The impact of sulfate reduction on the distribution of methylmercury in reservoirs in the city of Guiyang

In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs from Guiyang City, The methylmercury (MeHg) concentrations of lake water in the Aha Reservoir were greatly elevated as compared to those of the...

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Published inActa geochimica Vol. 32; no. 1; pp. 104 - 109
Main Authors He, Tianrong, Li, Ting, Yang, Ruidong, Luo, Guangjun, Lang, Xiaofang, An, Yanling, Yan, Haiyu
Format Journal Article
LanguageEnglish
Published Heidelberg SP Science Press 01.03.2013
Springer Nature B.V
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Abstract In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs from Guiyang City, The methylmercury (MeHg) concentrations of lake water in the Aha Reservoir were greatly elevated as compared to those of the Hongfeng and Baihua reser- voirs, which was correlated with its distinctly high SRB abundance, SO42, and S2 concentrations. Among the three reservoirs, however, the highest MeHg was observed in in the top several centimenters of pore water profile in the Hongfeng Reservoir where the lowest S2 in pore water occurred. The distributions of MeHg in lake water and pore water showed the highest methylation potential occurred at water-sediment surface for the Aha Reservoir and the in the top several centimenters of sediments for the Hongfeng Reservoir. It is guessed that the highest mercury methy- lation only occurs at the sites with certain sulfide concentrations.
AbstractList In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs from Guiyang City. The methylmercury (MeHg) concentrations of lake water in the Aha Reservoir were greatly elevated as compared to those of the Hongfeng and Baihua reservoirs, which was correlated with its distinctly high SRB abundance, SO sub(4) super(2-), and S super(2-) concentrations. Among the three reservoirs, however, the highest MeHg was observed in in the top several centimenters of pore water profile in the Hongfeng Reservoir where the lowest S super(2-) in pore water occurred. The distributions of MeHg in lake water and pore water showed the highest methylation potential occurred at water-sediment surface for the Aha Reservoir and the in the top several centimenters of sediments for the Hongfeng Reservoir. It is guessed that the highest mercury methylation only occurs at the sites with certain sulfide concentrations.
In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs from Guiyang City, The methylmercury (MeHg) concentrations of lake water in the Aha Reservoir were greatly elevated as compared to those of the Hongfeng and Baihua reser- voirs, which was correlated with its distinctly high SRB abundance, SO42, and S2 concentrations. Among the three reservoirs, however, the highest MeHg was observed in in the top several centimenters of pore water profile in the Hongfeng Reservoir where the lowest S2 in pore water occurred. The distributions of MeHg in lake water and pore water showed the highest methylation potential occurred at water-sediment surface for the Aha Reservoir and the in the top several centimenters of sediments for the Hongfeng Reservoir. It is guessed that the highest mercury methy- lation only occurs at the sites with certain sulfide concentrations.
In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs from Guiyang City. The methylmercury (MeHg) concentrations of lake water in the Aha Reservoir were greatly elevated as compared to those of the Hongfeng and Baihua reservoirs, which was correlated with its distinctly high SRB abundance, SO^sub 4^ ^sup 2-^, and S^sup 2-^ concentrations. Among the three reservoirs, however, the highest MeHg was observed in in the top several centimenters of pore water profile in the Hongfeng Reservoir where the lowest S^sup 2-^ in pore water occurred. The distributions of MeHg in lake water and pore water showed the highest methylation potential occurred at water-sediment surface for the Aha Reservoir and the in the top several centimenters of sediments for the Hongfeng Reservoir. It is guessed that the highest mercury methylation only occurs at the sites with certain sulfide concentrations.[PUBLICATION ABSTRACT]
In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs from Guiyang City. The methylmercury (MeHg) concentrations of lake water in the Aha Reservoir were greatly elevated as compared to those of the Hongfeng and Baihua reservoirs, which was correlated with its distinctly high SRB abundance, SO 4 2− , and S 2− concentrations. Among the three reservoirs, however, the highest MeHg was observed in in the top several centimenters of pore water profile in the Hongfeng Reservoir where the lowest S 2− in pore water occurred. The distributions of MeHg in lake water and pore water showed the highest methylation potential occurred at water-sediment surface for the Aha Reservoir and the in the top several centimenters of sediments for the Hongfeng Reservoir. It is guessed that the highest mercury methylation only occurs at the sites with certain sulfide concentrations.
Author HE Tianrong LI Ting Yang Ruidong LUO Guangjun LANG Xiaofang An Yanling YAN Haiyu
AuthorAffiliation Key Laboratory of Karst Environment and Geohazard Prevention, Guizhou University, Guiyang 550003, China State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550002, China
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Cites_doi 10.1002/etc.5620090713
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Keywords methylmercury
Hongfeng, Aha and Baihua reservoirs
sulfate reduction
sulfate-reducing bacterium
pore water
Language English
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Notes In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs from Guiyang City, The methylmercury (MeHg) concentrations of lake water in the Aha Reservoir were greatly elevated as compared to those of the Hongfeng and Baihua reser- voirs, which was correlated with its distinctly high SRB abundance, SO42, and S2 concentrations. Among the three reservoirs, however, the highest MeHg was observed in in the top several centimenters of pore water profile in the Hongfeng Reservoir where the lowest S2 in pore water occurred. The distributions of MeHg in lake water and pore water showed the highest methylation potential occurred at water-sediment surface for the Aha Reservoir and the in the top several centimenters of sediments for the Hongfeng Reservoir. It is guessed that the highest mercury methy- lation only occurs at the sites with certain sulfide concentrations.
52-1043/P
sulfate reduction; methylmercury; sulfate-reducing bacterium; pore water; Hongfeng, Aha and Baihua reservoirs
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Snippet In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs...
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StartPage 104
SubjectTerms Earth and Environmental Science
Earth Sciences
Elevated
Geochemistry
Lakes
Limnology
Mercury
Methylation
Methylmercury
Pore water
Porosity
Reservoirs
Sulfate reduction
Sulfates
Sulfides
孔隙水
水浓度
甲基化
甲基汞
硫酸盐还原菌
红枫湖
贵阳市
阿哈水库
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Title The impact of sulfate reduction on the distribution of methylmercury in reservoirs in the city of Guiyang
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