations (including excitons, polarons, plasmons and other charge-density excitations) Condensed matter: electronic structure, electrical, magnetic, and optical properties Condensed matter: structure, mechanical and thermal properties Cross-disciplinary physics: materials science; rheology Electron and ion emission by liquids and solids; impact phenomena Electron emission Electronic structure and electrical properties of surfaces, interfaces, thin films and low-dimensional structures Exact sciences and technology Far fields Gold Interfaces, heterostructures, nanostructures Joining Low-dimensional structures (superlattices, quantum well structures, multilayers): structure, and nonelectronic properties Materials science Nanocrystalline materials Nanoscale materials and structures: fabrication and characterization Nanostructure Nonlinearity Photoemission and photoelectron spectra Physics Plasmons Scattering Spectroscopy Surface and interface electron states Surfaces and interfaces; thin films and whiskers (structure and nonelectronic properties) |
Title | Near Field of Strongly Coupled Plasmons: Uncovering Dark Modes |
URI | http://dx.doi.org/10.1021/nl204277y https://www.ncbi.nlm.nih.gov/pubmed/22429148 https://search.proquest.com/docview/1762049414 |
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