Surface Plasmon-Driven Water Reduction: Gold Nanoparticle Size Matters
Water reduction under two different visible-light ranges (λ > 400 nm and λ > 435 nm) was investigated in gold-loaded titanium dioxide (Au-TiO2) heterostructures with different sizes of Au nanoparticles (NPs). Our study clearly demonstrates the essential role played by Au NP size in plasmon-dri...
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| Published in | Journal of the American Chemical Society Vol. 136; no. 28; pp. 9842 - 9845 |
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| Main Authors | , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
16.07.2014
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Water reduction under two different visible-light ranges (λ > 400 nm and λ > 435 nm) was investigated in gold-loaded titanium dioxide (Au-TiO2) heterostructures with different sizes of Au nanoparticles (NPs). Our study clearly demonstrates the essential role played by Au NP size in plasmon-driven H2O reduction and reveals two distinct mechanisms to clarify visible-light photocatalytic activity under different excitation conditions. The size of the Au NP governs the efficiency of plasmon-mediated electron transfer and plays a critical role in determining the reduction potentials of the electrons transferred to the TiO2 conduction band. Our discovery provides a facile method of manipulating photocatalytic activity simply by varying the Au NP size and is expected to greatly facilitate the design of suitable plasmonic photocatalysts for solar-to-fuel energy conversion. |
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| AbstractList | Water reduction under two different visible-light ranges (λ > 400 nm and λ > 435 nm) was investigated in gold-loaded titanium dioxide (Au-TiO₂) heterostructures with different sizes of Au nanoparticles (NPs). Our study clearly demonstrates the essential role played by Au NP size in plasmon-driven H₂O reduction and reveals two distinct mechanisms to clarify visible-light photocatalytic activity under different excitation conditions. The size of the Au NP governs the efficiency of plasmon-mediated electron transfer and plays a critical role in determining the reduction potentials of the electrons transferred to the TiO₂ conduction band. Our discovery provides a facile method of manipulating photocatalytic activity simply by varying the Au NP size and is expected to greatly facilitate the design of suitable plasmonic photocatalysts for solar-to-fuel energy conversion. Water reduction under two different visible-light ranges (λ > 400 nm and λ > 435 nm) was investigated in gold-loaded titanium dioxide (Au-TiO2) heterostructures with different sizes of Au nanoparticles (NPs). Our study clearly demonstrates the essential role played by Au NP size in plasmon-driven H2O reduction and reveals two distinct mechanisms to clarify visible-light photocatalytic activity under different excitation conditions. The size of the Au NP governs the efficiency of plasmon-mediated electron transfer and plays a critical role in determining the reduction potentials of the electrons transferred to the TiO2 conduction band. Our discovery provides a facile method of manipulating photocatalytic activity simply by varying the Au NP size and is expected to greatly facilitate the design of suitable plasmonic photocatalysts for solar-to-fuel energy conversion.Water reduction under two different visible-light ranges (λ > 400 nm and λ > 435 nm) was investigated in gold-loaded titanium dioxide (Au-TiO2) heterostructures with different sizes of Au nanoparticles (NPs). Our study clearly demonstrates the essential role played by Au NP size in plasmon-driven H2O reduction and reveals two distinct mechanisms to clarify visible-light photocatalytic activity under different excitation conditions. The size of the Au NP governs the efficiency of plasmon-mediated electron transfer and plays a critical role in determining the reduction potentials of the electrons transferred to the TiO2 conduction band. Our discovery provides a facile method of manipulating photocatalytic activity simply by varying the Au NP size and is expected to greatly facilitate the design of suitable plasmonic photocatalysts for solar-to-fuel energy conversion. Water reduction under two different visible-light ranges (λ > 400 nm and λ > 435 nm) was investigated in gold-loaded titanium dioxide (Au-TiO2) heterostructures with different sizes of Au nanoparticles (NPs). Our study clearly demonstrates the essential role played by Au NP size in plasmon-driven H2O reduction and reveals two distinct mechanisms to clarify visible-light photocatalytic activity under different excitation conditions. The size of the Au NP governs the efficiency of plasmon-mediated electron transfer and plays a critical role in determining the reduction potentials of the electrons transferred to the TiO2 conduction band. Our discovery provides a facile method of manipulating photocatalytic activity simply by varying the Au NP size and is expected to greatly facilitate the design of suitable plasmonic photocatalysts for solar-to-fuel energy conversion. |
| Author | Niu, Wenxin Qian, Kun DuChene, Joseph S Stach, Eric A Wei, Wei David Graham, Jeremy O Su, Dong Qiu, Jingjing Engelhard, Mark H Wang, Yi-Chung Sweeny, Brendan C Johnston-Peck, Aaron C |
| AuthorAffiliation | Department of Chemistry and Center for Nanostructured Electronic Materials Center for Functional Nanomaterials Environmental Molecular Sciences Laboratory University of Florida Brookhaven National Laboratory Pacific Northwest National Laboratory |
| AuthorAffiliation_xml | – name: Center for Functional Nanomaterials – name: Department of Chemistry and Center for Nanostructured Electronic Materials – name: Brookhaven National Laboratory – name: Pacific Northwest National Laboratory – name: University of Florida – name: Environmental Molecular Sciences Laboratory |
| Author_xml | – sequence: 1 givenname: Kun surname: Qian fullname: Qian, Kun organization: University of Florida – sequence: 2 givenname: Brendan C surname: Sweeny fullname: Sweeny, Brendan C organization: University of Florida – sequence: 3 givenname: Aaron C surname: Johnston-Peck fullname: Johnston-Peck, Aaron C organization: Brookhaven National Laboratory – sequence: 4 givenname: Wenxin surname: Niu fullname: Niu, Wenxin organization: University of Florida – sequence: 5 givenname: Jeremy O surname: Graham fullname: Graham, Jeremy O organization: University of Florida – sequence: 6 givenname: Joseph S surname: DuChene fullname: DuChene, Joseph S organization: University of Florida – sequence: 7 givenname: Jingjing surname: Qiu fullname: Qiu, Jingjing organization: University of Florida – sequence: 8 givenname: Yi-Chung surname: Wang fullname: Wang, Yi-Chung organization: University of Florida – sequence: 9 givenname: Mark H surname: Engelhard fullname: Engelhard, Mark H organization: Pacific Northwest National Laboratory – sequence: 10 givenname: Dong surname: Su fullname: Su, Dong organization: Brookhaven National Laboratory – sequence: 11 givenname: Eric A surname: Stach fullname: Stach, Eric A organization: Brookhaven National Laboratory – sequence: 12 givenname: Wei David surname: Wei fullname: Wei, Wei David email: wei@chem.ufl.edu organization: University of Florida |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/24972055$$D View this record in MEDLINE/PubMed |
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| Snippet | Water reduction under two different visible-light ranges (λ > 400 nm and λ > 435 nm) was investigated in gold-loaded titanium dioxide (Au-TiO2)... Water reduction under two different visible-light ranges (λ > 400 nm and λ > 435 nm) was investigated in gold-loaded titanium dioxide (Au-TiO₂)... |
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| SubjectTerms | electron transfer energy conversion gold nanogold photocatalysis photocatalysts titanium dioxide |
| Title | Surface Plasmon-Driven Water Reduction: Gold Nanoparticle Size Matters |
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