Molybdenum Disulfide Nanosheets Aligned Vertically on Carbonized Silk Fabric as Smart Textile for Wearable Pressure-Sensing and Energy Devices
Flexible electronics have gained considerable research concern due to their wide prospect for health monitoring, soft robotics, and artificial intelligence, wherein flexible pressure sensors are necessary components of wearable devices. It is well known that the synergistic functions and multiscale...
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| Published in | ACS applied materials & interfaces Vol. 12; no. 10; pp. 11825 - 11832 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
11.03.2020
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Flexible electronics have gained considerable research concern due to their wide prospect for health monitoring, soft robotics, and artificial intelligence, wherein flexible pressure sensors are necessary components of wearable devices. It is well known that the synergistic functions and multiscale structures of hybrid materials exert tremendous effects on the performance of flexible devices. Herein, inspired by the unique structure of the faceplate of sunflowers, we construct a hierarchical structure by in situ grown vertically aligned molybdenum disulfide (MoS2) nanosheets on carbonized silk fabric (MoS2/CSilk), which is applied as the sensing material in flexible pressure sensors. The MoS2/CSilk sensor displayed high sensitivity and good stability. We demonstrated its applications in monitoring subtle physiology signals, such as pulse wave and voice vibrations. In addition, it served as electrodes in lithium-ion batteries. The MoS2/CSilk electrode delivered ultrahigh first-cycle discharge and charge capacities of 2895 and 1594 mA h g–1, respectively. The MoS2/CSilk electrode exhibited a high capacity of 810 mA h g–1 with a CE close to 100% even after 300 cycles, suggesting good stability. The excellent overall performances are ascribed to the unique structure of the MoS2/CSilk and the synergistic effect of CSilk and MoS2. The concept and strategy of this work can be extended to the design and fabrication of other multifunctional devices. |
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| AbstractList | Flexible electronics have gained considerable research concern due to their wide prospect for health monitoring, soft robotics, and artificial intelligence, wherein flexible pressure sensors are necessary components of wearable devices. It is well known that the synergistic functions and multiscale structures of hybrid materials exert tremendous effects on the performance of flexible devices. Herein, inspired by the unique structure of the faceplate of sunflowers, we construct a hierarchical structure by in situ grown vertically aligned molybdenum disulfide (MoS
) nanosheets on carbonized silk fabric (MoS
/CSilk), which is applied as the sensing material in flexible pressure sensors. The MoS
/CSilk sensor displayed high sensitivity and good stability. We demonstrated its applications in monitoring subtle physiology signals, such as pulse wave and voice vibrations. In addition, it served as electrodes in lithium-ion batteries. The MoS
/CSilk electrode delivered ultrahigh first-cycle discharge and charge capacities of 2895 and 1594 mA h g
, respectively. The MoS
/CSilk electrode exhibited a high capacity of 810 mA h g
with a CE close to 100% even after 300 cycles, suggesting good stability. The excellent overall performances are ascribed to the unique structure of the MoS
/CSilk and the synergistic effect of CSilk and MoS
. The concept and strategy of this work can be extended to the design and fabrication of other multifunctional devices. Flexible electronics have gained considerable research concern due to their wide prospect for health monitoring, soft robotics, and artificial intelligence, wherein flexible pressure sensors are necessary components of wearable devices. It is well known that the synergistic functions and multiscale structures of hybrid materials exert tremendous effects on the performance of flexible devices. Herein, inspired by the unique structure of the faceplate of sunflowers, we construct a hierarchical structure by in situ grown vertically aligned molybdenum disulfide (MoS2) nanosheets on carbonized silk fabric (MoS2/CSilk), which is applied as the sensing material in flexible pressure sensors. The MoS2/CSilk sensor displayed high sensitivity and good stability. We demonstrated its applications in monitoring subtle physiology signals, such as pulse wave and voice vibrations. In addition, it served as electrodes in lithium-ion batteries. The MoS2/CSilk electrode delivered ultrahigh first-cycle discharge and charge capacities of 2895 and 1594 mA h g-1, respectively. The MoS2/CSilk electrode exhibited a high capacity of 810 mA h g-1 with a CE close to 100% even after 300 cycles, suggesting good stability. The excellent overall performances are ascribed to the unique structure of the MoS2/CSilk and the synergistic effect of CSilk and MoS2. The concept and strategy of this work can be extended to the design and fabrication of other multifunctional devices.Flexible electronics have gained considerable research concern due to their wide prospect for health monitoring, soft robotics, and artificial intelligence, wherein flexible pressure sensors are necessary components of wearable devices. It is well known that the synergistic functions and multiscale structures of hybrid materials exert tremendous effects on the performance of flexible devices. Herein, inspired by the unique structure of the faceplate of sunflowers, we construct a hierarchical structure by in situ grown vertically aligned molybdenum disulfide (MoS2) nanosheets on carbonized silk fabric (MoS2/CSilk), which is applied as the sensing material in flexible pressure sensors. The MoS2/CSilk sensor displayed high sensitivity and good stability. We demonstrated its applications in monitoring subtle physiology signals, such as pulse wave and voice vibrations. In addition, it served as electrodes in lithium-ion batteries. The MoS2/CSilk