Precise Synthesis at the Atomic Scale
Precise synthesis at the atomic scale is a highly desirable and controllable route for the preparation of heterogeneous catalysts with the desired structure and properties, which promotes the rational design of highly efficient catalysts and facilitates the understanding of structure-properties rela...
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| Published in | Precision Chemistry Vol. 1; no. 4; pp. 199 - 225 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
University of Science and Technology of China and American Chemical Society
26.06.2023
American Chemical Society |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Precise synthesis at the atomic scale is a highly desirable and controllable route for the preparation of heterogeneous catalysts with the desired structure and properties, which promotes the rational design of highly efficient catalysts and facilitates the understanding of structure-properties relationship. The precise construction of the active sites of the catalysts provides important opportunities for atomic insight into the correlation between structure and catalytic performance. In this review, the atomic-level tuning strategies for the precise synthesis of heterogeneous catalysts are summarized with the emphasis on the precise control of the structure of active sites, including single atom sites, dual atom sites and complex active sites. Furthermore, we illustrate the crucial role of atomic-level regulation of structure in determining the catalytic performance by providing typical catalysis examples in different reactions. In the end, some perspectives on the further development of precise synthesis of catalysts at the atomic level are presented. |
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| AbstractList | Precise synthesis at the atomic scale is a highly desirable
and
controllable route for the preparation of heterogeneous catalysts
with the desired structure and properties, which promotes the rational
design of highly efficient catalysts and facilitates the understanding
of structure-properties relationship. The precise construction of
the active sites of the catalysts provides important opportunities
for atomic insight into the correlation between structure and catalytic
performance. In this review, the atomic-level tuning strategies for
the precise synthesis of heterogeneous catalysts are summarized with
the emphasis on the precise control of the structure of active sites,
including single atom sites, dual atom sites and complex active sites.
Furthermore, we illustrate the crucial role of atomic-level regulation
of structure in determining the catalytic performance by providing
typical catalysis examples in different reactions. In the end, some
perspectives on the further development of precise synthesis of catalysts
at the atomic level are presented. Precise synthesis at the atomic scale is a highly desirable and controllable route for the preparation of heterogeneous catalysts with the desired structure and properties, which promotes the rational design of highly efficient catalysts and facilitates the understanding of structure-properties relationship. The precise construction of the active sites of the catalysts provides important opportunities for atomic insight into the correlation between structure and catalytic performance. In this review, the atomic-level tuning strategies for the precise synthesis of heterogeneous catalysts are summarized with the emphasis on the precise control of the structure of active sites, including single atom sites, dual atom sites and complex active sites. Furthermore, we illustrate the crucial role of atomic-level regulation of structure in determining the catalytic performance by providing typical catalysis examples in different reactions. In the end, some perspectives on the further development of precise synthesis of catalysts at the atomic level are presented. |
| Author | Ji, Shufang Wang, Dingsheng Jun, Caroline Chen, Yuanjun |
| AuthorAffiliation | Department of Chemistry Department of Electrical and Computer Engineering |
| AuthorAffiliation_xml | – name: Department of Electrical and Computer Engineering – name: Department of Chemistry |
| Author_xml | – sequence: 1 givenname: Shufang surname: Ji fullname: Ji, Shufang email: shufang.ji@utoronto.ca organization: Department of Chemistry – sequence: 2 givenname: Caroline surname: Jun fullname: Jun, Caroline organization: Department of Chemistry – sequence: 3 givenname: Yuanjun surname: Chen fullname: Chen, Yuanjun organization: Department of Electrical and Computer Engineering – sequence: 4 givenname: Dingsheng orcidid: 0000-0003-0074-7633 surname: Wang fullname: Wang, Dingsheng email: wangdingsheng@mail.tsinghua.edu.cn organization: Department of Chemistry |
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| Keywords | active sites heterogeneous catalysts catalysis atomic scale Precise synthesis |
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| Snippet | Precise synthesis at the atomic scale is a highly desirable and controllable route for the preparation of heterogeneous catalysts with the desired structure... Precise synthesis at the atomic scale is a highly desirable and controllable route for the preparation of heterogeneous catalysts with the desired structure... |
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| Title | Precise Synthesis at the Atomic Scale |
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