Development of a Fuel-Based Oil and Gas Inventory of Nitrogen Oxides Emissions

In this study, we develop an alternative Fuel-based Oil and Gas inventory (FOG) of nitrogen oxides (NO x ) from oil and gas production using publicly available fuel use records and emission factors reported in the literature. FOG is compared with the Environmental Protection Agency’s 2014 National E...

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Published inEnvironmental science & technology Vol. 52; no. 17; pp. 10175 - 10185
Main Authors Gorchov Negron, Alan M, McDonald, Brian C, McKeen, Stuart A, Peischl, Jeff, Ahmadov, Ravan, de Gouw, Joost A, Frost, Gregory J, Hastings, Meredith G, Pollack, Ilana B, Ryerson, Thomas B, Thompson, Chelsea, Warneke, Carsten, Trainer, Michael
Format Journal Article
LanguageEnglish
Published United States American Chemical Society 04.09.2018
Subjects
Aircraft
Alternative fuels
Basins
Emission
Emission inventories
Emission measurements
Emissions
Environmental protection
Estimates
Fog
Fuels
Gas production
Gases
Methane
New records
Nitrogen
Nitrogen oxides
Oil and gas production
Oxides
Photochemicals
Reactive nitrogen species
Online AccessGet full text

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Abstract In this study, we develop an alternative Fuel-based Oil and Gas inventory (FOG) of nitrogen oxides (NO x ) from oil and gas production using publicly available fuel use records and emission factors reported in the literature. FOG is compared with the Environmental Protection Agency’s 2014 National Emissions Inventory (NEI) and with new top-down estimates of NO x emissions derived from aircraft and ground-based field measurement campaigns. Compared to our top-down estimates derived in four oil and gas basins (Uinta, UT, Haynesville, TX/LA, Marcellus, PA, and Fayetteville, AR), the NEI overestimates NO x by over a factor of 2 in three out of four basins, while FOG is generally consistent with atmospheric observations. Challenges in estimating oil and gas engine activity, rather than uncertainties in NO x emission factors, may explain gaps between the NEI and top-down emission estimates. Lastly, we find a consistent relationship between reactive odd nitrogen species (NO y ) and ambient methane (CH4) across basins with different geological characteristics and in different stages of production. Future work could leverage this relationship as an additional constraint on CH4 emissions from oil and gas basins.
AbstractList In this study, we develop an alternative Fuel-based Oil and Gas inventory (FOG) of nitrogen oxides (NO ) from oil and gas production using publicly available fuel use records and emission factors reported in the literature. FOG is compared with the Environmental Protection Agency's 2014 National Emissions Inventory (NEI) and with new top-down estimates of NO emissions derived from aircraft and ground-based field measurement campaigns. Compared to our top-down estimates derived in four oil and gas basins (Uinta, UT, Haynesville, TX/LA, Marcellus, PA, and Fayetteville, AR), the NEI overestimates NO by over a factor of 2 in three out of four basins, while FOG is generally consistent with atmospheric observations. Challenges in estimating oil and gas engine activity, rather than uncertainties in NO emission factors, may explain gaps between the NEI and top-down emission estimates. Lastly, we find a consistent relationship between reactive odd nitrogen species (NO ) and ambient methane (CH ) across basins with different geological characteristics and in different stages of production. Future work could leverage this relationship as an additional constraint on CH emissions from oil and gas basins.
In this study, we develop an alternative Fuel-based Oil and Gas inventory (FOG) of nitrogen oxides (NOx) from oil and gas production using publicly available fuel use records and emission factors reported in the literature. FOG is compared with the Environmental Protection Agency’s 2014 National Emissions Inventory (NEI) and with new top-down estimates of NOx emissions derived from aircraft and ground-based field measurement campaigns. Compared to our top-down estimates derived in four oil and gas basins (Uinta, UT, Haynesville, TX/LA, Marcellus, PA, and Fayetteville, AR), the NEI overestimates NOx by over a factor of 2 in three out of four basins, while FOG is generally consistent with atmospheric observations. Challenges in estimating oil and gas engine activity, rather than uncertainties in NOx emission factors, may explain gaps between the NEI and top-down emission estimates. Lastly, we find a consistent relationship between reactive odd nitrogen species (NOy) and ambient methane (CH4) across basins with different geological characteristics and in different stages of production. Future work could leverage this relationship as an additional constraint on CH4 emissions from oil and gas basins.
In this study, we develop an alternative Fuel-based Oil and Gas inventory (FOG) of nitrogen oxides (NO x ) from oil and gas production using publicly available fuel use records and emission factors reported in the literature. FOG is compared with the Environmental Protection Agency’s 2014 National Emissions Inventory (NEI) and with new top-down estimates of NO x emissions derived from aircraft and ground-based field measurement campaigns. Compared to our top-down estimates derived in four oil and gas basins (Uinta, UT, Haynesville, TX/LA, Marcellus, PA, and Fayetteville, AR), the NEI overestimates NO x by over a factor of 2 in three out of four basins, while FOG is generally consistent with atmospheric observations. Challenges in estimating oil and gas engine activity, rather than uncertainties in NO x emission factors, may explain gaps between the NEI and top-down emission estimates. Lastly, we find a consistent relationship between reactive odd nitrogen species (NO y ) and ambient methane (CH4) across basins with different geological characteristics and in different stages of production. Future work could leverage this relationship as an additional constraint on CH4 emissions from oil and gas basins.
Author McKeen, Stuart A
Warneke, Carsten
Trainer, Michael
Gorchov Negron, Alan M
Ahmadov, Ravan
Hastings, Meredith G
de Gouw, Joost A
McDonald, Brian C
Thompson, Chelsea
Peischl, Jeff
Pollack, Ilana B
Frost, Gregory J
Ryerson, Thomas B
AuthorAffiliation Department of Earth, Environmental, and Planetary Sciences
Cooperative Institute for Research in Environmental Sciences
Chemical Sciences Division
Global Systems Division
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Snippet In this study, we develop an alternative Fuel-based Oil and Gas inventory (FOG) of nitrogen oxides (NO x ) from oil and gas production using publicly available...
In this study, we develop an alternative Fuel-based Oil and Gas inventory (FOG) of nitrogen oxides (NO ) from oil and gas production using publicly available...
In this study, we develop an alternative Fuel-based Oil and Gas inventory (FOG) of nitrogen oxides (NOx) from oil and gas production using publicly available...
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SubjectTerms Aircraft
Alternative fuels
Basins
Emission
Emission inventories
Emission measurements
Emissions
Environmental protection
Estimates
Fog
Fuels
Gas production
Gases
Methane
New records
Nitrogen
Nitrogen oxides
Oil and gas production
Oxides
Photochemicals
Reactive nitrogen species
Title Development of a Fuel-Based Oil and Gas Inventory of Nitrogen Oxides Emissions
URI http://dx.doi.org/10.1021/acs.est.8b02245
https://www.ncbi.nlm.nih.gov/pubmed/30071716
https://www.proquest.com/docview/2116628038/abstract/
https://search.proquest.com/docview/2083724215
Volume 52
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