Nanostructured Black Phosphorus/Ketjenblack–Multiwalled Carbon Nanotubes Composite as High Performance Anode Material for Sodium-Ion Batteries
Sodium-ion batteries are promising alternatives to lithium-ion batteries for large-scale applications. However, the low capacity and poor rate capability of existing anodes for sodium-ion batteries are bottlenecks for future developments. Here, we report a high performance nanostructured anode mater...
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| Published in | Nano letters Vol. 16; no. 6; pp. 3955 - 3965 |
|---|---|
| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
08.06.2016
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Sodium-ion batteries are promising alternatives to lithium-ion batteries for large-scale applications. However, the low capacity and poor rate capability of existing anodes for sodium-ion batteries are bottlenecks for future developments. Here, we report a high performance nanostructured anode material for sodium-ion batteries that is fabricated by high energy ball milling to form black phosphorus/Ketjenblack–multiwalled carbon nanotubes (BPC) composite. With this strategy, the BPC composite with a high phosphorus content (70 wt %) could deliver a very high initial Coulombic efficiency (>90%) and high specific capacity with excellent cyclability at high rate of charge/discharge (∼1700 mAh g–1 after 100 cycles at 1.3 A g–1 based on the mass of P). In situ electrochemical impedance spectroscopy, synchrotron high energy X-ray diffraction, ex situ small/wide-angle X-ray scattering, high resolution transmission electronic microscopy, and nuclear magnetic resonance were further used to unravel its superior sodium storage performance. The scientific findings gained in this work are expected to serve as a guide for future design on high performance anode material for sodium-ion batteries. |
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| AbstractList | Sodium-ion batteries are promising alternatives to lithium-ion batteries for large-scale applications. However, the low capacity and poor rate capability of existing anodes for sodium-ion batteries are bottlenecks for future developments. Here, we report a high performance nanostructured anode material for sodium-ion batteries that is fabricated by high energy ball milling to form black phosphorus/Ketjenblack-multiwalled carbon nanotubes (BPC) composite. With this strategy, the BPC composite with a high phosphorus content (70 wt %) could deliver a very high initial Coulombic efficiency (>90%) and high specific capacity with excellent cyclability at high rate of charge/discharge (∼1700 mAh g(-1) after 100 cycles at 1.3 A g(-1) based on the mass of P). In situ electrochemical impedance spectroscopy, synchrotron high energy X-ray diffraction, ex situ small/wide-angle X-ray scattering, high resolution transmission electronic microscopy, and nuclear magnetic resonance were further used to unravel its superior sodium storage performance. The scientific findings gained in this work are expected to serve as a guide for future design on high performance anode material for sodium-ion batteries. Sodium-ion batteries are promising alternatives to lithium-ion batteries for large-scale applications. However, the low capacity and poor rate capability of existing anodes for sodium-ion batteries are bottlenecks for future developments. Here, we report a high performance nanostructured anode material for sodium-ion batteries that is fabricated by high energy ball milling to form black phosphorus/Ketjenblack–multiwalled carbon nanotubes (BPC) composite. With this strategy, the BPC composite with a high phosphorus content (70 wt %) could deliver a very high initial Coulombic efficiency (>90%) and high specific capacity with excellent cyclability at high rate of charge/discharge (~1700 mAh g–1 after 100 cycles at 1.3 A g–1 based on the mass of P). In situ electrochemical impedance spectroscopy, synchrotron high energy X-ray diffraction, ex situ small/wide-angle X-ray scattering, high resolution transmission electronic microscopy, and nuclear magnetic resonance were further used to unravel its superior sodium storage performance. The scientific findings gained in this work are expected to serve as a guide for future design on high performance anode material for sodium-ion batteries. |
| Author | Chen, Zonghai Liu, Yuzi Ren, Yang Wu, Xue-Hang Ma, Tianyuan Amine, Khalil Zuo, Xiaobing Zhang, Xiaoyi Xu, Gui-Liang Zhong, Gui-Ming Yang, Yong |
| AuthorAffiliation | Collaborative Innovation Center of Chemistry for Energy Materials, State Key Laboratory Physical Chemistry Solid Surfaces, Department of Chemistry Nanoscience and Technology Division Chemical Sciences and Engineering Division University of Rochester Materials Science Program Argonne National Laboratory Xiamen University X-ray Science Division, Advanced Photon Source |
| AuthorAffiliation_xml | – name: University of Rochester – name: X-ray Science Division, Advanced Photon Source – name: Nanoscience and Technology Division – name: Argonne National Laboratory – name: Materials Science Program – name: Collaborative Innovation Center of Chemistry for Energy Materials, State Key Laboratory Physical Chemistry Solid Surfaces, Department of Chemistry – name: Xiamen University – name: Chemical Sciences and Engineering Division |
| Author_xml | – sequence: 1 givenname: Gui-Liang surname: Xu fullname: Xu, Gui-Liang – sequence: 2 givenname: Zonghai surname: Chen fullname: Chen, Zonghai email: zonghai.chen@anl.gov – sequence: 3 givenname: Gui-Ming surname: Zhong fullname: Zhong, Gui-Ming – sequence: 4 givenname: Yuzi surname: Liu fullname: Liu, Yuzi – sequence: 5 givenname: Yong surname: Yang fullname: Yang, Yong – sequence: 6 givenname: Tianyuan surname: Ma fullname: Ma, Tianyuan – sequence: 7 givenname: Yang surname: Ren fullname: Ren, Yang – sequence: 8 givenname: Xiaobing surname: Zuo fullname: Zuo, Xiaobing – sequence: 9 givenname: Xue-Hang surname: Wu fullname: Wu, Xue-Hang – sequence: 10 givenname: Xiaoyi surname: Zhang fullname: Zhang, Xiaoyi – sequence: 11 givenname: Khalil surname: Amine fullname: Amine, Khalil email: amine@anl.gov |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/27222911$$D View this record in MEDLINE/PubMed https://www.osti.gov/biblio/1390938$$D View this record in Osti.gov |
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| Snippet | Sodium-ion batteries are promising alternatives to lithium-ion batteries for large-scale applications. However, the low capacity and poor rate capability of... |
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| SubjectTerms | anode material ball milling black phosphorus ENERGY STORAGE nanostructured sodiation/de-sodiation Sodium ion batteries |
| Title | Nanostructured Black Phosphorus/Ketjenblack–Multiwalled Carbon Nanotubes Composite as High Performance Anode Material for Sodium-Ion Batteries |
| URI | http://dx.doi.org/10.1021/acs.nanolett.6b01777 https://www.ncbi.nlm.nih.gov/pubmed/27222911 https://www.proquest.com/docview/1795867390 https://www.osti.gov/biblio/1390938 |
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