Approaching the Intrinsic Properties of Moiré Structures Using Atomic Force Microscopy Ironing
Stacking monolayers of transition metal dichalcogenides (TMDs) has led to the discovery of a plethora of new exotic phenomena, resulting from moiré pattern formation. Due to the atomic thickness and high surface-to-volume ratio of heterostructures, the interfaces play a crucial role. Fluctuations i...
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| Published in | Nano letters Vol. 23; no. 11; pp. 4749 - 4755 |
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| Main Authors | , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
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American Chemical Society
14.06.2023
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| Abstract | Stacking monolayers of transition metal dichalcogenides (TMDs) has led to the discovery of a plethora of new exotic phenomena, resulting from moiré pattern formation. Due to the atomic thickness and high surface-to-volume ratio of heterostructures, the interfaces play a crucial role. Fluctuations in the interlayer distance affect interlayer coupling and moiré effects. Therefore, to access the intrinsic properties of the TMD stack, it is essential to obtain a clean and uniform interface between the layers. Here, we show that this is achieved by ironing with the tip of an atomic force microscope. This post-stacking procedure dramatically improves the homogeneity of the interfaces, which is reflected in the optical response of the interlayer exciton. We demonstrate that ironing improves the layer coupling, enhancing moiré effects and reducing disorder. This is crucial for the investigation of TMD heterostructure physics, which currently suffers from low reproducibility. |
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| AbstractList | Stacking monolayers of transition metal dichalcogenides (TMDs) has led to the discovery of a plethora of new exotic phenomena, resulting from moirépattern formation. Due to the atomic thickness and high surface-to-volume ratio of heterostructures, the interfaces play a crucial role. Fluctuations in the interlayer distance affect interlayer coupling and moiréeffects. Therefore, to access the intrinsic properties of the TMD stack, it is essential to obtain a clean and uniform interface between the layers. Here, we show that this is achieved by ironing with the tip of an atomic force microscope. This post-stacking procedure dramatically improves the homogeneity of the interfaces, which is reflected in the optical response of the interlayer exciton. We demonstrate that ironing improves the layer coupling, enhancing moiréeffects and reducing disorder. This is crucial for the investigation of TMD heterostructure physics, which currently suffers from low reproducibility. Stacking monolayers of transition metal dichalcogenides (TMDs) has led to the discovery of a plethora of new exotic phenomena, resulting from moiré pattern formation. Due to the atomic thickness and high surface-to-volume ratio of heterostructures, the interfaces play a crucial role. Fluctuations in the interlayer distance affect interlayer coupling and moiré effects. Therefore, to access the intrinsic properties of the TMD stack, it is essential to obtain a clean and uniform interface between the layers. Here, we show that this is achieved by ironing with the tip of an atomic force microscope. This post-stacking procedure dramatically improves the homogeneity of the interfaces, which is reflected in the optical response of the interlayer exciton. We demonstrate that ironing improves the layer coupling, enhancing moiré effects and reducing disorder. This is crucial for the investigation of TMD heterostructure physics, which currently suffers from low reproducibility. Stacking monolayers of transition metal dichalcogenides (TMDs) has led to the discovery of a plethora of new exotic phenomena, resulting from moiré pattern formation. Due to the atomic thickness and high surface-to-volume ratio of heterostructures, the interfaces play a crucial role. Fluctuations in the interlayer distance affect interlayer coupling and moiré effects. Therefore, to access the intrinsic properties of the TMD stack, it is essential to obtain a clean and uniform interface between the layers. Here, we show that this is achieved by ironing with the tip of an atomic force microscope. This post-stacking procedure dramatically improves the homogeneity of the interfaces, which is reflected in the optical response of the interlayer exciton. We demonstrate that ironing improves the layer coupling, enhancing moiré effects and reducing disorder. This is crucial for the investigation of TMD heterostructure physics, which currently suffers from low reproducibility. Stacking monolayers of transition metal dichalcogenides (TMDs) has led to the discovery of a plethora of new exotic phenomena, resulting