Highly Ordered Hierarchical Pt and PtNi Nanowire Arrays for Enhanced Electrocatalytic Activity toward Methanol Oxidation

Highly ordered hierarchical Pt and PtNi nanowire arrays were prepared using CdS hierarchical nanowire arrays (HNWAs) as sacrificial templates and demonstrated high electrochemical active surface areas. For the resulting Pt HNWAs sample, the peak current for methanol oxidation at +0.74 V was almost 1...

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Published inACS applied materials & interfaces Vol. 10; no. 11; pp. 9444 - 9450
Main Authors Wang, Changzheng, Zhang, Yang, Zhang, Yajun, Xu, Ping, Feng, Cuimin, Chen, Tao, Guo, Tao, Yang, Fengnan, Wang, Qiang, Wang, Jingxiao, Shi, Mengtong, Fan, Louzhen, Chen, Shaowei
Format Journal Article
LanguageEnglish
Published United States American Chemical Society 21.03.2018
Subjects
anodes
catalysts
electrochemistry
fuel cells
methanol
nanowires
nickel
oxidation
CdS nanoparticles
nanowire arrays
hierarchical nanostructure
methanol oxidation reaction
DMFCs
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Abstract Highly ordered hierarchical Pt and PtNi nanowire arrays were prepared using CdS hierarchical nanowire arrays (HNWAs) as sacrificial templates and demonstrated high electrochemical active surface areas. For the resulting Pt HNWAs sample, the peak current for methanol oxidation at +0.74 V was almost 1 order of magnitude higher than that of Pt solid nanowire arrays prepared in a similar manner but without the use of CdS template, and the addition of a Ni cocatalyst effectively enhanced the tolerance against CO poisoning. The results demonstrated that highly ordered Pt and PtNi HNWAs may be exploited as promising anode catalysts in the application of direct methanol fuel cells.
AbstractList Highly ordered hierarchical Pt and PtNi nanowire arrays were prepared using CdS hierarchical nanowire arrays (HNWAs) as sacrificial templates and demonstrated high electrochemical active surface areas. For the resulting Pt HNWAs sample, the peak current for methanol oxidation at +0.74 V was almost 1 order of magnitude higher than that of Pt solid nanowire arrays prepared in a similar manner but without the use of CdS template, and the addition of a Ni cocatalyst effectively enhanced the tolerance against CO poisoning. The results demonstrated that highly ordered Pt and PtNi HNWAs may be exploited as promising anode catalysts in the application of direct methanol fuel cells.Highly ordered hierarchical Pt and PtNi nanowire arrays were prepared using CdS hierarchical nanowire arrays (HNWAs) as sacrificial templates and demonstrated high electrochemical active surface areas. For the resulting Pt HNWAs sample, the peak current for methanol oxidation at +0.74 V was almost 1 order of magnitude higher than that of Pt solid nanowire arrays prepared in a similar manner but without the use of CdS template, and the addition of a Ni cocatalyst effectively enhanced the tolerance against CO poisoning. The results demonstrated that highly ordered Pt and PtNi HNWAs may be exploited as promising anode catalysts in the application of direct methanol fuel cells.
Highly ordered hierarchical Pt and PtNi nanowire arrays were prepared using CdS hierarchical nanowire arrays (HNWAs) as sacrificial templates and demonstrated high electrochemical active surface areas. For the resulting Pt HNWAs sample, the peak current for methanol oxidation at +0.74 V was almost 1 order of magnitude higher than that of Pt solid nanowire arrays prepared in a similar manner but without the use of CdS template, and the addition of a Ni cocatalyst effectively enhanced the tolerance against CO poisoning. The results demonstrated that highly ordered Pt and PtNi HNWAs may be exploited as promising anode catalysts in the application of direct methanol fuel cells.
Author Chen, Shaowei
Wang, Jingxiao
Zhang, Yajun
Chen, Tao
Wang, Qiang
Shi, Mengtong
Yang, Fengnan
Zhang, Yang
Feng, Cuimin
Wang, Changzheng
Xu, Ping
Fan, Louzhen
Guo, Tao
AuthorAffiliation Department of Chemistry
Chinese Academy of Sciences
Beijing University of Civil Engineering and Architecture
Beijing Normal University
Key Laboratory of Urban Stormwater System and Water Environment, Ministry of Education
Beijing Institute of Nanoenergy and Nanosystems
Department of Chemistry and Biochemistry
University of California
Capital Normal University
Laboratory for Micro-sized Functional Materials, College of Elementary Education
AuthorAffiliation_xml – name: University of California
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– name: Key Laboratory of Urban Stormwater System and Water Environment, Ministry of Education
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– name: Laboratory for Micro-sized Functional Materials, College of Elementary Education
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hierarchical nanostructure
methanol oxidation reaction
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Snippet Highly ordered hierarchical Pt and PtNi nanowire arrays were prepared using CdS hierarchical nanowire arrays (HNWAs) as sacrificial templates and demonstrated...
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SubjectTerms anodes
catalysts
electrochemistry
fuel cells
methanol
nanowires
nickel
oxidation
Title Highly Ordered Hierarchical Pt and PtNi Nanowire Arrays for Enhanced Electrocatalytic Activity toward Methanol Oxidation
URI http://dx.doi.org/10.1021/acsami.7b19727
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