The role of reactive surface sites and complexation by humic acids in the interaction of clay mineral and iron oxide particles
Aggregation and dispersion of mineral particles spontaneously take place under changing environmental conditions in natural systems. The structure of particle network in soils, the retardation or release of colloidal particles, and their mobility and transport are inherently influenced by natural or...
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| Published in | Organic geochemistry Vol. 35; no. 3; pp. 257 - 267 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article Conference Proceeding |
| Language | English |
| Published |
Oxford
Elsevier Ltd
01.03.2004
Elsevier Science |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0146-6380 1873-5290 |
| DOI | 10.1016/j.orggeochem.2003.11.002 |
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| Abstract | Aggregation and dispersion of mineral particles spontaneously take place under changing environmental conditions in natural systems. The structure of particle network in soils, the retardation or release of colloidal particles, and their mobility and transport are inherently influenced by natural organic matter bound to the mineral matrix. Since the surface properties of clay mineral and metal oxide particles, and the electrified mineral–water interfaces play a major role in formation, structure and strength of aggregates, any surface modification, especially by polyanionic organic complexants such as humic substances, has a significant affect on particle interaction in a mineral assemblage. The permanently and/or conditionally charged clay minerals (montmorillonite and kaolinite) and iron oxides (hematite and magnetite), as known major mineral components in natural waters, were selected for studying their surface charge characteristics and pH dependent interactions. We discuss how the surface charge correlates with particle aggregation through some characteristic examples for homo and heterocoagulation of similar and dissimilar mineral particles under acidic condition (at pH ∼4) in the dilute and concentrated systems studied by means of light scattering and rheology, respectively. The adsorption of a brown coal derived humic acid, and its influence on the surface charge character and particle aggregation of clay and iron oxide particles were also studied in dilute and concentrated suspensions. Humic acids can be bound to the most reactive surface sites of clay and oxide particles, i.e. to
Al
-OH mainly at the edges of clay lamellae, and to
Fe
-OH on iron oxides, in surface complexation reaction, therefore their role in particle aggregation is specific. Relations between surface complexation, surface charge modification, and particle aggregation in pure and mixed montmorillonite–iron oxide systems are explained. |
|---|---|
| AbstractList | Aggregation and dispersion of mineral particles spontaneously take place under changing environmental conditions in natural systems. The structure of particle network in soils, the retardation or release of colloidal particles, and their mobility and transport are inherently influenced by natural organic matter bound to the mineral matrix. Since the surface properties of clay mineral and metal oxide particles, and the electrified mineral–water interfaces play a major role in formation, structure and strength of aggregates, any surface modification, especially by polyanionic organic complexants such as humic substances, has a significant affect on particle interaction in a mineral assemblage. The permanently and/or conditionally charged clay minerals (montmorillonite and kaolinite) and iron oxides (hematite and magnetite), as known major mineral components in natural waters, were selected for studying their surface charge characteristics and pH dependent interactions. We discuss how the surface charge correlates with particle aggregation through some characteristic examples for homo and heterocoagulation of similar and dissimilar mineral particles under acidic condition (at pH ∼4) in the dilute and concentrated systems studied by means of light scattering and rheology, respectively. The adsorption of a brown coal derived humic acid, and its influence on the surface charge character and particle aggregation of clay and iron oxide particles were also studied in dilute and concentrated suspensions. Humic acids can be bound to the most reactive surface sites of clay and oxide particles, i.e. to
Al
-OH mainly at the edges of clay lamellae, and to
Fe
-OH on iron oxides, in surface complexation reaction, therefore their role in particle aggregation is specific. Relations between surface complexation, surface charge modification, and particle aggregation in pure and mixed montmorillonite–iron oxide systems are explained. |
| Author | Klumpp, Erwin Majzik, Andrea Tombácz, Etelka Libor, Zsuzsanna Illés, Erzsébet |
| Author_xml | – sequence: 1 givenname: Etelka surname: Tombácz fullname: Tombácz, Etelka email: tombacz@chem.u-szeged.hu organization: Department of Colloid Chemistry, University of Szeged, Szeged, H-6720, Hungary – sequence: 2 givenname: Zsuzsanna surname: Libor fullname: Libor, Zsuzsanna organization: Department of Colloid Chemistry, University of Szeged, Szeged, H-6720, Hungary – sequence: 3 givenname: Erzsébet surname: Illés fullname: Illés, Erzsébet organization: Department of Colloid Chemistry, University of Szeged, Szeged, H-6720, Hungary – sequence: 4 givenname: Andrea surname: Majzik fullname: Majzik, Andrea organization: Department of Colloid Chemistry, University of Szeged, Szeged, H-6720, Hungary – sequence: 5 givenname: Erwin surname: Klumpp fullname: Klumpp, Erwin organization: Institute of Chemistry and Dynamics of the Geosphere, RCJ, Jülich, D-52425, Germany |
| BackLink | http://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=15645746$$DView record in Pascal Francis |
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| IngestDate | Mon Jul 21 09:16:43 EDT 2025 Tue Jul 01 00:40:59 EDT 2025 Thu Apr 24 23:12:25 EDT 2025 Fri Feb 23 02:30:30 EST 2024 |
| IsPeerReviewed | true |
| IsScholarly | true |
| Issue | 3 |
| Keywords | mobility Chordata oxides kaolinite strength metals aggregation Eutheria networks aggregate mineral assemblages montmorillonite Primates pH sheet silicates silicates Theria particles soils Hominidae Tetrapoda magnetite interfaces rheology iron oxides structures hematite Homo transport smectite mineral waters spinel humic acids Vertebrata Mammalia clay minerals dispersion surface properties |
| Language | English |
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| PublicationDate | 2004-03-00 |
| PublicationDateYYYYMMDD | 2004-03-01 |
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| PublicationTitle | Organic geochemistry |
| PublicationYear | 2004 |
| Publisher | Elsevier Ltd Elsevier Science |
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| Title | The role of reactive surface sites and complexation by humic acids in the interaction of clay mineral and iron oxide particles |
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