from moiré pattern formation. Due to the atomic thickness and high surface-to-volume ratio of heterostructures, the interfaces play a crucial role. Fluctuations in the interlayer distance affect interlayer coupling and moiré effects. Therefore, to access the intrinsic properties of the TMD stack, it is essential to obtain a clean and uniform interface between the layers. Here, we show that this is achieved by ironing with the tip of an atomic force microscope. This post-stacking procedure dramatically improves the homogeneity of the interfaces, which is reflected in the optical response of the interlayer exciton. We demonstrate that ironing improves the layer coupling, enhancing moiré effects and reducing disorder. This is crucial for the investigation of TMD heterostructure physics, which currently suffers from low reproducibility. |
| Author | Taniguchi, Takashi Maude, Duncan K. Castellanos-Gomez, Andres Baranowski, Michał Munuera, Carmen Dyksik, Mateusz Sokolowski, Nikodem Palai, Swaroop Kumar Surrente, Alessandro Xie, Yong Ciorga, Mariusz Schubert, Alina Watanabe, Kenji Plochocka, Paulina Sánchez Viso, Estrella |
| AuthorAffiliation | International Center for Materials Nanoarchitectonics Research Center for Functional Materials Wrocław University of Science and Technology Laboratoire National des Champs Magnétiques Intenses, EMFL, CNRS UPR 3228 Materials Science Factory Department of Experimental Physics, Faculty of Fundamental Problems of Technology National Institute for Materials Science Université Toulouse |
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| Author_xml | – sequence: 1 givenname: Swaroop Kumar surname: Palai fullname: Palai, Swaroop Kumar organization: Université Toulouse – sequence: 2 givenname: Mateusz orcidid: 0000-0003-4945-8795 surname: Dyksik fullname: Dyksik, Mateusz organization: Wrocław University of Science and Technology – sequence: 3 givenname: Nikodem surname: Sokolowski fullname: Sokolowski, Nikodem organization: Université Toulouse – sequence: 4 givenname: Mariusz surname: Ciorga fullname: Ciorga, Mariusz organization: Wrocław University of Science and Technology – sequence: 5 givenname: Estrella orcidid: 0000-0003-0202-4340 surname: Sánchez Viso fullname: Sánchez Viso, Estrella organization: Materials Science Factory – sequence: 6 givenname: Yong orcidid: 0000-0001-7904-664X surname: Xie fullname: Xie, Yong organization: Materials Science Factory – sequence: 7 givenname: Alina surname: Schubert fullname: Schubert, Alina organization: Materials Science Factory – sequence: 8 givenname: Takashi orcidid: 0000-0002-1467-3105 surname: Taniguchi fullname: Taniguchi, Takashi organization: International Center for Materials Nanoarchitectonics – sequence: 9 givenname: Kenji orcidid: 0000-0003-3701-8119 surname: Watanabe fullname: Watanabe, Kenji organization: National Institute for Materials Science – sequence: 10 givenname: Duncan K. surname: Maude fullname: Maude, Duncan K. organization: Université Toulouse – sequence: 11 givenname: Alessandro orcidid: 0000-0003-4078-4965 surname: Surrente fullname: Surrente, Alessandro organization: Wrocław University of Science and Technology – sequence: 12 givenname: Michał orcidid: 0000-0002-5974-0850 surname: Baranowski fullname: Baranowski, Michał organization: Wrocław University of Science and Technology – sequence: 13 givenname: Andres orcidid: 0000-0002-3384-3405 surname: Castellanos-Gomez fullname: Castellanos-Gomez, Andres organization: Materials Science Factory – sequence: 14 givenname: Carmen surname: Munuera fullname: Munuera, Carmen email: cmunuera@icmm.csic.es organization: Materials Science Factory – sequence: 15 givenname: Paulina orcidid: 0000-0002-4019-6138 surname: Plochocka fullname: Plochocka, Paulina email: paulina.plochocka@lncmi.cnrs.fr organization: Université Toulouse |
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| Keywords | interlayer exciton heterostructures photoluminescence transition metal dichalcogenides atomic force microscopy |
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| Snippet | Stacking monolayers of transition metal dichalcogenides (TMDs) has led to the discovery of a plethora of new exotic phenomena, resulting from moiré pattern... Stacking monolayers of transition metal dichalcogenides (TMDs) has led to the discovery of a plethora of new exotic phenomena, resulting from moiré pattern... Stacking monolayers of transition metal dichalcogenides (TMDs) has led to the discovery of a plethora of new exotic phenomena, resulting from moirépattern... Stacking monolayers of transition metal dichalcogenides (TMDs) has led to the discovery of a plethora of new exotic phenomena, resulting from moiré pattern... |
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| Title | Approaching the Intrinsic Properties of Moiré Structures Using Atomic Force Microscopy Ironing |
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