electrode delivered ultrahigh first-cycle discharge and charge capacities of 2895 and 1594 mA h g-1, respectively. The MoS2/CSilk electrode exhibited a high capacity of 810 mA h g-1 with a CE close to 100% even after 300 cycles, suggesting good stability. The excellent overall performances are ascribed to the unique structure of the MoS2/CSilk and the synergistic effect of CSilk and MoS2. The concept and strategy of this work can be extended to the design and fabrication of other multifunctional devices. Flexible electronics have gained considerable research concern due to their wide prospect for health monitoring, soft robotics, and artificial intelligence, wherein flexible pressure sensors are necessary components of wearable devices. It is well known that the synergistic functions and multiscale structures of hybrid materials exert tremendous effects on the performance of flexible devices. Herein, inspired by the unique structure of the faceplate of sunflowers, we construct a hierarchical structure by in situ grown vertically aligned molybdenum disulfide (MoS₂) nanosheets on carbonized silk fabric (MoS₂/CSilk), which is applied as the sensing material in flexible pressure sensors. The MoS₂/CSilk sensor displayed high sensitivity and good stability. We demonstrated its applications in monitoring subtle physiology signals, such as pulse wave and voice vibrations. In addition, it served as electrodes in lithium-ion batteries. The MoS₂/CSilk electrode delivered ultrahigh first-cycle discharge and charge capacities of 2895 and 1594 mA h g–¹, respectively. The MoS₂/CSilk electrode exhibited a high capacity of 810 mA h g–¹ with a CE close to 100% even after 300 cycles, suggesting good stability. The excellent overall performances are ascribed to the unique structure of the MoS₂/CSilk and the synergistic effect of CSilk and MoS₂. The concept and strategy of this work can be extended to the design and fabrication of other multifunctional devices. Flexible electronics have gained considerable research concern due to their wide prospect for health monitoring, soft robotics, and artificial intelligence, wherein flexible pressure sensors are necessary components of wearable devices. It is well known that the synergistic functions and multiscale structures of hybrid materials exert tremendous effects on the performance of flexible devices. Herein, inspired by the unique structure of the faceplate of sunflowers, we construct a hierarchical structure by in situ grown vertically aligned molybdenum disulfide (MoS2) nanosheets on carbonized silk fabric (MoS2/CSilk), which is applied as the sensing material in flexible pressure sensors. The MoS2/CSilk sensor displayed high sensitivity and good stability. We demonstrated its applications in monitoring subtle physiology signals, such as pulse wave and voice vibrations. In addition, it served as electrodes in lithium-ion batteries. The MoS2/CSilk electrode delivered ultrahigh first-cycle discharge and charge capacities of 2895 and 1594 mA h g–1, respectively. The MoS2/CSilk electrode exhibited a high capacity of 810 mA h g–1 with a CE close to 100% even after 300 cycles, suggesting good stability. The excellent overall performances are ascribed to the unique structure of the MoS2/CSilk and the synergistic effect of CSilk and MoS2. The concept and strategy of this work can be extended to the design and fabrication of other multifunctional devices. |
| Author | Yu, Peng Liang, Xiaoping Wang, Haomin Wang, Huimin Lu, Wangdong Jian, Muqiang Zhang, Yingying |
| AuthorAffiliation | Department of Chemistry, Key Laboratory of Bioorganic Phosphorus Chemistry & Chemical Biology Key Laboratory of Organic Optoelectronics and Molecular Engineering of the Ministry of Education, Department of Chemistry |
| AuthorAffiliation_xml | – name: Key Laboratory of Organic Optoelectronics and Molecular Engineering of the Ministry of Education, Department of Chemistry – name: Department of Chemistry, Key Laboratory of Bioorganic Phosphorus Chemistry & Chemical Biology |
| Author_xml | – sequence: 1 givenname: Wangdong surname: Lu fullname: Lu, Wangdong organization: Key Laboratory of Organic Optoelectronics and Molecular Engineering of the Ministry of Education, Department of Chemistry – sequence: 2 givenname: Peng surname: Yu fullname: Yu, Peng organization: Department of Chemistry, Key Laboratory of Bioorganic Phosphorus Chemistry & Chemical Biology – sequence: 3 givenname: Muqiang surname: Jian fullname: Jian, Muqiang organization: Key Laboratory of Organic Optoelectronics and Molecular Engineering of the Ministry of Education, Department of Chemistry – sequence: 4 givenname: Haomin surname: Wang fullname: Wang, Haomin organization: Key Laboratory of Organic Optoelectronics and Molecular Engineering of the Ministry of Education, Department of Chemistry – sequence: 5 givenname: Huimin surname: Wang fullname: Wang, Huimin organization: Key Laboratory of Organic Optoelectronics and Molecular Engineering of the Ministry of Education, Department of Chemistry – sequence: 6 givenname: Xiaoping orcidid: 0000-0002-2119-1921 surname: Liang fullname: Liang, Xiaoping organization: Key Laboratory of Organic Optoelectronics and Molecular Engineering of the Ministry of Education, Department of Chemistry – sequence: 7 givenname: Yingying orcidid: 0000-0002-8448-3059 surname: Zhang fullname: Zhang, Yingying email: yingyingzhang@tsinghua.edu.cn organization: Key Laboratory of Organic Optoelectronics and Molecular Engineering of the Ministry of Education, Department of Chemistry |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/32054269$$D View this record in MEDLINE/PubMed |
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| Keywords | carbonized silk energy devices hierarchical structures flexible pressure sensors molybdenum disulfide nanosheets |
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| Title | Molybdenum Disulfide Nanosheets Aligned Vertically on Carbonized Silk Fabric as Smart Textile for Wearable Pressure-Sensing and Energy Devices |
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