The impact of sulfate reduction on the distribution of methylmercury in reservoirs in the city of Guiyang
In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs from Guiyang City, The methylmercury （MeHg） concentrations of lake water in the Aha Reservoir were greatly elevated as compared to those of the...
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| Published in | Acta geochimica Vol. 32; no. 1; pp. 104 - 109 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Heidelberg
SP Science Press
01.03.2013
Springer Nature B.V |
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| Abstract | In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs from Guiyang City, The methylmercury （MeHg） concentrations of lake water in the Aha Reservoir were greatly elevated as compared to those of the Hongfeng and Baihua reser- voirs, which was correlated with its distinctly high SRB abundance, SO42, and S2 concentrations. Among the three reservoirs, however, the highest MeHg was observed in in the top several centimenters of pore water profile in the Hongfeng Reservoir where the lowest S2 in pore water occurred. The distributions of MeHg in lake water and pore water showed the highest methylation potential occurred at water-sediment surface for the Aha Reservoir and the in the top several centimenters of sediments for the Hongfeng Reservoir. It is guessed that the highest mercury methy- lation only occurs at the sites with certain sulfide concentrations. |
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| AbstractList | In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs from Guiyang City. The methylmercury (MeHg) concentrations of lake water in the Aha Reservoir were greatly elevated as compared to those of the Hongfeng and Baihua reservoirs, which was correlated with its distinctly high SRB abundance, SO sub(4) super(2-), and S super(2-) concentrations. Among the three reservoirs, however, the highest MeHg was observed in in the top several centimenters of pore water profile in the Hongfeng Reservoir where the lowest S super(2-) in pore water occurred. The distributions of MeHg in lake water and pore water showed the highest methylation potential occurred at water-sediment surface for the Aha Reservoir and the in the top several centimenters of sediments for the Hongfeng Reservoir. It is guessed that the highest mercury methylation only occurs at the sites with certain sulfide concentrations. In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs from Guiyang City, The methylmercury （MeHg） concentrations of lake water in the Aha Reservoir were greatly elevated as compared to those of the Hongfeng and Baihua reser- voirs, which was correlated with its distinctly high SRB abundance, SO42, and S2 concentrations. Among the three reservoirs, however, the highest MeHg was observed in in the top several centimenters of pore water profile in the Hongfeng Reservoir where the lowest S2 in pore water occurred. The distributions of MeHg in lake water and pore water showed the highest methylation potential occurred at water-sediment surface for the Aha Reservoir and the in the top several centimenters of sediments for the Hongfeng Reservoir. It is guessed that the highest mercury methy- lation only occurs at the sites with certain sulfide concentrations. In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs from Guiyang City. The methylmercury (MeHg) concentrations of lake water in the Aha Reservoir were greatly elevated as compared to those of the Hongfeng and Baihua reservoirs, which was correlated with its distinctly high SRB abundance, SO^sub 4^ ^sup 2-^, and S^sup 2-^ concentrations. Among the three reservoirs, however, the highest MeHg was observed in in the top several centimenters of pore water profile in the Hongfeng Reservoir where the lowest S^sup 2-^ in pore water occurred. The distributions of MeHg in lake water and pore water showed the highest methylation potential occurred at water-sediment surface for the Aha Reservoir and the in the top several centimenters of sediments for the Hongfeng Reservoir. It is guessed that the highest mercury methylation only occurs at the sites with certain sulfide concentrations.[PUBLICATION ABSTRACT] In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs from Guiyang City. The methylmercury (MeHg) concentrations of lake water in the Aha Reservoir were greatly elevated as compared to those of the Hongfeng and Baihua reservoirs, which was correlated with its distinctly high SRB abundance, SO 4 2− , and S 2− concentrations. Among the three reservoirs, however, the highest MeHg was observed in in the top several centimenters of pore water profile in the Hongfeng Reservoir where the lowest S 2− in pore water occurred. The distributions of MeHg in lake water and pore water showed the highest methylation potential occurred at water-sediment surface for the Aha Reservoir and the in the top several centimenters of sediments for the Hongfeng Reservoir. It is guessed that the highest mercury methylation only occurs at the sites with certain sulfide concentrations. |
| Author | HE Tianrong LI Ting Yang Ruidong LUO Guangjun LANG Xiaofang An Yanling YAN Haiyu |
| AuthorAffiliation | Key Laboratory of Karst Environment and Geohazard Prevention, Guizhou University, Guiyang 550003, China State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550002, China |
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| CitedBy_id | crossref_primary_10_1016_j_chemosphere_2020_126634 |
| Cites_doi | 10.1002/etc.5620090713 10.1021/es9808200 10.1016/0143-148X(86)90031-5 10.1139/f04-205 10.1021/es0496672 10.1016/S0025-326X(00)00193-4 10.1289/ehp.9196159 10.1016/0269-7491(91)90031-Q 10.1021/es040561g 10.1007/BF00542429 10.1128/AEM.66.4.1479-1488.2000 10.1007/BF01189725 |
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| Notes | In this paper, the relationship between sulfate reduction potential and mercury methylation potential was studied in the Aha, Baihua and Hongfeng reservoirs from Guiyang City, The methylmercury （MeHg） concentrations of lake water in the Aha Reservoir were greatly elevated as compared to those of the Hongfeng and Baihua reser- voirs, which was correlated with its distinctly high SRB abundance, SO42, and S2 concentrations. Among the three reservoirs, however, the highest MeHg was observed in in the top several centimenters of pore water profile in the Hongfeng Reservoir where the lowest S2 in pore water occurred. The distributions of MeHg in lake water and pore water showed the highest methylation potential occurred at water-sediment surface for the Aha Reservoir and the in the top several centimenters of sediments for the Hongfeng Reservoir. It is guessed that the highest mercury methy- lation only occurs at the sites with certain sulfide concentrations. 52-1043/P sulfate reduction; methylmercury; sulfate-reducing bacterium; pore water; Hongfeng, Aha and Baihua reservoirs ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
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Berman – volume: 96 start-page: 159 year: 1991 ident: 612_CR7 publication-title: Environ. Health Perspect. doi: 10.1289/ehp.9196159 contributor: fullname: W.F. Fitzgerald – volume-title: Sulfate Reduction and Mercury Methylation Potential in the Sediments of Clear Lake year: 1998 ident: 612_CR11 contributor: fullname: E.E. Mack – volume: 39 start-page: 4747 year: 2005 ident: 612_CR16 publication-title: Environmental Science and Technology. doi: 10.1021/es040561g contributor: fullname: C.J. Watras |
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| SubjectTerms | Earth and Environmental Science Earth Sciences Elevated Geochemistry Lakes Limnology Mercury Methylation Methylmercury Pore water Porosity Reservoirs Sulfate reduction Sulfates Sulfides 孔隙水 水浓度 甲基化 甲基汞 硫酸盐还原菌 红枫湖 贵阳市 阿哈水库 |
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| Title | The impact of sulfate reduction on the distribution of methylmercury in reservoirs in the city of Guiyang |
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