Realizing Efficient Single Organic Molecular White Light-Emitting Diodes from Conformational Isomerization of Quinazoline-Based Emitters
Single pure organic molecular white light emitters (SPOMWLEs) are of significance as a new class of material for white lighting applications; however, few of them are able to emit white electroluminescence from organic light-emitting diodes. Herein, donor−π–acceptor conjugated emitters, 2PQ–PTZ and...
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| Published in | ACS applied materials & interfaces Vol. 12; no. 12; pp. 14233 - 14243 |
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| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
25.03.2020
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| Abstract | Single pure organic molecular white light emitters (SPOMWLEs) are of significance as a new class of material for white lighting applications; however, few of them are able to emit white electroluminescence from organic light-emitting diodes. Herein, donor−π–acceptor conjugated emitters, 2PQ–PTZ and 4PQ–PTZ, were designed and synthesized as SPOMWLEs for white light emission considering the distinct advantages of their conformation isomers. The coexistence of conformational isomers in 2PQ–PTZ, which is the first experimental evidence of the coexisting quasi-axial and quasi-equatorial conformers, provides ideal flexibility to obtain white light emission from their simultaneous and well-separated fluorescence and thermally activated delayed fluorescence. With these remarkable properties, a 2PQ–PTZ-based white light-emitting diode (LED) with a CIE of (0.32, 0.34) and color rendering index (CRI) of 89 is demonstrated. Further, the white organic light-emitting diode (OLED) of 2PQ–PTZ exhibits a high external quantum efficiency (EQE) of 10.1%, which is the reported highest performance among SPOMWLE-based OLEDs. |
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| AbstractList | Single pure organic molecular white light emitters (SPOMWLEs) are of significance as a new class of material for white lighting applications; however, few of them are able to emit white electroluminescence from organic light-emitting diodes. Herein, donor−π–acceptor conjugated emitters, 2PQ–PTZ and 4PQ–PTZ, were designed and synthesized as SPOMWLEs for white light emission considering the distinct advantages of their conformation isomers. The coexistence of conformational isomers in 2PQ–PTZ, which is the first experimental evidence of the coexisting quasi-axial and quasi-equatorial conformers, provides ideal flexibility to obtain white light emission from their simultaneous and well-separated fluorescence and thermally activated delayed fluorescence. With these remarkable properties, a 2PQ–PTZ-based white light-emitting diode (LED) with a CIE of (0.32, 0.34) and color rendering index (CRI) of 89 is demonstrated. Further, the white organic light-emitting diode (OLED) of 2PQ–PTZ exhibits a high external quantum efficiency (EQE) of 10.1%, which is the reported highest performance among SPOMWLE-based OLEDs. Single pure organic molecular white light emitters (SPOMWLEs) are of significance as a new class of material for white lighting applications; however, few of them are able to emit white electroluminescence from organic light-emitting diodes. Herein, donor-π-acceptor conjugated emitters, 2PQ-PTZ and 4PQ-PTZ, were designed and synthesized as SPOMWLEs for white light emission considering the distinct advantages of their conformation isomers. The coexistence of conformational isomers in 2PQ-PTZ, which is the first experimental evidence of the coexisting quasi-axial and quasi-equatorial conformers, provides ideal flexibility to obtain white light emission from their simultaneous and well-separated fluorescence and thermally activated delayed fluorescence. With these remarkable properties, a 2PQ-PTZ-based white light-emitting diode (LED) with a CIE of (0.32, 0.34) and color rendering index (CRI) of 89 is demonstrated. Further, the white organic light-emitting diode (OLED) of 2PQ-PTZ exhibits a high external quantum efficiency (EQE) of 10.1%, which is the reported highest performance among SPOMWLE-based OLEDs.Single pure organic molecular white light emitters (SPOMWLEs) are of significance as a new class of material for white lighting applications; however, few of them are able to emit white electroluminescence from organic light-emitting diodes. Herein, donor-π-acceptor conjugated emitters, 2PQ-PTZ and 4PQ-PTZ, were designed and synthesized as SPOMWLEs for white light emission considering the distinct advantages of their conformation isomers. The coexistence of conformational isomers in 2PQ-PTZ, which is the first experimental evidence of the coexisting quasi-axial and quasi-equatorial conformers, provides ideal flexibility to obtain white light emission from their simultaneous and well-separated fluorescence and thermally activated delayed fluorescence. With these remarkable properties, a 2PQ-PTZ-based white light-emitting diode (LED) with a CIE of (0.32, 0.34) and color rendering index (CRI) of 89 is demonstrated. Further, the white organic light-emitting diode (OLED) of 2PQ-PTZ exhibits a high external quantum efficiency (EQE) of 10.1%, which is the reported highest performance among SPOMWLE-based OLEDs. Single pure organic molecular white light emitters (SPOMWLEs) are of significance as a new class of material for white lighting applications; however, few of them are able to emit white electroluminescence from organic light-emitting diodes. Herein, donor-π-acceptor conjugated emitters, 2PQ-PTZ and 4PQ-PTZ, were designed and synthesized as SPOMWLEs for white light emission considering the distinct advantages of their conformation isomers. The coexistence of conformational isomers in 2PQ-PTZ, which is the first experimental evidence of the coexisting quasi-axial and quasi-equatorial conformers, provides ideal flexibility to obtain white light emission from their simultaneous and well-separated fluorescence and thermally activated delayed fluorescence. With these remarkable properties, a 2PQ-PTZ-based white light-emitting diode (LED) with a CIE of (0.32, 0.34) and color rendering index (CRI) of 89 is demonstrated. Further, the white organic light-emitting diode (OLED) of 2PQ-PTZ exhibits a high external quantum efficiency (EQE) of 10.1%, which is the reported highest performance among SPOMWLE-based OLEDs. |
| Author | Gao, Shiyong Guo, Fengyun Li, Zhiyi Jiang, Xi Zhao, Liancheng Wang, Ying Li, Bowen Song, Jinsheng Wang, Jinzhong Pang, Xinchang Zhang, Yong |
| AuthorAffiliation | Key Laboratory of Photochemical Conversion and Optoelectronic Materials School of Materials Science and Engineering Engineering Research Center for Nanomaterials University of Chinese Academy of Sciences |
| AuthorAffiliation_xml | – name: Key Laboratory of Photochemical Conversion and Optoelectronic Materials – name: Engineering Research Center for Nanomaterials – name: University of Chinese Academy of Sciences – name: School of Materials Science and Engineering |
| Author_xml | – sequence: 1 givenname: Bowen surname: Li fullname: Li, Bowen organization: School of Materials Science and Engineering – sequence: 2 givenname: Zhiyi surname: Li fullname: Li, Zhiyi organization: University of Chinese Academy of Sciences – sequence: 3 givenname: Fengyun surname: Guo fullname: Guo, Fengyun organization: School of Materials Science and Engineering – sequence: 4 givenname: Jinsheng orcidid: 0000-0001-9223-8590 surname: Song fullname: Song, Jinsheng organization: Engineering Research Center for Nanomaterials – sequence: 5 givenname: Xi surname: Jiang fullname: Jiang, Xi organization: School of Materials Science and Engineering – sequence: 6 givenname: Ying orcidid: 0000-0001-6638-8026 surname: Wang fullname: Wang, Ying email: wangy@mail.ipc.ac.cn organization: University of Chinese Academy of Sciences – sequence: 7 givenname: Shiyong surname: Gao fullname: Gao, Shiyong organization: School of Materials Science and Engineering – sequence: 8 givenname: Jinzhong surname: Wang fullname: Wang, Jinzhong organization: School of Materials Science and Engineering – sequence: 9 givenname: Xinchang surname: Pang fullname: Pang, Xinchang organization: School of Materials Science and Engineering – sequence: 10 givenname: Liancheng surname: Zhao fullname: Zhao, Liancheng organization: School of Materials Science and Engineering – sequence: 11 givenname: Yong orcidid: 0000-0002-9587-4039 surname: Zhang fullname: Zhang, Yong email: yongzhang@hit.edu.cn organization: School of Materials Science and Engineering |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/32103662$$D View this record in MEDLINE/PubMed |
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| Title | Realizing Efficient Single Organic Molecular White Light-Emitting Diodes from Conformational Isomerization of Quinazoline-Based Emitters |
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